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The ion distribution of electrolytes near interfaces with dielectric contrast has important consequences for electrochemical processes and many other applications. To date, most studies of such systems have focused on geometrically simple…

Soft Condensed Matter · Physics 2018-11-14 Huanxin Wu , Honghao Li , Francisco J. Solis , Monica Olvera de la Cruz , Erik Luijten

We study, using Monte Carlo simulations, the interaction between infinite heterogeneously charged surfaces inside an electrolyte solution. The surfaces are overall neutral with quenched charged domains. An average over the quenched disorder…

Soft Condensed Matter · Physics 2015-08-12 Amin Bakhshandeh , Alexandre P. dos Santos , Alexandre Diehl , Yan Levin

We study the dependence of the surface tension of a fluid interface on the density profile of a third suspended phase. By means of an approximated model for the binary mixture and of a perturbative approach we derive close formulas for the…

Statistical Mechanics · Physics 2021-02-03 Alessio Squarcini , Paolo Malgaretti

In this paper, we study electrostatic properties between two similar or oppositely charged surfaces immersed in an electrolyte solution by using mean-field approach accounting for solvent polarization and non-uniform size effect. Applying a…

Soft Condensed Matter · Physics 2022-02-11 Jun-Sik Sin

Ice-water, water-vapor interfaces and ice surface are studied by molecular dynamics simulations with the SPC/E model of water molecules having the purpose to estimate the profiles of electrostatic potential across the interfaces. We have…

Soft Condensed Matter · Physics 2016-03-08 T. Bryk , A. D. J. Haymet

We examine an electric double layer containing an antagonistic salt in an aqueous mixture, where the cations are small and hydrophilic but the anions are large and hydrophobic. In this situation, a strong coupling arises between the charge…

Soft Condensed Matter · Physics 2017-10-11 Shunsuke Yabunaka , Akira Onuki

Surface fractal dimension Ds is a quantity describing the roughness of pore-solid interface where all interactions between solid matrix and fluid in the pore space occur. Ds also quantifies surface area; the higher the surface fractal…

Geophysics · Physics 2019-09-23 Behzad Ghanbarian

Recent advances in experimental and computational techniques have allowed for an accurate description of the adsorption of ionic liquids on metallic electrodes. It is now well established that they adopt a multi-layered structure, and that…

Materials Science · Physics 2016-03-15 Benjamin Rotenberg , Mathieu Salanne

An ultra-strong photovoltaic effect has recently been reported for electrons trapped on a liquid Helium surface under a microwave excitation tuned at intersubband resonance [D. Konstantinov et. al. : J. Phys. Soc. Jpn. 81, 093601 (2012) ].…

Mesoscale and Nanoscale Physics · Physics 2013-07-24 F. Closa , E. Raphael , A. D. Chepelianskii

The adsorption at the interface between an aqueous solution of several surface-active agents and another fluid (air or oil) phase is addressed theoretically. We derive the kinetic equations from a variation of the interfacial free energy,…

Soft Condensed Matter · Physics 2007-05-23 G. Ariel , H. Diamant , D. Andelman

The wetting of solid surfaces by fluids is a problem of great practical importance that has been extensively studied over the years. Most often, the experimental work has involved measurements of the contact angle made by a liquid on the…

Statistical Mechanics · Physics 2007-05-23 S. Curtarolo , M. J. Bojan , G. Stan , M. W. Cole , W. A. Steele

The variation of energies associated with soft matter interfaces where surface inhomogeneities are present. These energies include the total bending and splay energy, the variable surface tension energy, a coupling energy between the total…

Soft Condensed Matter · Physics 2016-12-02 Prerna Gera , David Salac

Molecular dynamics simulations of aqueous NaCl, KCl, NaI, and KI solutions are used to study the effects of salts on the properties of the liquid/vapor interface. The simulations use the models which include both charge transfer and…

Soft Condensed Matter · Physics 2016-03-24 J. D. Smith , S. W. Rick

We predict the nature (attractive or repulsive) and range (exponentially screened or long-range power law) of the electrostatic interactions of oppositely charged and planar plates as a function of the salt concentration and surface charge…

Soft Condensed Matter · Physics 2012-01-31 Dan Ben-Yaakov , Yoram Burak , David Andelman , S. A. Safran

We study the two dimensional water waves problem with surface tension in the case when there is a non-zero contact angle between the free surface and the bottom. In the presence of surface tension, dissipations take place at the contact…

Analysis of PDEs · Mathematics 2020-04-21 Mei Ming , Chao Wang

We study discrete solvent effects on the interaction of two parallel charged surfaces in ionic aqueous solution. These effects are taken into account by adding a bilinear non-local term to the free energy of Poisson-Boltzmann theory. We…

Soft Condensed Matter · Physics 2009-10-31 Yoram Burak , David Andelman

The concept of the partial osmotic pressure of ions in an electrolyte solution is critically examined. In principle these can be defined by introducing a solvent-permeable wall and measuring the force per unit area which can certainly be…

Soft Condensed Matter · Physics 2022-12-09 Patrick B. Warren

The structure of an aqueous solution of sodium chloride at a planar electrode is investigated by integral equation techniques. With the central force water model the aqueous electrolyte is modelled as a mixture of sodium and chloride ions…

chem-ph · Physics 2009-10-28 M. Vossen , F. Forstmann

We report on the onset of fluid entrainment when a contact line is forced to advance over a dry solid of arbitrary wettability. We show that entrainment occurs at a critical advancing speed beyond which the balance between capillary,…

Soft Condensed Matter · Physics 2015-06-16 Rodrigo Ledesma-Aguilar , Aurora Hernández-Machado , Ignacio Pagonabarraga

We present an analytical model of salt- and water-ion transport across an ion-selective interface based on an assumption of local equilibrium of the water-dissociation reaction. The model yields current-voltage characteristics and curves of…

Fluid Dynamics · Physics 2014-04-18 Christoffer P. Nielsen , Henrik Bruus