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The characteristics of intrinsic defects are important for the understanding of self-diffusion processes, mechanical strength, brittleness, and plasticity of tungsten carbide, which present in the divertor of fusion reactors. Here, we use…

Materials Science · Physics 2015-05-19 Xiang-Shan Kong , Yu-Wei You , J. H. Xia , C. S. Liu , Q. F. Fang , G. -N. Luo , Qun-Ying Huang

The different point defects formed by two hydrogen atoms or two helium atoms in tungsten were investigated through first-principles calculation. The energetically favorable site for a hydrogen atom is tetrahedral interstitial site while…

Materials Science · Physics 2017-10-16 Qiang Zhao , Zheng Zhang , Yang Li , Xiao-Ping Ouyang

The behaviors of hydrogen (H) in MAX phase material Ti3SiC2 have been investigated using first-principles method. We show that a single H atom prefers to stay 1.01 {\AA} down of the Si vacancy with solution energy of about -4.07 eV,…

Materials Science · Physics 2013-08-06 Yi-Guo Xu , Xue-Dong Ou , Xi-Ming Rong

The existence of intrinsic vacancies in cubic (monoclinic) TiO suggests opportunity for hydrogen absorption, which was addressed in recent experiments. In the present work, based on first principle calculations, the preferences are studied…

Materials Science · Physics 2023-08-01 S. Vahid Hosseini , Andrei Postnikov , Mohammad Reza Mohammadizadeh

We examine the behaviour of hydrogen ions, atoms and molecules in alpha-boron using density functional calculations. Hydrogen behaves as a negative-U centre, with positive H ions preferring to sit off-center on inter-layer bonds and…

We have studied the fundamental process of hydrogen binding at interstitial, vacancy and grain boundary (GB) in palladium crystals using Density-Functional Theory. It showed that hydrogen prefers to occupy the octahedral interstitial site…

Materials Science · Physics 2015-06-02 Hieu H. Pham , Tahir Cagin

Interaction between hydrogen (H) and metals is central to many materials problems of scientific and technological importance. Chief among them is the development of H storage and H-resistant materials. H segregation or trapping at lattice…

Materials Science · Physics 2013-11-06 Weiwei Xing , Xing-Qiu Chen , Gang Lu , Dianzhong Li , Yiyi Li

We performed molecular dynamics simulations of coalescence of two vacancies in a tungsten (W) crystal to elucidate the effect of temperature and hydrogen atoms. Simulations were performed for two types of vacancy structures, $\mathrm{V}_9 +…

Materials Science · Physics 2024-07-03 Sotaro Tsuru , Hiroaki Nakamura , Yuki Goto , Miyuki Yajima , Seiki Saito , Shunsuke Usami

Adsorption of hydrogen atoms to a carbon atom vacancy in graphene is investigated by means of periodic \emph{first principles} calculations, up to the fully hydrogenated state where six H atoms chemically bind to the vacancy. Addition of a…

Materials Science · Physics 2013-12-30 M. Casartelli , S. Casolo , G. F. Tantardini , R. Martinazzo

In a recent Letter Scanlon and Watson reported their first principles results on hydrogen in Cu2O. Their main conclusions are: (1) an interstitial H in Cu2O prefers to occupy the tetrahedral site, which is coordinated with four Cu cations,…

Materials Science · Physics 2011-12-22 K. Biswas , M. -H. Du , J. T. -Thienprasert , S. Limpijumnong , D. J. Singh

Properties of point defects resulting from the incorporation of inert-gas atoms in bcc tungsten are investigated systematically using first-principles density functional theory (DFT) calculations. The most stable configuration for the…

Materials Science · Physics 2015-10-29 Duc Nguyen-Manh , S. L. Dudarev

In this work, we combine Density Functional Theory data with a Thermodynamic and a kinetic model to determine the total concentration of hydrogen implanted in the sub-surface of tungsten exposed to a hydrogen flux. The sub-surface hydrogen…

Materials Science · Physics 2019-04-30 E. Hodille , N Fernandez , Z. Piazza , M. Ajmalghan , Y. Ferro

Absorption of hydrogen molecules on Nickel and Rhodium doped hexagonal boron nitride(BN) sheet is investigated by using the first principle method. The most stable site for the Ni atom was the on top side of nitrogen atom, while Rh atoms…

Low-energy hydrogen irradiation is known to induce bubble formation in tungsten, while its atomistic mechanisms remain little understood. Using first-principles calculations and statistical models, we studied the self-clustering behavior of…

Materials Science · Physics 2018-07-11 Jie Hou , Xiang-Shan Kong , Jingjing Sun , Yu-Wei You , Xuebang Wu , C. S. liu , Jun Song

Adsorption of hydrogen atoms on a single graphite sheet (graphene) has been investigated by first-principles electronic structure means, employing plane-wave based, periodic density functional theory. A reasonably large 5x5 surface unit…

Materials Science · Physics 2009-11-13 Simone Casolo , Ole Martin Lovvik , Rocco Martinazzo , Gian Franco Tantardini

The hydrogen dynamics on a graphene sheet is studied in the presence of carbon vacancies. We analyze the motion of atomic H by means of molecular dynamics (MD) simulations, using a tight-binding Hamiltonian fitted to density-functional…

Chemical Physics · Physics 2022-09-29 Carlos P. Herrero , Jose A. Verges , Rafael Ramirez

We describe the parameterization of a tungsten-hydrogen empirical potential designed for use with large-scale molecular dynamics simulations of highly irradiated tungsten containing hydrogen isotope atoms, and report test results.…

An H atom inserted into hydrogen monolayer on the Si(100)-2x1 surface has been studied using the density functional theory. Hydrogen-induced defects were considered in their neutral, negative, and positive charge states. It was found that…

Mesoscale and Nanoscale Physics · Physics 2020-10-28 T. V. Pavlova

The effect of solute hydrogen on the stability of vacancy clusters in hexagonal closed packed zirconium is investigated with an ab initio approach, including contributions of H vibrations. Atomistic simulations within the density functional…

Materials Science · Physics 2015-09-29 Céline Varvenne , Olivier Mackain , Laurent Proville , Emmanuel Clouet

We investigate the effect of hydrogen on the mobility of a screw dislocation in body-centered cubic (bcc) iron using first-principles calculations, and show that an increase of screw dislocation velocity is expected for a limited…

Materials Science · Physics 2013-10-16 M. Itakura , H. Kaburaki , M. Yamaguchi , T. Okita
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