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Related papers: The Stark effect on $H_2^+$-like molecules

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The H$_2$+H$_2$ system has long been considered as a benchmark system for ro-vibrational energy transfer in bimolecular collisions. However, most studies thus far have focused on collisions involving H$_2$ molecules in the ground…

Chemical Physics · Physics 2022-12-20 James F. E. Croft , Pablo G. Jambrina , F. Javier Aoiz , Hua Guo , N. Balakrishnan

The broadening of lines by Stark effect is an important tool for inferring electron density and temperature in plasmas. Stark-effect calculations often rely on atomic data (transition rates, energy levels,...) not always exhaustive and/or…

Atomic Physics · Physics 2016-06-22 Jean-Christophe Pain , Franck Gilleron , Dominique Gilles

Matching for a wavefunction the WKB expansion at large distances and Taylor expansion at small distances leads to a compact, few-parametric uniform approximation found in {\it J. Phys. B44, 101002 (2011)}. The ten low-lying eigenstates of…

Quantum Physics · Physics 2019-08-13 Horacio Olivares-Pilón , Alexander V. Turbiner

We define and measure the ratio (R) of the vector ac-Stark effect (or light shift) in the 6S_1/2 and 5D_3/2 states of a single trapped barium ion to 0.2% accuracy at two different off-resonant wavelengths. We earlier found R = -11.494(13)…

Atomic Physics · Physics 2009-11-13 J. A. Sherman , A. Andalkar , W. Nagourney , E. N. Fortson

Cross sections are presented for dissociative recombination and electron-impact vibrational excitation of the ArH+ molecular ion at electron energies appropriate for the interstellar environment. The R-matrix method is employed to determine…

Astrophysics of Galaxies · Physics 2018-08-21 A. Abdoulanziz , F. Colboc , D. A. Little , Y. Moulane , J. Zs. Mezei , E. Roueff , J. Tennyson , I. F. Schneider , V. Laporta

We develop a model for predicting fine- and hyperfine intensities in the direct photoionization of molecules based on the separability of electron and nuclear spin states from vibrational-electronic states. Using spherical tensor algebra,…

Chemical Physics · Physics 2016-08-24 Matthias Germann , Stefan Willitsch

In the present work, we analyze the influence of the polarization effects taking place during the course of a 2DIR spectroscopy experiment performed on a molecular system undergoing an intermolecular vibrational energy transfer process.…

Chemical Physics · Physics 2017-08-18 Albert A. Villaeys , Mabrouk Zouari , Kuo Kan Liang

Vibrational modes of molecules are fundamental properties determined by intramolecular bonding, atomic masses, and molecular geometry, and often serve as important channels for dissipation in nanoscale processes. Although single-molecule…

Mesoscale and Nanoscale Physics · Physics 2014-03-06 Y. Li , P. Doak , L. Kronik , J. B. Neaton , D. Natelson

Based on a combined quantum-classical treatment, a complete study of the strong field dynamics of H2+, i.e. including all nuclear and electronic DOF as well as dissociation and ionization, is presented. We find that the ro-vibrational…

Atomic and Molecular Clusters · Physics 2011-08-09 J. Handt , S. M. Krause , J. M. Rost , M. Fischer , F. Grossmann , R. Schmidt

Probing optical Stark effect at the single-molecule or atomic scale is crucial for understanding many photo-induced chemical and physical processes on surfaces. Here we report a study about optical Stark effect of single atomic defects on…

Mesoscale and Nanoscale Physics · Physics 2018-08-15 Lihuan Sun , Anning Dong , Jianmei Li , Dong Hao , Xiangqian Tang , Shichao Yan , Yang Guo , Xinyan Shan , Xinghua Lu

The excitation of the carbon $2^+$ state at 4.439 MeV by $70-150$ MeV electron impact and its subsequent decay to the ground state by photon emission is described within the distorted-wave Born approximation. The transition densities are…

Nuclear Theory · Physics 2020-07-15 D. H. Jakubassa-Amundsen , V. Yu. Ponomarev

We theoretically investigate the properties of highly polar diatomic molecules containing $^2S$-state transition-metal atoms. We calculate potential energy curves, permanent electric dipole moments, spectroscopic constants, and leading…

Atomic Physics · Physics 2021-02-16 Michał Śmiałkowski , Michał Tomza

Simultaneously, the vibrational nuclear dynamics and full dimensional electronic dynamics of the deuterium molecular ion exposed to the linear polarized intense laser field are studied. The time dependent Schr\"odinger equation of the…

Atomic Physics · Physics 2010-11-23 Mohsen Vafaee

The rotational excitation of the three asymmetric-top molecular ion isotopologues H$_2$O$^+$, HDO$^+$, and D$_2$O$^+$ is studied theoretically using a combined framework of electron-molecule R-matrix scattering theory, multichannel…

Atomic Physics · Physics 2026-03-19 Joshua Forer

Calculations have been carried out for the vibrational quenching of excited H$_2$ molecules which collide with Li$^+$ ions at ultralow energies. The dynamics has been treated exactly using the well known quantum coupled-channel expansions…

Chemical Physics · Physics 2009-11-13 S. Bovino , E. Bodo , F. A. Gianturco

The hydrogen molecules $H_2$ and $(H_2)_2$ are analyzed with electronic correlations taken into account between the $1s$ electrons exactly. The optimal single-particle Slater orbitals are evaluated in the correlated state of $H_2$ by…

Strongly Correlated Electrons · Physics 2015-02-03 Andrzej P. Kądzielawa , Agata Bielas , Marcello Acquarone , Andrzej Biborski , Maciej M. Maśka , Józef Spałek

A new variational technique is developed to investigate the polaronic features of the Holstein Molecular Crystal Model. It is based on a linear superposition of Bloch states that describe large and small polaron wave functions. It is shown…

Materials Science · Physics 2009-10-31 V. Cataudella , G. De Filippis , G. Iadonisi

Accurate low and high-lying bound states of Tietz-Hua oscillator potential are presented. The radial Schr\"odinger equation is solved efficiently by means of the generalized pseudospectral method that enables optimal spatial discretization.…

Chemical Physics · Physics 2014-09-10 Amlan K. Roy

The Stark coefficient of the Er 3+ ion in Y 2 SiO 5 is determined for transition). The stark photon echo beating method (SPEB) was used: the pseudo-Stark frequency shift was measured from the period of beats of the temporal form of the…

Materials Science · Physics 2018-12-12 V. N. Lisin , A. M. Shegeda , V. V. Samartsev , S. A. Kutovoi , Yu. D. Zavartsev

We present the first theoretical treatment of the formation of highly excited neutral H atoms (H$^{*}$) for strongly driven H$_{2}$. This process, with one electron ionizing and one captured in a Rydberg state, was recently reported in an…

Atomic Physics · Physics 2015-05-28 A. Emmanouilidou , D. Tchitchekova , C. Lazarou , U. Eichmann