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We reported a detailed experimental study of the cold collision of Barium monofluoride (BaF) with buffer gas and the high-resolution spectroscopy relevant with direct laser cooling. BaF molecules are efficiently produced with laser ablation…

Atomic Physics · Physics 2017-03-22 Wenhao Bu , Tao Chen , Guitao Lv , Bo Yan

Polar heavy-atom molecules have been well recognized as promising candidates for precision measurements and tests of fundamental physics. A much slower molecular beam to increase the interaction time should lead to a more sensitive…

Atomic Physics · Physics 2018-04-11 Yanning Yin , Supeng Xu , Meng Xia , Yong Xia , Jianping Yin

Ultrafast laser ablation is an extremely precise and clean method of removing material, applied in material processing as well as medical applications. And due to its violent nature, it tests our understanding of the interplay between…

Applied Physics · Physics 2018-10-17 Javier Hernandez-Rueda , Dries van Oosten

Cryogenic buffer gas cells have been a workhorse for the cooling of molecules in the last decades. The straightforward sympathetic cooling principle makes them applicable to a huge variety of different species. Notwithstanding this success,…

Chemical Physics · Physics 2020-08-26 Thomas Gantner , Manuel Koller , Xing Wu , Gerhard Rempe , Martin Zeppenfeld

A cryogenic buffer gas beam, an electrostatic hexapole lens, and 2D transverse Doppler laser cooling are combined to produce a bright beam of barium monofluoride ($^{138}$Ba$^{19}$F) molecules. Experimental results and trajectory…

The precise control and knowledge over the atomic dynamics is central to the advancement of quantum technology. The different experimental conditions namely, atoms in a vacuum, an anti-relaxation coated and a buffer gas filled atomic cell…

Atomic Physics · Physics 2022-07-21 Swarupananda Pradhan , Saptarshi Roy Chowdhury

We demonstrate slowing and longitudinal cooling of a supersonic beam of CaF molecules using counter-propagating laser light resonant with a closed rotational and almost closed vibrational transition. A group of molecules are decelerated by…

We describe the generation and properties of a cryogenic beam of $^7$Li$_2$ dimers from sublimation of a neon matrix where lithium atoms have been implanted via laser ablation of solid precursors of metallic lithium or lithium hydride…

In this paper we report on the production and characterization of a cold beam of BaOH molecules using a cryogenic buffer-gas beam source. BaOH is a highly suitable molecule for studies of the violation of fundamental symmetries, such as the…

We demonstrate that buffer-gas cooling combined with laser ablation can be used to create coherent optical media with high optical depth and low Doppler broadening that offers metastable states with low collisional and motional decoherence.…

We demonstrate a high-flux and low transverse temperature atomic beam of ytterbium by applying two-dimensional cooling using the ${}^1\mathrm{S}_0\text{-}{}^3\mathrm{P}_1$ intercombination transition to the cold atomic beam produced by the…

Atomic Physics · Physics 2022-10-27 Toshiyuki Hosoya , Ryotaro Inoue , Tomoya Sato , Mikio Kozuma

The creation of well-thermalized, hot and dense plasmas is attractive for warm dense matter studies. We investigate collisionally induced energy absorption of an ultraintense and ultrashort laser pulse in a solid copper target using…

Plasma Physics · Physics 2020-04-29 Andréas Sundström , Laurent Gremillet , Evangelos Siminos , István Pusztai

Barium monohydride (BaH) is an attractive candidate for extending laser cooling and trapping techniques to diatomic hydrides. The apparatus and high-resolution optical spectroscopy presented here demonstrate progress toward this goal. A…

Atomic Physics · Physics 2017-08-08 G. Z. Iwata , R. L. McNally , T. Zelevinsky

We present experimental measurements of photodesorption from ices of astrophysical relevance. Layers of benzene and water ice were irradiated with a laser tuned to an electronic transition in the benzene molecule. The translational energy…

Beams of atoms and molecules are stalwart tools for spectroscopy and studies of collisional processes. The supersonic expansion technique can create cold beams of many species of atoms and molecules. However, the resulting beam is typically…

Atomic Physics · Physics 2012-10-02 Nicholas R. Hutzler , Hsin-I Lu , John M. Doyle

In the laser processing of glass, a ~50-1000 $\mu$m-thick layer of glass is heated to a high temperature by the laser beam. Due to the shallow depth of this hot layer, the infrared emission and absorption spectra may deviate from the…

Materials Science · Physics 2025-01-15 Grigory Kolesov

We realize a novel high flux source of cold atoms and molecules employing hydrodynamic enhancement of an effusive aperture at cryogenic temperatures. Molecular oxygen from the source is coupled to a magnetic guide, delivering a cold,…

Chemical Physics · Physics 2007-05-23 David Patterson , John M. Doyle

We present the results of a study on relaxation and diffusion processes of rubidium atoms in a rubidium cell with an internal vapor source. The cell is an evacuated glass bulb, which is characterized in that the source of atomic vapors in…

We describe an approach to optically trapping small, chemically stable molecules at cryogenic temperatures by buffer-gas loading a deep optical dipole trap. The ~10 K trap depth will be produced by a tightly-focused, 1064-nm cavity capable…

We demonstrate one-dimensional sub-Doppler laser cooling of a beam of YbF molecules to 100 $\mu$K. This is a key step towards a measurement of the electron's electric dipole moment using ultracold molecules. We compare the effectiveness of…