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Diamond is studied by path integral molecular dynamics simulations of the atomic nuclei in combination with a tight-binding Hamiltonian to describe its electronic structure and total energy. This approach allows us to quantify the influence…

Materials Science · Physics 2009-11-11 Rafael Ramirez , Carlos P. Herrero , Eduardo R. Hernandez

Motivated by the physics of spin-orbital liquids, we study a model of interacting Dirac fermions on a bilayer honeycomb lattice at half filling, featuring an explicit global SO(3)$\times$U(1) symmetry. Using large-scale auxiliary-field…

Strongly Correlated Electrons · Physics 2022-02-25 Zi Hong Liu , Matthias Vojta , Fakher F. Assaad , Lukas Janssen

In diffusion Monte Carlo (DMC) methods, the nodes (or zeroes) of the trial wave function dictate the magnitude of the fixed-node (FN) error. Within standard DMC implementations, they emanate from short multideterminant expansions,…

Chemical Physics · Physics 2018-05-31 Anthony Scemama , Yann Garniron , Michel Caffarel , Pierre-François Loos

The negatively charged nitrogen-vacancy center in diamond is a prototype photoluminescent point defect spin qubit with promising quantum technology applications, enabled by its efficient optical spin polarization and readout. Its low-lying…

The Diffusion Monte Carlo method with constant number of walkers, also called Stochastic Reconfiguration as well as Sequential Monte Carlo, is a widely used Monte Carlo methodology for computing the ground-state energy and wave function of…

Statistics Theory · Mathematics 2024-12-09 Michel Caffarel , Pierre del Moral , Luc de Montella

Transition metal dichalcogenide superlattices provide an exciting new platform for exploring and understanding a variety of phases of matter. The moir\'e continuum Hamiltonian, of two-dimensional jellium in a modulating potential, provides…

Strongly Correlated Electrons · Physics 2024-02-16 Yubo Yang , Miguel Morales , Shiwei Zhang

A quantum Monte Carlo study of the atomization energies for the G2 set of molecules is presented. Basis size dependence of diffusion Monte Carlo atomization energies is studied with a single determinant Slater-Jastrow trial wavefunction…

Chemical Physics · Physics 2015-06-04 F. R. Petruzielo , Julien Toulouse , C. J. Umrigar

In this comprehensive and detailed study, vacancy-mediated self-diffusion of A- and B-elements in 'triple-defect' B2-ordered ASB(1-S) binaries is simulated by means of a kinetic Monte Carlo (KMC) algorithm involving atomic jumps to…

Materials Science · Physics 2019-10-16 Jan Betlej , Piotr Sowa , Rafal Kozubski , Graeme E. Murch , Irina V. Belova

The dissociation energies of four transition metal dimers are determined using diffusion Monte Carlo. The Jastrow, CI, and molecular orbital parameters of the wave function are both partially and fully optimized with respect to the…

Chemical Physics · Physics 2019-09-06 Jil Ludovicy , Kaveh Haghighi Mood , Arne Lüchow

Dirac semimetals (DSMs), characterized by linear dispersion relations in their electronic band structure, have gained prominence due to their unique topological features and potential applications in electronic devices. Through systematic…

Materials Science · Physics 2026-03-31 Shivendra Kumar Gupta , Nikhilesh Singh , Saurabh Kumar Sen , Poorva Singh

Fixed node diffusion quantum Monte Carlo (FN-DMC) is an increasingly used computational approach for investigating the electronic structure of molecules, solids, and surfaces with controllable accuracy. It stands out among equally accurate…

Computational Physics · Physics 2019-10-03 Andrea Zen , Jan Gerit Brandenburg , Angelos Michaelides , Dario Alfè

We present clear numerical evidence for the coexistence of metallic and insulating dynamical mean field theory(DMFT) solutions in a half-filled single-band Hubbard model with bare semicircular density of states at finite temperatures.…

Strongly Correlated Electrons · Physics 2009-10-31 Jaewook Joo , Viktor Oudovenko

We investigate how the fixed-node diffusion Monte Carlo energy of solids depends on single-particle orbitals used in Slater--Jastrow wave functions. We demonstrate that the dependence can be significant, in particular in the case of 3d…

Materials Science · Physics 2010-09-09 Jindrich Kolorenc , Shuming Hu , Lubos Mitas

We theoretically study the excitation spectrum of a two-dimensional Dirac semimetal in the presence of an incommensurate potential. Such models have been shown to possess magic-angle critical points in the single particle wavefunctions,…

Strongly Correlated Electrons · Physics 2022-11-23 Jinjing Yi , Elio J. König , J. H. Pixley

Silicon telluride (Si2Te3) is a two-dimensional semiconductor with unique structural properties due to the size contrast between Si and Te atoms. A recent experiment shows that the material turns metallic under hydrostatic pressure, while…

Materials Science · Physics 2021-01-11 Romakanta Bhattarai , Xiao Shen

We employ the projector quantum Monte Carlo simulations to study the ground-state properties of the square-lattice SU(4) Hubbard model with a $\pi$ flux per plaquette. In the weak coupling regime, its ground state is in the gapless Dirac…

Quantum Gases · Physics 2018-05-25 Zhichao Zhou , Congjun Wu , Yu Wang

Layered material $\alpha$-RuCl$_3$ has caught wide attention due to its possible realization of Kitaev's spin liquid and its electronic structure that involves the interplay of electron-electron correlations and spin-orbit effects. Several…

Strongly Correlated Electrons · Physics 2022-08-16 Abdulgani Annaberdiyev , Cody A. Melton , Guangming Wang , Lubos Mitas

The neutral silicon--vacancy (SiV$^{0}$) center in diamond combines inversion symmetry with optical emission, making it a robust quantum emitter resilient to stray electric fields. Using first-principles density-functional theory, we…

Quantum Physics · Physics 2026-02-12 Meysam Mohseni , Gergő Thiering , Adam Gali

Diffusion Monte Carlo (DMC) simulations for fermions are becoming the standard to provide high quality reference data in systems that are too large to be investigated via quantum chemical approaches. DMC with the fixed-node approximation…

Chemical Physics · Physics 2016-07-06 Andrea Zen , Sandro Sorella , Michael J. Gillan , Angelos Michaelides , Dario Alfè

The symmetric spin-1/2 Ising-Heisenberg diamond chain with different Land\'e g-factors of Ising and Heisenberg spins is exactly solved by combining the generalized decoration-iteration transformation and transfer-matrix method. The ground…

Statistical Mechanics · Physics 2015-06-23 Lucia Galisova