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A molecular-dynamics thermal annealing model is proposed to investigate the mechanisms involved in picosecond pulsed laser ablation of crystalline silicon. In accordance with the thermal annealing model, a detailed description of the…
Ultracold molecules represent a fascinating research frontier in physics and chemistry, but it has proven challenging to prepare dense samples at low velocities. Here we present a solution to this goal by a non-conventional approach dubbed…
The simulation of the metabolism in mammalian cells becomes a severe problem if spatial distributions must be taken into account. Especially the cytoplasm has a very complex geometric structure which cannot be handled by standard…
A quantitative theory is developed, which accounts for heating artifacts in three-pulse photon echo (3PE) experiments. The heat diffusion equation is solved and the average value of the temperature in the focal volume of the laser is…
Hydrogenated amorphous carbon (a-C:H) has been proposed as one of the carbonaceous solids detected in the interstellar medium. Energetic processing of the a-C:H particles leads to the dissociation of the C-H bonds and the formation of…
We report an experimental investigation on the Doppler-free saturated absorption spectroscopy of buffer-gas-cooled Barium monofluoride (BaF) molecules in a 4~K cryogenic cell. The obtained spectra with a resolution of 19~MHz, much smaller…
The ecologically best way to produce nanoparticles (NP) is based on laser ablation in liquid (LAL). In the considered here case the LAL means that a gold target is irradiated through transparent water. During and after irradiation the…
We demonstrate a technique for obtaining the density of atomic vapor, by doing a fit of the resonant absorption spectrum to a density-matrix model. In order to demonstrate the usefulness of the technique, we apply it to absorption in the…
We demonstrate a scheme for direct absorption imaging of an ultracold ground-state polar molecular gas near quantum degeneracy. A challenge in imaging molecules is the lack of closed optical cycling transitions. Our technique relies on…
The femtosecond laser pulse heating of silver film is investigated by performing quantum mechanics (QM), molecular dynamics (MD) and two temperature model (TTM) integrated multiscale simulation. The laser excitation dependent electron…
The paper investigates cold molecules formation in the photoassociation of two cold atoms by a strong laser pulse applied at short interatomic distances, which lead to a molecular dynamics taking place in the light-induced (adiabatic)…
The modeling of stellar spectra is pervasive in astronomy. Conventionally, the shapes of absorption lines are modeled by convolving thermal profiles (computed given some model stellar atmosphere and line list) with broadening kernels…
A cryogenic neon solid doped with barium monofluoride (BaF) is created on a cryogenic substrate using a stream of Ne gas and a high-intensity beam of BaF molecules produced in a cryogenic helium-buffer-gas laser-ablation source. The…
We have investigated the all-optical generation of ions by photo-ionisation of atoms generated by pulsed laser ablation. A direct comparison between a resistively heated oven source and pulsed laser ablation is reported. Pulsed laser…
We report the complete characterization of various cooling grade Tm-doped crystals including the first demonstration of optical refrigeration in Tm:YLF crystals. Room temperature laser cooling efficiencies of 1% and 2% (mol) Tm:YLF, and 1%…
The formation of the first galaxies is accompanied by large accretion flows and virialization shocks, during which the gas is shock-heated to temperatures of $\sim10^4$ K, leading to potentially strong fluxes in the Lyman alpha line.…
The methods producing cold molecules from cold atoms tend to leave molecular ensembles with substantial residual internal energy. For instance, Cs2 molecules initially formed via photoassociation of cold Cs atoms are in several vibrational…
Under continuous laser irradiation, noble metal nanoparticles immersed in water can quickly heat up, leading to the nucleation of so-called plasmonic bubbles. In this work, we want to further understand the bubble nucleation and growth…
Molecular laser cooling and trapping requires addressing all spontaneous decays to excited vibrational states that occur at the $\gtrsim 10^{-4} - 10^{-5}$ level, which is accomplished by driving repumping transitions out of these states.…
A method for specular reflection of polar molecules is proposed. Electrostatatic potentials and forces are calculated for a low-field-seeking molecule near a series of long cylindrical electrodes of radius $r$ with dc potentials of $+V$ and…