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We report on important influence of single domain wall (DW) of electrically poled ferroelectric crystal on parametric processes via Cherenkov-type phase matching. It shows that the effective nonlinear polarization is confined in DW and its…

Optics · Physics 2010-08-03 Xuewei Deng , Huaijin Ren , Yuanlin Zheng , Xianfeng Chen

Significantly enhanced second order nonlinearity resulting from local symmetry breaking in domain walls is reported. By this new giant nonlinearity, novel hexagonally, conically and trigonally distributed second harmonic beams closely…

Optics · Physics 2010-05-18 Xuewei Deng , Huaijin Ren , Yuanlin Zheng , Kun Liu , Xianfeng Chen

We observe enhanced second-harmonic generation in monolayer graphene in the presence of an ultra-strong terahertz field pulse with a peak amplitude of 250 kV/cm. This is a strongly nonperturbative regime of light-matter interaction in which…

We show that the second harmonic generation (SHG) is enhanced in the chiral one-dimensional electron currents in a broad frequency range. The origin of the enhancement is two-fold: first, the linear dispersion of the current and the…

Mesoscale and Nanoscale Physics · Physics 2020-04-17 Ivan Iorsh , Gulnaz Rakhmanova

Second harmonic generation is a powerful tool directly connected to the symmetry of materials. Phase transitions, lattice rotations or electromagnetic coupling in multiferroic compounds can be revealed by using second harmonic…

Optics · Physics 2010-01-11 Pablo Molina , Mariola O Ramirez , Basilio J. Garcia , Luisa E. Bausa

We demonstrate unexpectedly strong second harmonic generation (SHG) in Argon gas by use of spatiotemporally focused (SF) femtosecond laser pulses. The resulting SHG by the SF scheme at a 75 cm distance shows a significantly enhanced…

The random laser action with coherent feedback by second-harmonic generation (SHG) was experimentally demonstrated in this paper. Compared with the conventional random laser action based on photoluminescence effect, which needs strong…

Optics · Physics 2016-11-24 Yanqi Qiao , Yuanlin Zheng , Zengyan Cai , Xianfeng Chen

Second-harmonic generation (SHG) is a direct measure of the strength of second-order nonlinear optical effects, which also include frequency mixing and parametric oscillations. Natural and artificial materials with broken…

Anomalously high generation efficiency of coherent higher field-harmonics in collisions between {\em oppositely charged particles} in the field of femtosecond lasers is predicted. This is based on rigorous numerical solutions of a quantum…

Condensed Matter · Physics 2009-10-31 H. Haberland , M. Bonitz , D. Kremp

Understanding the mechanisms and spatial correlations of crystallographic symmetry breaking in ferroelectric materials is essential to tuning their functional properties. While optical second harmonic generation (SHG) has long been utilized…

Materials Science · Physics 2022-08-10 Wei Li , Yunpeng Ma , Tianyi Feng , Sergei V. Kalinin , Jing-Feng Li , Qian Li

Domain-engineered quasi-phase-matching (QPM) devices are known for its versatility and ability to tune the nonlinear optical frequency conversion process. In this paper, a simple approach is presented to generate multiple…

Second harmonic generation is considered in lossy negative-index metamaterials. It is shown that energy transfer from fundamental to harmonic takes place in the entire sample for the range of phase mismatch values. Note that in conventional…

True phase-matched second-harmonic generation in a waveguide of crosslinkable ferroelectric liquid crystals is demonstrated. These materials allow the formation of macroscopically polar structures whose order can be frozen by…

Soft Condensed Matter · Physics 2009-10-31 Valentina S. U. Fazio , S. T. Lagerwall , P. Busson , A. Hult , H. Motschmann

Dielectric metasurfaces have shown prominent applications in nonlinear optics due to strong field enhancement and low dissipation losses at the nanoscale. Chalcogenide glasses are one of the promising materials for the observation of…

We report a systematic investigation into the processes behind a near hundredfold enhanced second harmonic wave generated from a laser-induced air plasma, by examining the temporal dynamics of the frequency conversion processes, and the…

We study second and third harmonic generation in centrosymmetric semiconductors at visible and UV wavelengths in bulk and cavity environments. Second harmonic generation is due to a combination of symmetry breaking, the magnetic portion of…

We demonstrate phase-matched second-harmonic generation (SHG) from three-dimensional metamaterials consisting of stacked metasurfaces. To achieve phase matching, we utilize a novel mechanism based on phase engineering of the metasurfaces at…

The nonlinear frequency conversion of low-temporal-coherent light holds a variety of applications and has attracted considerable interest. However, its physical mechanism remains relatively unexplored, and the conversion efficiency and…

Anomalous high-harmonic generation (HHG) arises in certain solids when irradiated by an intense laser field, as the result of a nonlinear perpendicular current akin to a Hall current. Here, we theoretically characterize the anomalous HHG…

Optics · Physics 2023-05-03 Lun Yue , Mette B. Gaarde

Resonant metasurfaces are an attractive platform for enhancing the non-linear optical processes, such as second harmonic generation (SHG), since they can generate very large local electromagnetic fields while relaxing the phase-matching…

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