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We develop numerical methods to calculate electron dynamics in crystalline solids in real-time time-dependent density functional theory employing exchange-correlation potentials which reproduce band gap energies of dielectrics; a meta…

Materials Science · Physics 2016-01-07 Shunsuke A. Sato , Yasutaka Taniguchi , Yasushi Shinohara , Kazuhiro Yabana

The nonequilibrium Green's function formalism provides a versatile and powerful framework for numerical studies of nonequilibrium phenomena in correlated many-body systems. For calculations starting from an equilibrium initial state, a…

Strongly Correlated Electrons · Physics 2024-07-11 Matthias Murray , Hiroshi Shinaoka , Philipp Werner

We introduce the time-dependent restricted active space Configuration Interaction method to solve the time-dependent Schr\"odinger equation for many-electron atoms, and particularly apply it to the treatment of photoionization processes in…

Atomic Physics · Physics 2013-05-30 David Hochstuhl , Michael Bonitz

In this work we examine the time-resolved, instantaneous current response for the spinless Falicov-Kimball model at half-filling, on both sides of the Mott-Hubbard metal-insulator transition, driven by a strong electric field pump pulse.…

Strongly Correlated Electrons · Physics 2015-05-18 B. Moritz , T. P. Devereaux , J. K. Freericks

If one-electron observables of a many-electron system are of interest, a many-electron dynamics can be represented exactly by a one-electron dynamics with effective potentials. The formalism for this reduction is provided by the Exact…

Chemical Physics · Physics 2021-01-04 Jakub Kocák , Axel Schild

We study the equilibration and relaxation processes within the time-dependent Hartree-Fock approach using the Wigner distribution function. On the technical side we present a geometrically unrestricted framework which allows us to calculate…

Nuclear Theory · Physics 2012-01-26 N. Loebl , A. S. Umar , J. A. Maruhn , P. -G. Reinhard , P. D. Stevenson , V. E. Oberacker

We present a Kadanoff-Baym formalism to study time-dependent phenomena for systems of interacting electrons and phonons in the framework of many-body perturbation theory. The formalism takes correctly into account effects of the initial…

Mesoscale and Nanoscale Physics · Physics 2016-01-20 N. Säkkinen , Y. Peng , H. Appel , R. van Leeuwen

Error estimates are proved for finite element approximations to the solution of second-order hyperbolic partial differential equations with coefficients varying in both space and time. Optimal rates of convergence in the energy norm are…

Numerical Analysis · Mathematics 2026-03-17 Oussama Al Jarroudi , Marcus J. Grote

Fully numerical mesh solutions of 2D quantum equations of Schroedinger and Hartree-Fock type allow us to work with wavefunctions which possess a very flexible geometry. This flexibility is especially important for calculations of atoms and…

Atomic Physics · Physics 2015-06-26 Mikhail V. Ivanov , Peter Schmelcher

We present a real-time second-order Green's function (GF) method for computing excited states in molecules and nanostructures, with a computational scaling of $O(N_{\rm e}^3$), where $N_{\rm e}$ is the number of electrons. The cubic scaling…

Chemical Physics · Physics 2024-01-29 Leopoldo Mejía , Jia Yin , David R. Reichman , Roi Baer , Chao Yang , Eran Rabani

Based on the nonequilibrium Green's function (NEGF), we develop a quantum nonlinear theory to study time-dependent ac transport properties in the low frequency and nonlinear bias voltage regimes. By expanding NEGF in terms of time to the…

Mesoscale and Nanoscale Physics · Physics 2023-11-07 Lei Zhang , Fuming Xu , Jian Chen , Yanxia Xing , Jian Wan

Photoelectron emission from excited states of laser-dressed atomic helium is analyzed with respect to laser intensity-dependent excitation energy shifts and angular distributions. In the two-color XUV (exteme ultra\-violet) -- IR (infrared)…

We present a straightforward implementation scheme for solving the time dependent Schr\"odinger equation for systems described by the Hubbard Hamiltonian with time dependent hoppings. The computations can be performed for clusters of up to…

Strongly Correlated Electrons · Physics 2020-12-08 Michael Innerberger , Paul Worm , Paul Prauhart , Anna Kauch

Real-time time-dependent density functional theory, in conjunction with the Ehrenfest molecular dynamics scheme, is becoming a popular methodology to investigate ultrafast phenomena on the nanoscale. Thanks to recent developments, it is…

Materials Science · Physics 2020-08-18 Jannis Krumland , Ana M. Valencia , Stefano Pittalis , Carlo A. Rozzi , Caterina Cocchi

We formulate a time-dependent density functional theory for the coupled dynamics of electrons and nuclei that goes beyond the Born-Oppenheimer (BO) approximation. We prove that the time-dependent marginal nuclear probability density…

Chemical Physics · Physics 2025-11-14 Chen Li , Ryan Requist , E. K. U. Gross

This article examines the time-dependent Hartree-Fock (TDHF) approximation of single-particle dynamics in systems of interacting fermions. We find the TDHF approximation to be accurate when there are sufficiently many particles and the…

Mathematical Physics · Physics 2007-05-23 Claude Bardos , Francois Golse , Alex D. Gottlieb , Norbert J. Mauser

We define the model of hydrogen atom for twist-deformed acceleration-enlarged Newton-Hooke space-time. Further, using time-dependent perturbation theory, we find in first step of iteration procedure the solution of corresponding…

High Energy Physics - Theory · Physics 2013-12-10 Marcin Daszkiewicz

The time-dependent density functional (TDDFT) equations may be written either for the Kohn-Sham orbitals in Hilbert space or for the single electron density matrix in Liouville space. A collective-oscillator, quasiparticle, representation…

Strongly Correlated Electrons · Physics 2009-11-10 Oleg Berman , Shaul Mukamel

We consider a non-relativistic two-dimensional (2D) hydrogen-like atom in a weak, static, uniform magnetic field perpendicular to the atomic plane. Within the framework of the Rayleigh-Schr\"odinger perturbation theory, using the Sturmian…

Quantum Physics · Physics 2018-06-12 Radosław Szmytkowski

A nonadiabatic scheme for the description of the coupled electron and nuclear motions in the ozone molecule was proposed recently. An initial coherent nonstationary state was prepared as a superposition of the ground state and the excited…

Atomic and Molecular Clusters · Physics 2015-06-18 A. Perveaux , D. Lauvergnat , B. Lasorne , F. Gatti , M. A. Robb , G. J. Halász , Á. Vibók