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Magnesium hydride (MgH2) is the mostly used material for solid-state hydrogen storage. However, their slow kinetics and highly unfavorable thermodynamics make them unsuitable for the practical applications. The current study describes the…

Materials Science · Physics 2023-07-25 S. K. Verma , S. S. Mishra , N. K. Mukhopadhyay , T. P. Yadav

Rovibronic molecular hydrogen (H$_2$) transitions at redshift $z_{\rm abs} \simeq 2.659$ towards the background quasar B0642$-$5038 are examined for a possible cosmological variation in the proton-to-electron mass ratio, $\mu$. We utilise…

Cosmology and Nongalactic Astrophysics · Physics 2015-06-16 Julija Bagdonaite , Wim Ubachs , Michael T. Murphy , Jonathan B. Whitmore

The molecular phase of hydrogen converts to the atomic metallic phase at high pressures estimated usually as 300 - 500 GPa. We analyze the decay of metallic phase as the pressure is relieved below the transition one. The metallic state is…

Other Condensed Matter · Physics 2018-01-03 S. N. Burmistrov , L. B. Dubovskii

The compression of arsenolite (cubic As2O3) has been studied from a joint experimental and theoretical point of view. Experimental X-ray diffraction and Raman scattering measurements of this molecular solid at high pressures with different…

We describe measurements demonstrating laser cooling of an atomic gas by means of collisional redistribution of radiation. The experiment uses rubidium atoms in the presence of several hundred bar of argon buffer gas pressure. Frequent…

Atomic Physics · Physics 2012-01-04 Ulrich Vogl , Anne Saß , Simon Haßelmann , Martin Weitz

The desorption dynamics of rubidium dimers (Rb_2) off the surface of helium nanodroplets induced by laser excitation is studied employing both nanosecond and femtosecond ion imaging spectroscopy. Similarly to alkali metal atoms, we find…

Atomic and Molecular Clusters · Physics 2017-02-08 A. Sieg , J. von Vangerow , F. Stienkemeier , O. Dulieu , M. Mudrich

A theoretical model for the effect of water hydrogen bonding on the thermodynamics of hydrophobic hydration is proposed as a combination of the classical density functional theory with the recently developed probabilistic approach to water…

Statistical Mechanics · Physics 2011-06-16 Yuri S. Djikaev

Aims. The mobility of H atoms on the surface of interstellar dust grains at low temperature is still a matter of debate. In dense clouds, the hydrogenation of adsorbed species (i.e., CO), as well as the subsequent deuteration of the…

Astrophysics · Physics 2009-11-13 E. Matar , E. Congiu , F. Dulieu , A. Momeni , J. L. Lemaire

Density-functional theory calculations are performed to investigate hydrogen transport in the proton conductor BaSnO$_3$. Structural optimizations in the stable and saddle point configurations for transfer and reorientation allow…

Materials Science · Physics 2014-11-13 Grégory Geneste , Alistar Ottochian , Jessica Hermet , Guilhem Dezanneau

Two dimensional transition metal dichalcogenides appear as good candidates for gas sensing and catalysis. Here, by means of density functional theory, we characterize the adsorption and dissociation of selected diatomic molecules (CO,…

Materials Science · Physics 2022-01-06 Raúl Bombín , Maite Alducin , Iñaki Juaristi

In recent years the advance of chemical synthesis has made it possible to obtain \textquotedblleft naked\textquotedblright clusters of different transition metals. It is well known that cluster experiments allow studying the fundamental…

Materials Science · Physics 2023-02-01 Maximiliano L. Riddick , Enrique E. Álvarez , Félix G. Requejo , Leandro Andrini

Developing efficient hydrogen storage and conversion technologies is essential for sustainable energy. This study investigates the catalytic potential of a dicalcium nitride (Ca2N) monolayer for hydrogen dissociation using density…

Mesoscale and Nanoscale Physics · Physics 2025-01-28 Gwan Woo Kim , Soonmin Jang , Gunn Kim

Zero-dimensional kinetic modeling of atmospheric pressure Ar-N2-H2 nonthermal plasma was carried out to gain mechanistic insights into ammonia formation during plasma-assisted catalysis of ammonia synthesis. The kinetic model was developed…

Plasma Physics · Physics 2024-03-26 Zihan Lin , Shota Abe , Zhe Chen , Surabhi Jaiswal , Bruce E. Koel

We report the presence of a systematic excess in the molecular hydrogen fraction ($f_{\mathrm{H2}} = 2 \, n_{\mathrm{H2}}/n_{\mathrm{H}}$) in studies that use a reduced chemistry network to calculate $f_{\mathrm{H2}}$ of gas with a non-zero…

Astrophysics of Galaxies · Physics 2026-03-03 Sylvia Ploeckinger

We report the first experimental evidence for a metallic phase in fluid molecular oxygen. Our electrical conductivity measurements of fluid oxygen under dynamic quasi-isentropic compression show that a non-metal/metal transition occurs at…

Condensed Matter · Physics 2007-05-23 Marina Bastea , Arthur C. Mitchell , William J. Nellis

Lakshtanov et al. (2007) showed that incorporation of aluminum and some water into SiO2 significantly reduces the post-stishovite transition pressure in SiO2. This discovery suggested that the ferroelastic post-stishovite transition in…

Materials Science · Physics 2016-04-27 Koichiro Umemoto , Katsuyuki Kawamura , Kei Hirose , Renata M. Wentzcovitch

We study the temperature relaxation dynamics of nodal-line semimetals after a sudden excitation in the presence of acoustic and optical phonon modes. We find that the nodal line constrains the electron momenta in scattering processes and,…

Materials Science · Physics 2022-04-11 Benjamin M. Fregoso , Madhab Neupane , Anup Pradhan Sakhya

The ability to partially oxidize methane at low temperatures and pressures would have important environmental and economic applications. Although methane oxidation on gold nanoparticles has been observed experimentally, our density…

Materials Science · Physics 2014-08-28 Duncan J. Mowbray , Annapaola Migani , Guido Walther , David M. Cardamone , Angel Rubio

Understanding high-pressure transitions in prototypical linear diatomic molecules, such as hydrogen, nitrogen, and oxygen, is an important objective in high-pressure physics. Recent ultrahigh-pressure study on hydrogen revealed that there…

Materials Science · Physics 2019-10-31 Shan Liu , Meifang Pu , Qiqi Tang , Feng Zhang , Binbin Wu , Li Lei

Absorption of ultraviolet radiation by water ice coating interstellar grains can lead to dissociation and desorption of the ice molecules. These processes are thought to be important in the gas-grain chemistry in molecular clouds and…

Astrophysics · Physics 2009-11-13 S. Andersson , E. F. van Dishoeck