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The geometric and electronic structures of NaN, CuN, and AgN metal clusters are systematically studied based on the density functional theory over a wide range of cluster sizes 2=<N=<75. A remarkable similarity is observed between the…

Materials Science · Physics 2015-05-13 Masahiro Itoh , Vijay Kumar , Tadafumi Adschiri , Yoshiyuki Kawazoe

This work explores the enhancement of ionization clusters around a gold nanoparticle (NP), indicative of the induction of DNA lesions, a potential trigger for cell-death. Monte Carlo track structure simulations were performed to determine…

Medical Physics · Physics 2024-03-08 Leo Thomas , Miriam Schwarze , Hans Rabus

We apply Density Functional Theory (DFT) and the DFT+U technique to study the adsorption of transition metal porphine molecules on atomistically flat Au(111) surfaces. DFT calculations using the Perdew-Burke-Ernzerhof (PBE) exchange…

Reactivity of Aluminum Clusters has been found to exhibit size sensitive variations. This work is motivated by a recent report1 predicting higher reactivity of melted Aluminum clusters towards the N2 molecule as compared to the non-melted…

Materials Science · Physics 2010-06-02 Bhakti S. Kulkarni , Sailaja Krishnamurty , Sourav Pal

The adsorption of metal atoms on nanostructures, such as graphene and nanotubes, plays an important role in catalysis, electronic doping, and tuning material properties. Quantum chemical calculations permit the investigation of this process…

Mesoscale and Nanoscale Physics · Physics 2020-02-18 Christoph Rohmann , Maicol A. Ochoa , Michael Zwolak

Thiol-based self-assembled monolayers (SAMs) on gold surfaces are one of the fundamental building blocks of molecular electronics. The strong chemical affinity of the gold and sulfur (Au-S) enables the formation of close-packed SAMs, but it…

First-principles density functional theory (DFT) study of embedding V and Nb atom in monovacant and divacant graphene is reported. Complete/almost complete spin polarization is verified for V/Nb embedding in MV/DV graphene. The origin of…

Materials Science · Physics 2018-04-26 Jyoti Thakur , Manish K. Kashyap , Hardev S. Saini , Ali H. Reshak

Owing to extremely large band gap of 5.5 eV and high thermal conductivity, diamond is recognized as the most important semiconductor. The superconductivity of polycrystalline diamond has always been reported, but there are also many…

Superconductivity · Physics 2024-03-04 Shisheng Lin , Xutao Yu , Minhui Yang , Huikai Zhong , Jiarui Guo

We report the effects of variation in length on the electronic structure of CdSe nanorods derived from atomic clusters and passivated by fictitious hydrogen atoms. These nanorods are augmented by attaching gold clusters at both the ends to…

Mesoscale and Nanoscale Physics · Physics 2017-09-13 Deepashri Saraf , Anjali Kshirsagar

The recent synthesis of Goldene, a 2D atomic monolayer of gold, has opened new avenues in exploring novel materials. However, the question of when multilayer Goldene transitions into bulk gold remains unresolved. This study used density…

We present a density functional theory study of low density bromination of graphene and graphite, finding significantly different behaviour in these two materials. On graphene we find a new Br2 form where the molecule sits perpendicular to…

Mesoscale and Nanoscale Physics · Physics 2011-03-18 A. Yaya , C. P. Ewels , I. Suarez-Martinez , Ph. Wagner , S. Lefrant , A. Okotrub , L. Bulusheva , P. R. Briddon

An ever present challenge for Li-ion batteries is the formation of metallic dendrites on cycling that dramatically reduces cycle life and leads to the untimely failure of the cell. In this work we investigate the modes of Li-cluster…

Materials Science · Physics 2023-11-01 Jonathon Cottom , Qiong Cai , Emilia Olsson

Metal atoms adsorbed on few layer graphenes condense to form nanometer-size droplets whose growth is size limited by a competition between the surface tension and repulsive electrostatic interactions from charge transfer between the metal…

Mesoscale and Nanoscale Physics · Physics 2015-05-19 L. A. Somers , N. A. Zimbovskaya , A. T. Johnson , E. J. Mele

Metal clusters are partway between molecular and bulk systems and thus exhibit special physical and chemical properties. Atoms can rearrange within a cluster to form different structural isomers. Internal degrees of freedom and the…

Materials Science · Physics 2019-07-31 Barbara A. J. Lechner , Fabian Knoller , Alexander Bourgund , Ueli Heiz , Friedrich Esch

This paper reviews the theoretical work undertaken using density functional theory (DFT) to explore graphene's interactions with its surroundings. We look at the impact of substrates, gate dielectrics and edge effects on the properties of…

Mesoscale and Nanoscale Physics · Physics 2012-07-31 Priyamvada Jadaun , Bhagawan R. Sahu , Leonard F. Register , Sanjay K. Banerjee

The lowest energy configurations of Cn(n =< 55) clusters are obtained using the energy mini- mization technique with the conjugate gradient (CG) method where a modified Brenner potential is invoked to describe the carbon and hydrocarbon…

Mesoscale and Nanoscale Physics · Physics 2015-05-18 D. P. Kosimov , A. A. Dzhurakhalov , F. M. Peeters

Gold nanoparticle assemblies show a strong plasmonic response due to the combined effects of the individual nanoparticles' plasmon modes. Increasing the number of nanoparticles in structured assemblies leads to significant shifts in the…

Optics · Physics 2022-07-13 Aditya K. Sahu , Satyabrata Raj

We investigate ground state properties of singly charged chlorine (Cl$^-$) and gold (Au$^-$) negative ions by employing four-component relativistic many-body methods. In our approach, we attach an electron to the respective outer orbitals…

Atomic Physics · Physics 2021-01-08 B. K. Sahoo

The so-called spin-orbit proximity effect experimentally realized in graphene (G) on several different heavy metal surfaces opens a new perspective to engineer the spin-orbit coupling (SOC) for new generation spintronics devices. Here, via…

Materials Science · Physics 2019-07-10 Jagoda Slawinska , Jorge I. Cerdá

We present density functional theory calculations of the binding energies of one, two and three fluorine adatoms on the same side of monolayer graphene. We show that fluorine dimers on graphene in a spin-singlet state are stable against…

Materials Science · Physics 2017-09-18 F Marsusi , N D Drummond