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Quantum coherent control of ultrafast bond making and the subsequent molecular dynamics is crucial for the realization of a new photochemistry, where a shaped laser field is actively driving the chemical system in a coherent way from the…
Understanding and controlling the electronic as well as ro-vibrational motion and, thus, the entire chemical dynamics in molecules is the ultimate goal of ultrafast laser and imaging science. In photochemistry, laser-induced dissociation…
To date X-ray spectroscopy has become a routine tool that can reveal highly local and element-specific information on the electronic structure of atoms in complex environments. Here, we focus on nuclear dynamical effects in X-ray spectra…
A highly asymmetric dynamic nuclear spin pumping is observed in a single self assembled InGaAs quantum dot subject to resonant optical pumping of the neutral exciton transition leading to a large maximum polarization of 54%. This dynamic…
We consider the cooperative decay of incoherently pumped atoms in a disordered medium, where light undergoes multiple scattering. It is shown that the cooperation number, which determines the duration and amplitude of superfluorescent…
We propose a method for enacting the unitary time propagation of two interacting neutrons at leading order of chiral effective field theory by efficiently encoding the nuclear dynamics into a single multi-level quantum device. The emulated…
The effect of collectivity on the loading of an atom laser via optical pumping is discussed. In our model, atoms in a beam are laser-excited and subsequently spontaneously decay into a trapping state. We consider the case of sufficiently…
In recent years, ultrafast pump-probe spectroscopy has provided insightful information about nonequilibrium dynamics of excitations in materials. In a typical experiment of time-resolved x-ray absorption spectroscopy, the systems are…
The precise control and knowledge over the atomic dynamics is central to the advancement of quantum technology. The different experimental conditions namely, atoms in a vacuum, an anti-relaxation coated and a buffer gas filled atomic cell…
Long-lived excited states of atomic nuclei can act as energy traps. These states, known as nuclear isomers, can store a large amount of energy over long periods of time, with a very high energy-to-mass ratio. Under natural conditions, the…
We analyze the optically driven dynamics of a qubit implemented on a singlet-triplet subspace of two-electron states in a self-assembled quantum dot molecule. We study two possible control schemes based on the coupling to an excited…
We study the quantum dynamics of N coherently driven two-level atoms coupled to an optical resonator. In the strong coupling regime the cavity field generated by atomic scattering interferes destructively with the pump on the atoms. This…
Cooperative spontaneous emission of a single photon from a cloud of N atoms modifies substantially the radiation pressure exerted by a far-detuned laser beam exciting the atoms. On one hand, the force induced by photon absorption depends on…
We explore the coherent dynamics of a three-level V-system interacting with a thermal bath in the regime where thermal excitation occurs much faster than spontaneous decay. We present analytic solutions of the Bloch-Redfield quantum master…
We investigate the performance of dynamical decoupling methods at suppressing electron spin decoherence from a low-temperature nuclear spin reservoir in a quantum dot. The controlled dynamics is studied through exact numerical simulation,…
The collective atomic recoil lasing is studied for an ultra-cold and collisionless atomic gas in a partially coherent pump with a colored noise. Compared to white noise, correlations in colored noise are found to be able to greatly enhance…
An excited emitter decays by radiating a photon into a quantized mode of the electromagnetic field, a process known as spontaneous emission. If the emitter is driven to a higher excited state, it radiates multiple photons in a cascade…
Nuclear coherent population transfer (NCPT) plays an important role in the exploration and application of atomic nuclei. How to achieve high-fidelity NCPT remains so far challenging. Here, we investigate the complete population transfer of…
Nuclear polarization dynamics are measured in the nuclear spin bi-stability regime in a single optically pumped InGaAs/GaAs quantum dot. The controlling role of nuclear spin diffusion from the dot into the surrounding material is revealed…
Within the framework of master equation, we study decay dynamics of an atom-molecule system strongly coupled by two photoassociation lasers. Summing over the infinite number of electromagnetic vacuum modes that are coupled to the…