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The dominant mechanism of low-energy positron annihilation in polyatomic molecules is through positron capture in vibrational Feshbach resonances (VFR). In this paper we investigate theoretically the effect of anharmonic terms in the…

Atomic Physics · Physics 2017-12-27 G. F. Gribakin , J. F. Stanton , J. R. Danielson , M. R. Natisin , C. M. Surko

Measurements of energy-resolved positron-molecule annihilation show the existence of positron binding and vibrational Feshbach resonances. The existing theory describes this phenomenon successfully for the case of infrared-active…

Atomic Physics · Physics 2017-09-25 M. R. Natisin , J. R. Danielson , G. F. Gribakin , A. R. Swann , C. M. Surko

The aim of this work is to identify the mechanisms responsible for very large rates and other peculiarities observed in low-energy positron annihilation on molecules. The two mechanisms considered are: (i) Direct annihilation of the…

Atomic Physics · Physics 2009-10-31 G. F. Gribakin

Enhanced positron annihilation on polyatomic molecules is a long-standing and complex problem. We report the results of calculations of resonant positron annihilation on methyl halides. A free parameter of our theory is the positron binding…

Atomic Physics · Physics 2010-02-16 G. F. Gribakin , C. M. R. Lee

The model-potential approach previously developed by the authors to study positron interactions with molecules is used to calculate the positron binding energy for $n$-alkanes (C$_n$H$_{2n+2}$) and the corresponding cycloalkanes…

Atomic Physics · Physics 2020-11-13 A. R. Swann , G. F. Gribakin

Annihilation spectra are presented for aromatic and heterocyclic ring molecules resolved as a function of incident positron energy using a trap-based positron beam. Comparisons with the vibrational mode spectra yield positron-molecule…

Positrons bind to molecules leading to vibrational excitation and spectacularly enhanced annihilation. Whilst positron binding energies have been measured via resonant annihilation spectra for $\sim$90 molecules in the past two decades, an…

Atomic Physics · Physics 2023-03-23 J. Hofierka , B. Cunningham , C. M. Rawlins , C. H. Patterson , D. G. Green

A method is proposed for detecting positron-atom bound states by observing enhanced positron annihilation due to electronic Feshbach resonances at electron-volt energies. The method is applicable to a range of open-shell transition metal…

Atomic Physics · Physics 2010-12-10 V. A. Dzuba , V. V. Flambaum , G. F. Gribakin

Calculations of gamma spectra for positron annihilation on a selection of molecules, including methane and its fluoro-substitutes, ethane, propane, butane and benzene are presented. The annihilation gamma spectra characterise the momentum…

Atomic Physics · Physics 2012-04-18 D. G. Green , S. Saha , F. Wang , G. F. Gribakin , C. M. Surko

A model-potential approach has been developed to study positron interactions with molecules. Binding energies and annihilation rates are calculated for positron bound states with a range of alkane molecules, including rings and isomers. The…

Atomic Physics · Physics 2019-09-17 A. R. Swann , G. F. Gribakin

In this paper we use a zero-range potential (ZRP) method to model positron interaction with molecules. This allows us to investigate the effect of molecular vibrations on positron-molecule annihilation using the van der Waals dimer Kr2 as…

Atomic Physics · Physics 2010-02-16 G. F. Gribakin , C. M. R. Lee

$\gamma$-ray spectra for positron annihilation with the core and valence electrons of the noble gas atoms Ar, Kr and Xe is calculated within the framework of diagrammatic many-body theory. The effect of positron-atom and short-range…

Atomic Physics · Physics 2015-03-06 D. G. Green , G. F. Gribakin

In this work, we observe a novel resonant mechanism, namely the modulation-induced Feshbach resonance. By applying a far-detuned laser to the cesium D2 transition with intensity modulation, we periodically shake the energy levels of atomic…

Quantum Physics · Physics 2025-12-30 Tongkang Wang , Yuqi Liu , Jundong Wang , Youjia Huang , Wenlan Chen , Zhendong Zhang , Jiazhong Hu

We study the rotational predissociation of atom - molecule complexes with very small binding energy. Such complexes can be produced by Feshbach resonance association of ultracold molecules with ultracold atoms. Numerical calculations of the…

Chemical Physics · Physics 2011-10-03 Alisdair O. G. Wallis , Roman V. Krems

A model-potential approach to calculating positron-molecule binding energies and annihilation rates is developed. Unlike existing ab initio calculations, which have mostly been applied to strongly polar molecules, the present methodology…

Atomic Physics · Physics 2018-12-31 A. R. Swann , G. F. Gribakin

We propose a new type of Feshbach resonance occurring when two different ultracold atoms in their ground state undergo an s-wave collision in the presence of a continuous-wave laser light. The atoms collide in the dissociation continuum of…

We have studied interspecies scattering in an ultracold mixture of $^{87}$Rb and $^{133}$Cs atoms, both in their lowest-energy spin states. The three-body loss signatures of 30 incoming s- and p-wave magnetic Feshbach resonances over the…

We present a simple technique for studying collisions of ultracold atoms in the presence of a magnetic field and radio-frequency radiation (rf). Resonant control of scattering properties can be achieved by using rf to couple a colliding…

Quantum Gases · Physics 2010-09-28 Thomas M. Hanna , Eite Tiesinga , Paul S. Julienne

A model for positron binding to polar molecules is considered by combining the dipole potential outside the molecule with a strongly repulsive core of a given radius. Using existing experimental data on binding energies leads to…

Atomic Physics · Physics 2015-09-24 G. F. Gribakin , A. R. Swann

R-matrix calculations on electron collisions with CO are reported whose aim is to identify any higher-lying resonances above the well-reported and lowest $^2\Pi$ resonance at about 1.6~eV. Extensive tests with respect to basis sets, target…

Chemical Physics · Physics 2016-10-11 Amar Dora , Jonathan Tennyson , Kalyan Chakrabarti
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