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We derive a general procedure for evaluating the ${\rm n}$th derivative of a time-dependent operator in the Heisenberg representation and employ this approach to calculate the zeroth to third spectral moment sum rules of the retarded…

Strongly Correlated Electrons · Physics 2023-02-14 Khadijeh Najafi , J. Alexander Jacoby , R. D. Nesselrodt , J. K. Freericks

Quantization of electrodynamics in curved space-time in the Lorenz gauge and with arbitrary gauge parameter makes it necessary to study Green functions of non-minimal operators with variable coefficients. Starting from the integral…

High Energy Physics - Theory · Physics 2009-11-10 Giuseppe Bimonte , Enrico Calloni , Luciano Di Fiore , Giampiero Esposito , Leopoldo Milano , Luigi Rosa

Measurements of the phase of two-photon matrix elements are presented for resonant and antiresonant two-color ionization of helium. A tunable, narrow-bandwidth, near-infrared (NIR) laser source is used for extreme ultra-violet (XUV)…

Atomic Physics · Physics 2022-02-02 Lorenz Drescher , Tobias Witting , Oleg Kornilov , Marc J. J. Vrakking

We derive exact operator average expressions for the first two spectral moments of nonequilibrium Green's functions for the Falicov-Kimball model and the Hubbard model in the presence of a spatially uniform, time-dependent electric field.…

Strongly Correlated Electrons · Physics 2009-11-11 V. M. Turkowski , J. K. Freericks

Theoretical approaches to the photoionization of few-electron atoms are discussed. These include nonequilibrium Greens functions and wave function based approaches. In particular, the Multiconfiguration Time-Dependent Hartree-Fock method is…

Atomic Physics · Physics 2015-05-14 M. Bonitz , D. Hochstuhl , S. Bauch , K. Balzer

The theory of Nonequilibrium Green functions (NEGF) has seen a rapid development over the recent three decades. Applications include diverse correlated many-body systems in and out of equilibrium. Very good agreement with experiments and…

Strongly Correlated Electrons · Physics 2026-04-02 Michael Bonitz , Jan-Philip Joost , Christopher Makait , Erik Schroedter , Tim Karsberger , Karsten Balzer

The exact quantum time-dependent optical response of hydrogen under strong field near infrared excitation is investigated and compared to the perturbative model widely used for describing the effective atomic polarization induced by intense…

The Hubbard model is a prototype for strongly correlated many-particle systems, including electrons in condensed matter and molecules, as well as for fermions or bosons in optical lattices. While the equilibrium properties of these systems…

Strongly Correlated Electrons · Physics 2014-09-10 Sebastian Hermanns , Niclas Schlünzen , Michael Bonitz

A mixed quantum-classical approach is introduced which allows the dynamical response of molecules driven far from equilibrium to be modeled. This method is applied to the interaction of molecules with intense, short-duration laser pulses.…

Atomic Physics · Physics 2012-05-21 Daniel Dundas

The time-dependent variational principle proposed by Balian and Veneroni is used to provide the best approximation to the generating functional for multi-time Green's functions of a set of (bosonic) observables $Q_{\mu)$. By suitably…

High Energy Physics - Theory · Physics 2016-09-06 Mohamed Benarous

The Born-Oppenheimer (BO) approximation is less accurate in the presence of a strong magnetic field than in the absence of a field. This is due to the complicated and unpredictable response of electronic structure to the field, especially…

Chemical Physics · Physics 2023-03-29 Tanner Culpitt , Laurens D. M. Peters , Erik I. Tellgren , Trygve Helgaker

A nonlocal quantum model is presented for calculating the atomic dielectric response to a strong laser electric field. By replacing the Coulomb potential with a nonlocal potential in the Schrodinger equation, a 3+1D calculation of the…

Atomic Physics · Physics 2015-06-18 T. C. Rensink , T. M. Antonsen , J. P. Palastro , D. Gordon

In the nonequilibrium Green's function approach, the approximation of the correlation self-energy at the second-Born level is of particular interest, since it allows for a maximal speed-up in computational scaling when used together with…

Computational Physics · Physics 2019-11-11 Riku Tuovinen , Fabio Covito , Michael A. Sentef

An efficient implementation of the nonequilibrium Green function (NEGF) method combined with the density functional theory (DFT) using localized pseudo-atomic orbitals (PAOs) is presented for electronic transport calculations of a system…

Mesoscale and Nanoscale Physics · Physics 2015-05-14 Taisuke Ozaki , Kengo Nishio , Hiori Kino

We present a time-dependent localized Hartree-Fock density-functional linear response approach for the treatment of photoionization of atomic systems. This approach employs a spin-dependent localized Hartree-Fock (SLHF) exchange potential…

Quantum Physics · Physics 2015-05-13 Zhongyuan Zhou , Shih-I Chu

We present accurate time-dependent ab initio calculations on fully differential and total integrated (generalized) cross sections for the nonsequential two-photon double ionization of helium at photon energies from 40 to 54 eV. Our…

Atomic Physics · Physics 2008-05-07 J. Feist , S. Nagele , R. Pazourek , E. Persson , B. I. Schneider , L. A. Collins , J. Burgdörfer

We provide a systematic approach to compute different kinds of non-equilibrium Green's functions for open quantum systems which are essentially two-point correlation functions in time. We reveal that the definition of Green's functions…

Statistical Mechanics · Physics 2023-09-08 Katha Ganguly , Bijay Kumar Agarwalla

Nonequilibrium Green's functions represent underutilized means of studying the time evolution of quantum many-body systems. In view of a rising computer power, an effort is underway to apply the Green's functions formalism to the dynamics…

Nuclear Theory · Physics 2008-11-26 Arnau Rios , Pawel Danielewicz

The electric conductance of a molecular junction is calculated by recasting the Keldysh formalism in Liouville space. Dyson equations for nonequilibrium many body Green's functions (NEGF) are derived directly in real (physical) time. The…

Quantum Physics · Physics 2007-05-23 U. Harbola , S. Mukamel

A method of solving the time-dependent Schr\"odinger equation is presented, in which a finite region of space is treated explicitly, with the boundary conditions for matching the wave-functions on to the rest of the system replaced by an…

Materials Science · Physics 2009-11-13 J. E. Inglesfield