Related papers: THz generation by dual-color pulse in prealigned m…
We investigate the persistent orientation of asymmetric-top molecules induced by time-delayed THz pulses that are either collinearly or cross polarized. Our theoretical and numerical results demonstrate that the orthogonal configuration…
We show that coherently driven atomic or molecular media potentially yield strong controllable short pulses of THz radiation. The method is based on excitation of maximal quantum coherence in a gas medium by optical pulses and coherent…
Waveform-controlled Terahertz (THz) radiation is of great importance due to its potential application in THz sensing and coherent control of quantum systems. We demonstrated a novel scheme to generate waveform-controlled THz radiation from…
Forward and backward THz emission by ionizing two-color laser pulses in gas is investigated by means of a simple semi-analytical model based on Jefimenko's equation and rigorous Maxwell simulations in one and two dimensions. We find the…
High-energy terahertz pulses are challenging to produce due to the low conversion efficiency and limited optical damage threshold of nonlinear crystals. Here, we describe the high-efficiency generation of terahertz radiation pulses with…
This study shows the unexpected and counter-intuitive possibility of simultaneously orienting a molecule while delocalizing its molecular axis in a plane in field-free conditions. The corresponding quantum states are characterized and…
Based on spatial-temporal symmetry breaking mechanism, we propose a novel scheme for terahertz (THz) wave generation from hyper-Raman lines associated with the 0th harmonic (a particular even harmonic) in a two-level quantum system driven…
Terahertz (THz) radiation by beating of two laser beams in a groove density and magnetized hot plasma is discussed theoretically. In this mechanism, the ponderomotive force leads to a nonlinear oscillatory current that resonantly excites…
We show experimentally that the terahertz (THz) emission of a plasma, generated in air by a two-color laser pulse (containing a near IR frequency and its second harmonic), can be enhanced by the addition of an 800-nm pulse. We observed…
It is shown, by simulation and theory, that circularly or elliptically polarized terahertz radiation can be generated when a static magnetic (B) field is imposed on a gas target along the propagation direction of a two-color laser driver.…
We investigate to which extend a THz laser pulse can be used to produce field-free molecular orientation at high temperature. We consider laser pulses that can be implemented with the state of the art technology and we show that the…
We demonstrate that pulsed THz radiation produced in air by a focused ultrashort laser pulse can be steered to large angles or even in the backward direction with respect to the laser propagation axis. The emission angle is adjusted by the…
The coherent radiation spectrum of two-level polar molecules with UV transition is studied at the multiphoton resonant excitation by a moderately strong laser field. The spectrum corresponding to harmonic generation and low-frequency…
We consider harmonics generation and wave-mixing by two-color multi photon resonant excitation of three-level atoms/molecules in strong laser fields. The coherent part of the spectra corresponding to multicolor harmonics generation is…
Using a canonical pump-probe experimental technique, we studied the terahertz (THz) waves generation and detection via optical rectification and mixing in Czochralski-grown periodically poled Mg:Y:LiNbO3 (PPLN) crystals. THz waves with…
High-order harmonic generation in the presence of a chirped THz pulse is investigated numerically with a complete 3D non-adiabatic model. The assisting THz pulse illuminates the HHG gas cell laterally inducing quasi-phase-matching. We…
The two-color strong-field mixing in gas medium is a widely-used approach to generate bright broadband terahertz (THz) radiation. Here, we present a new and counterintuitive method to promote THz performance in two-color scheme. Beyond our…
Two-color laser induced plasma filamentation in air could serve as tabletop sources of broadband terahertz (THz) pulses. Ubiquitous air in the earth facilitates its widespread utilities, particularly, in wireless communication and remote…
Controlling light polarization is one of the most essential routines in modern optical technology. Since the demonstration of optical pulse shaping by spatial light modulators and its potential in controlling the quantum reaction pathways,…
The ability to manipulate the space-time structure of light waves diversifies light-matter interaction and light-driven applications. Conventionally, metasurfaces are employed to locally control the amplitude and phase of light fields by…