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Due to the absence of matching carbon atoms at honeycomb centers with carbon atoms in adjacent graphene sheets, theorists predicted that a sliding process is needed to form AA, AB, or ABC stacking when directly converting graphite into sp3…

We carried out density functional calculation to study Co$_{13}$ clusters on graphene. We deposit several free isomers in different disposition respect to hexagonal lattice nodes, studying even the $hcp$ $2d$ isomer recently obtained as the…

Materials Science · Physics 2015-12-25 Tomás Alonso-Lanza , Andrés Ayuela , Faustino Aguilera-Granja

Gold nanorods grafted with short chain polymers are assembled into controlled open structures using polymer-induced depletion interactions and structurally characterized using small angle x-ray scattering. When the nanorod diameter is…

Soft Condensed Matter · Physics 2018-02-13 Ryan Poling-Skutvik , Jonghun Lee , Suresh Narayanan , Ramanan Krishnamoorti , Jacinta C. Conrad

Nearly two-dimensional diamond, or diamane, is coveted as ultrathin $sp^3$-carbon film with unique mechanics and electro-optics. The very thinness ($~h$) makes it possible for the surface chemistry, e.g. adsorbed atoms, to shift the bulk…

Materials Science · Physics 2020-10-27 Sergey V. Erohin , Qiyuan Ruan , Pavel B. Sorokin , Boris I. Yakobson

Global geometry optimization and time-dependent density functional theory calculations have been used to study the structural evolution and optical properties of (AgAu)n (n=2-6) nanoalloys both as individual clusters and as clusters…

Materials Science · Physics 2017-02-23 Dennis Palagin , Jonathan P. K. Doye

The electronic structure of selected rare-earth atoms adsorbed on a free-standing graphene was investigated using methods beyond the conventional density functional theory (DFT+U, DFT+HIA and DFT+ED). The influence of the electron…

Strongly Correlated Electrons · Physics 2016-09-12 Agnieszka L. Kozub , Alexander B. Shick , Frantisek Maca , Jindrich Kolorenc , Alexander I. Lichtenstein

Magnetism in bare uncapped gold nano-clusters is explored from a density functional theory perspective with scalar relativistic effects included via the pseudo-potential. The computed electronic structures of various nano-clusters reveal…

Materials Science · Physics 2007-05-23 R. J. Magyar , V. Mujica , M. Marquez , C. Gonzalez

We systematically investigate the magnetic and electronic properties of graphene adsorbed with diluted 3d-transition and noble metal atoms using first principles calculation methods. We find that most transition metal atoms (i.e. Sc, Ti, V,…

Materials Science · Physics 2011-11-16 Jun Ding , Zhenhua Qiao , Wanxiang Feng , Yugui Yao , Qian Niu

Single atoms and few-atom nanoclusters are of high interest in catalysis and plasmonics, but pathways for their fabrication and stable placement remain scarce. We report here the self-assembly of room-temperature-stable single indium (In)…

Here we show results of first-principles investigations aiming at tuning and controlling the catalytic activity of gold nanoclusters through the design of the underlying support. We show that gold clusters adsorbed on a very thin (2 layers)…

Materials Science · Physics 2011-02-16 Chun Zhang , Bokwon Yoon , Uzi Landman

This study investigates the structural stability of ionized gold clusters of sizes ranging from 22 to 100 atoms, contrasting compact, cage and planar structures. While it is well known that neutral clusters in the upper part of this size…

Materials Science · Physics 2026-02-18 Mohammad Ismaeil Safa , Ehsan Rahmatizad Khajehpasha , Stefan Goedecker

We have performed an ab initio investigation of the energetic stability, and the electronic properties of transition metals (TMs = Mn, Fe, Co, and Ru) adsorbed on graphene upon the presence of grain boundaries (GBs). Our results reveal an…

Materials Science · Physics 2017-10-12 F. D. C. de Lima , R. H. Miwa

Transistors operating at high frequencies are the basic building blocks of millimeter-wave communication and sensor systems. The high velocity and mobility of carriers in graphene can open way for ultra-fast group IV transistors with…

Mesoscale and Nanoscale Physics · Physics 2022-01-03 Muhammad Asad , Saman Majdi , Andrei Vorobiev , Kjell Jeppson , Jan Isberg , Jan Stake

Density function theory calculations were carried out to clarify storage states of Lithium (Li) ions in graphene clusters. The adsorption energy, spin polarization, charge distribution, electronic gap, surface curvature and dipole momentum…

Materials Science · Physics 2015-06-03 N. Kheirabadi , A. Shafiekhani

Density functional theory (DFT) modeling of the physisorption of four different types of molecules (toluene, bromine dimmer, water and nitrogen dioxide) over and above graphene ripples has been performed. For all types of molecules changes…

Mesoscale and Nanoscale Physics · Physics 2015-05-20 D. W. Boukhvalov

The growth of controlled 1D carbon-based nanostructures on metal surfaces is a multistep process whose path, activation energies and intermediate metastable states strongly depend on the employed substrate. Whereas this process has been…

We use density functional theory (DFT) to study the thermodynamic stability and migration of copper ions and small clusters embedded in amorphous silicon dioxide. We perform the calculations over an ensemble of statistically independent…

Materials Science · Physics 2015-06-11 David M. Guzman , Nicolas Onofrio , Alejandro Strachan

The ground state energies of Ag and Au in the face-centered cubic (FCC), body-centered cubic (BCC), simple cubic (SC) and the hypothetical diamond-like phase, and dimer were calculated as a function of bond length using density functional…

Materials Science · Physics 2015-06-12 John T. Titantah , Mikko Karttunen

The nucleation of graphene on a transition metal (TM) surface, either on a terrace or near a step edge, is systematically explored using density functional theory (DFT) calculations and applying the two-dimensional (2D) crystal nucleation…

Materials Science · Physics 2011-04-04 Junfeng Gao , Joanne Yip , Jijun Zhao , Boris I. Yakobson , Feng Ding

We use density functional theory (DFT) with a recently developed van der Waals density functional (vdW-DF) to study the adsorption of graphene on Al, Cu, Ag, Au, Pt, Pd, Co and Ni(111) surfaces. In constrast to the local density…

Mesoscale and Nanoscale Physics · Physics 2015-05-14 M. Vanin , J. J. Mortensen , A. K. Kelkkanen , J. M. Garcia-Lastra , K. S. Thygesen , K. W. Jacobsen