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Ultrafast stimuli can stabilize metastable states of matter inaccessible by equilibrium means. Establishing the spatiotemporal link between ultrafast excitation and metastability is crucial to understanding these phenomena. Here, we use…

We study the conditions under which and how an imposed cluster of fixed colloidal particles at prescribed positions triggers crystal nucleation from a metastable colloidal fluid. Dynamical density functional theory of freezing and Brownian…

Soft Condensed Matter · Physics 2009-11-13 Sven van Teeffelen , Christos N. Likos , Hartmut Löwen

When calcium titanate crystals are grown from stoichiometric melts, they crystallize in the cubic perovskite structure. Upon cooling to room temperature they undergo subsequent phase transitions to tetragonal and orthorhombic modifications.…

Materials Science · Physics 2018-02-02 Detlef Klimm , Max Schmidt , Nora Wolff , Christo Guguschev , Steffen Ganschow

We present experiments investigating the growth of ice crystals from water vapor in air using a free-fall convection chamber. We measured growth rates at temperatures of -5 C and -10 C as a function of supersaturation at an air pressure…

Materials Science · Physics 2009-12-15 K. G. Libbrecht , H. M. Arnold

Crystallization is a fundamental process in materials science, providing the primary route for the realization of a wide range of new materials. Crystallization rates are also considered to be useful probes of glass-forming ability. At the…

We study a quasi-two-dimensional macroscopic system of magnetic spherical particles settled on a shallow concave dish under a temporally oscillating magnetic field. The system reaches a stationary state where the energy losses from…

Soft Condensed Matter · Physics 2021-10-13 A. Escobar , F. Donado , R. E. Moctezuma , Eric R. Weeks

Control of the crystallization process at the microscopic level makes it possible to generate the nanocrystalline samples with the desired structural and morphological properties, that is of great importance for modern industry. In the…

Materials Science · Physics 2019-03-25 Bulat N. Galimzyanov , Dinar T. Yarullin , Anatolii V. Mokshin

Given the multitude of growth habits, pronounced sensitivity to ambient conditions and wide range of scales involved, snowflake crystals are one of the most challenging systems to model. The present work focuses on the development and…

Fluid Dynamics · Physics 2022-01-26 Q. Tan , S. A. Hosseini , A. Seidel-Morgenstern , D. Thévenin , H. Lorenz

We present observations of the formation of plate-like snow crystals that provide evidence for an edge-enhancing crystal growth instability. This instability arises when the condensation coefficient describing the growth of an ice prism…

Materials Science · Physics 2011-11-14 Kenneth G. Libbrecht

In 1897 Ostwald formulated his step rule for formation of the most stable crystal state for a system with crystal polymorphism. The rule describes the irreversible way a system converts to the crystal with lowest free energy. But in fact…

Chemical Physics · Physics 2016-09-07 Søren Toxvaerd

Based upon kinetic Monte Carlo simulations of crystallization in a simple polymer model we present a new picture of the mechanism by which the thickness of lamellar polymer crystals is constrained to a value close to the minimum…

Condensed Matter · Physics 2007-05-23 Jonathan Doye , Daan Frenkel

We have developed a novel Monte Carlo method for simulating the dynamical evolution of stellar systems in arbitrary geometry. The orbits of stars are followed in a smooth potential represented by a basis-set expansion and perturbed after…

Astrophysics of Galaxies · Physics 2014-12-04 Eugene Vasiliev

Certain models with purely repulsive pair interactions can form cluster crystals with multiply-occupied lattice sites. Simulating these models' equilibrium properties is, however, quite challenging. Here, we develop an expanded…

Soft Condensed Matter · Physics 2015-03-20 Kai Zhang , Patrick Charbonneau

Monte Carlo simulation, experiment and continuum theory are used to examine the anchoring exhibited by a nematic liquid crystal at a patterned substrate comprising a periodic array of rectangles that, respectively, promote vertical and…

Soft Condensed Matter · Physics 2013-08-09 Candy Anquetil-Deck , Douglas J. Cleaver , Jonathan P. Bramble , Timothy J. Atherton

We consider both equilibrium and kinetic aspects of the phase separation (``thermal faceting") of thermodynamically unstable crystal surfaces into a hill--valley structure. The model we study is an Ising lattice gas for a simple cubic…

Condensed Matter · Physics 2009-10-22 Joel D. Shore , Dirk Jan Bukman

The dynamics of the discrete Gaussian model for the surface of a crystal deposited on a disordered substrate is investigated by Monte Carlo simulations. The mobility of the growing surface was studied as a function of a small driving force…

Condensed Matter · Physics 2009-10-28 D. Cule

What are the mechanisms leading to the shape relaxation of three dimensional crystallites ? Kinetic Monte Carlo simulations of fcc clusters show that the usual theories of equilibration, via atomic surface diffusion driven by curvature, are…

Materials Science · Physics 2009-10-31 Nicolas Combe , Pablo Jensen , Alberto Pimpinelli

New charge transfer crystals of $\pi$-conjugated, aromatic molecules (phenanthrene and picene) as donors were obtained by physical vapor transport. The melting behavior, optimization of crystal growth and the crystal structure is reported…

The steady-state homogeneous vapor-to-liquid nucleation and the succeeding liquid droplet growth process are studied for water system by means of the coarse-grained molecular dynamics simulations with the mW-model suggested originally in…

Soft Condensed Matter · Physics 2012-10-03 Anatolii V. Mokshin , Bulat N. Galimzyanov

The growth of quasicrystals, i.e., aperiodic structures with long-range order, seeded from the melt is investigated using a dynamical phase field crystal model. Depending on the thermodynamic conditions, two different growth modes are…

Soft Condensed Matter · Physics 2014-07-31 C. V. Achim , M. Schmiedeberg , H. Löwen