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We demonstrate for the first time natural phase matching for optical frequency doubling in a high-Q whispering gallery mode resonator made of Lithium Niobate. A conversion efficiency of 9% is achieved at 30 micro Watt in-coupled continuous…

We observe enhanced second-harmonic generation in monolayer graphene in the presence of an ultra-strong terahertz field pulse with a peak amplitude of 250 kV/cm. This is a strongly nonperturbative regime of light-matter interaction in which…

We demonstrate the simultaneous generation of second and third harmonic signals from a telecom wavelength pump in a gallium phosphide (GaP) microdisk. Using analysis of the power scaling of both the second and third harmonic outputs and…

Second-harmonic generation (SHG) is a direct measure of the strength of second-order nonlinear optical effects, which also include frequency mixing and parametric oscillations. Natural and artificial materials with broken…

The 4-bar crystal symmetry in materials such as GaAs can enable quasi-phasematching for efficient frequency conversion without poling, twinning or other engineered domain inversions. 4-bar symmetry means that a 90 degree rotation is…

Mesoscale and Nanoscale Physics · Physics 2012-10-09 Paulina S. Kuo , Glenn S. Solomon

While two-dimensional (2D) materials have intriguing second-order nonlinearities with ultrahigh coefficient and electrical tunability, their atomic layer thicknesses hinder explorations of other optical frequency-conversions (OFCs) than…

We derive general conditions for 100 percent frequency conversion in any doubly resonant nonlinear cavity, for both second- and third-harmonic generation via chi2 and chi3 nonlinearities. We find that conversion efficiency is optimized for…

We report on double-resonant highly efficient sum-frequency generation in the blue range. The system consists of a 10-mm-long periodically poled KTP crystal placed in a double-resonant bow-tie cavity and pumped by a fiber laser at 1064.5 nm…

Second harmonic generation in nonlinear materials can be greatly enhanced by realizing doubly-resonant cavities with high quality factors. However, fulfilling such doubly resonant condition in photonic crystal (PhC) cavities is a…

We demonstrate a new, nonlinear optical effect of electric currents. First, a steady current is generated by applying a voltage on a doped GaAs crystal. We demonstrate that this current induces second-harmonic generation of a probe laser…

Materials Science · Physics 2015-06-03 Brian A. Ruzicka , Lalani K. Werake , Guowei Xu , Jacob B. Khurgin , E. Ya. Sherman , Judy Z. Wu , Hui Zhao

Here we employ the quasi-bound state in the continuum (quasi-BIC) resonance in all-dielectric metasurfaces for efficient nonlinear processes in consideration of the backward frequency conversion. We theoretically study the second-harmonic…

Optics · Physics 2024-06-28 Xu Tu , Siqi Feng , Jiajun Li , Yangguang Xing , Feng Wu , Tingting Liu , Shuyuan Xiao

Second-harmonic generation is of paramount importance in several fields of science and technology, including frequency conversion, self-referencing of frequency combs, nonlinear spectroscopy and pulse characterization. Advanced…

We investigate the effects of a squeezed pump on the quantum properties and conversion efficiency of the light produced in single-pass second harmonic generation. Using stochastic integration of the two-mode equations of motion in the…

Quantum Physics · Physics 2015-06-15 E. MArcellina , J. F. Corney , M. K. Olsen

Improving the conversion efficiency is critical for advancing nonlinear photonic devices, enabling applications in ultrafast optics, quantum light sources, and high-resolution imaging. Herein, we present a bilayer waveguide integrated with…

Optics · Physics 2025-08-21 Xin Huang , Qi Lin , Sheng-Xuan Xia , Xiang Zhai , Gui-Dong Liu

We show that the lack of inversion symmetry in monolayer MoS2 allows strong optical second harmonic generation. Second harmonic of an 810-nm pulse is generated in a mechanically exfoliated monolayer, with a nonlinear susceptibility on the…

Materials Science · Physics 2015-06-15 Nardeep Kumar , Sina Najmaei , Qiannan Cui , Frank Ceballos , Pulickel M. Ajayan , Jun Lou , Hui Zhao

We report on theoretical study of second-harmonic generation (SHG) in plasmonic nanostructures interacting with two-level quantum emitters (QE) under incoherent energy pump. We generalize driven-dissipative Tavis-Cummings model by…

Optics · Physics 2021-03-17 Maxim Sukharev , Oleksiy Roslyak , Andrei Piryatinski

We report on the observation of high efficiency frequency doubling of 1550 nm continuous-wave laser light in a nonlinear cavity containing a periodically poled potassium titanyl phosphate crystal (PPKTP). The fundamental field had a power…

The effective second-harmonic generation (SHG) coefficient is a crucial data that quantifies the efficiency of transforming fundamental frequency light into its second harmonic. With the help of the symmetry of nonlinear optical…

Optimization and Control · Mathematics 2026-02-24 Die Xiao , Yisheng Song

Plasmonic nanocavities have proven to be a powerful optical platform for confining light at a length scale much smaller than the diffraction limit. Enhanced electromagnetic fields within the cavity mode volume enable multiple significant…

The effect of slow light on second harmonic generation in a periodically poled $\chi^{(2)}$ nonlinear medium is investigated theoretically. A linear $\pi$ phase shifted grating is used to slow the group velocity of the fundamental frequency…

Optics · Physics 2022-02-02 Thomas E. Maybour , Devin H. Smith , Peter Horak