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We have performed inelastic scanning tunneling spectroscopy (ISTS) on individual Fe atoms adsorbed on a Ag(111) surface. ISTS reveals a magnetization excitation with a lifetime of about 400 fsec which decreases linearly upon application of…

Mesoscale and Nanoscale Physics · Physics 2015-05-30 B. Chilian , A. A. Khajetoorians , S. Lounis , A. T. Costa , D. L. Mills , J. Wiebe , R. Wiesendanger

The advent of milli-kelvin scanning tunneling microscopes (STM) with inbuilt magnetic fields has opened access to the study of magnetic phenomena with atomic resolution at surfaces. In the case of single atoms adsorbed on a surface, the…

Mesoscale and Nanoscale Physics · Physics 2012-06-19 Jean-Pierre Gauyacq , Nicolas Lorente , Frederico Dutilh Novaes

We demonstrate using inelastic scanning tunneling spectroscopy (ISTS) and simulations based on density functional theory that the amplitude and sign of the magnetic anisotropy energy for a single Fe atom adsorbed onto the Pt(111) surface…

The recently discovered giant magnetic anisotropy of single magnetic Co atoms raises the hope of magnetic storage in small clusters. We present a joint experimental and theoretical study of the magnetic anisotropy and the spin dynamics of…

Materials Science · Physics 2009-07-06 T. Balashov , T. Schuh , A. F. Takacs , A. Ernst , S. Ostanin , J. Henk , I. Mertig , P. Bruno , T. Miyamachi , S. Suga , W. Wulfhekel

Magnetic adatoms on surfaces are exchange coupled to their environment, inducing fast relaxation of excited spin states and decoherence. These interactions can be suppressed by inserting decoupling layers between the magnetic adsorbate and…

Mesoscale and Nanoscale Physics · Physics 2022-04-01 Sergey Trishin , Christian Lotze , Nils Bogdanoff , Felix von Oppen , Katharina J. Franke

We report magnetic properties of the layered itinerant system, Sr$_{1-x}$Ca$_x$Co$_2$P$_2$ in the magnetic field up to 70 T. As for the exchange-enhanced Pauli paramagnetic metal SrCo$_2$P$_2$, the magnetization curve shows two…

Strongly Correlated Electrons · Physics 2014-07-21 Masaki Imai , Chishiro Michioka , Hiroto Ohta , Akira Matsuo , Koichi Kindo , Hiroaki Ueda , Kazuyoshi Yoshimura

Excitation of finite chains of magnetic atoms adsorbed on a surface by tunnelling electrons from an STM (Scanning Tunnelling Microscope) tip is studied using a Heisenberg Hamiltonian description of the magnetic couplings along the chain and…

Strongly Correlated Electrons · Physics 2010-10-19 J. P. Gauyacq , N. Lorente

The determination of the mean lifetime of excited states has been undertaken by coulomb excitation that is a process of inelastic scattering in which the incident particle is charged and provokes an excitation of the target nucleus by mean…

Nuclear Experiment · Physics 2007-05-23 A. Belafrites , A. Boucenna , C. Benazzouz , M. A. Benammar

Magnetic excitations of single atoms on surfaces have been widely studied experimentally in the past decade. Lately, systems with unprecedented magnetic stability started to emerge. Here, we present a general theoretical investigation of…

Mesoscale and Nanoscale Physics · Physics 2018-01-17 Timofey Balashov , Christian Karlewski , Tobias Märkl , Gerd Schön , Wulf Wulfhekel

We consider quasi-two-dimensional gas of electrons in a typical Si-MOSFET, assuming repulsive contact interaction between electrons. Magnetisation and susceptibility are evaluated within the mean-field approach. Finite thickness of the…

Mesoscale and Nanoscale Physics · Physics 2017-06-28 D. I. Golosov

We report Resonant Inelastic X-ray Scattering (RIXS) study of the magnetic excitation spectrum in a highly insulating Eu$_{2}$Ir$_{2}$O$_{7}$ single crystal that exhibits a metal-insulator transition at $T_{MI}$ = 111(7) K. A propagating…

Strongly Correlated Electrons · Physics 2018-06-13 Sae Hwan Chun , Bo Yuan , Diego Casa , Jungho Kim , Chang-Yong Kim , Zhaoming Tian , Yang Qiu , Satoru Nakatsuji , Young-June Kim

An electron transport is studied in the system which consists of scanning tunneling microscopy-single molecule magnet-metal. Due to quantum tunneling of magnetization in single-molecule magnet, linear response conductance exhibits stepwise…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 Gwang-Hee Kim , Tae-Suk Kim

The magnetic behavior of the Ca3Co2O6 spin chain compound is characterized by a large Ising-like character of its ferromagnetic chains, set on triangular lattice, that are antiferromagnetically coupled. At low temperature, T < 7K, the 3D…

Strongly Correlated Electrons · Physics 2007-05-23 A. Maignan , V. Hardy , S. Hebert , M. Drillon , M. R. Lees , O. Petrenko , D. Mc K. Paul , D. Khomskii

The lifetimes of spin excitations of Mn adsorbates on CuN/Cu(100) are computed from first-principles. The theory is based on a strong-coupling T-matrix approach that evaluates the decay of a spin excitation due to electron-hole pair…

Mesoscale and Nanoscale Physics · Physics 2015-05-19 Frederico D. Novaes , Nicolás Lorente , Jean-Pierre Gauyacq

Neutron scattering measurements of the magnetic excitations in single crystals of antiferromagnetic CaFe2As2 reveal steeply dispersive and well-defined spin waves up to an energy of 100 meV. Magnetic excitations above 100 meV and up to the…

The duality between localized and itinerant nature of magnetism in $5\textit{f}$ electron systems has been a longstanding puzzle. Here, we report inelastic neutron scattering measurements, which reveal both local and itinerant aspects of…

A single molecule magnet (SMM) can maintain its magnetization direction over a long period of time [1,2]. It consists in a low number of atoms that facilitates the understanding and control of the ground state, which is essential in future…

First-principles calculations of the magnetic anisotropy energy for Mn- and Fe-atoms on CuN/Cu(001) surface are performed making use of the torque method. The easy magnetization direction is found to be different for Mn and Fe atoms in…

Materials Science · Physics 2015-05-13 A. B. Shick , F. Máca , A. I. Lichtenstein

Inelastic neutron scattering experiments have been conducted to investigate the semimetal system Yb$_3$Ir$_4$Ge$_{13}$. No clear crystal-field-split levels were observed up to an excitation energy of 60 meV, while a magnetic excitation…

Strongly Correlated Electrons · Physics 2019-01-28 Kazuaki Iwasa , C. -L. Huang , Binod K. Rai , E. Morosan , Seiko Ohira-Kawamura , Kenji Nakajima

The role of the tip in inelastic electron tunneling spectroscopy (IETS) performed with scanning tunneling microscopes (STM) is theoretically addressed via first-principles simulations of vibrational spectra of single carbon monoxide (CO)…

Mesoscale and Nanoscale Physics · Physics 2011-04-12 Aran Garcia-Lekue , Daniel Sanchez-Portal , Andres Arnau , Thomas Frederiksen
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