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The variational procedure to construct compact and accurate wave functions for three-electron atoms and ions is developed. The procedure is based on the use of six-dimensional gaussoids written in the relative four-body coordinates $r_{12},…

Atomic Physics · Physics 2011-01-11 Alexei M. Frolov , David M. Wardlaw

A variational approach is developed for bound state calculations in three- and four-electron atomic systems. This approach can be applied to determine, in principle, an arbitrary bound state in three- and four-electron ions and atoms. Our…

Atomic Physics · Physics 2015-05-19 Alexei M Frolov , David M. Wardlaw

The energy levels of the ground states of the three-particle and four-particle bound states of leptons in quantum electrodynamics are calculated. For the calculation, the variational method with Gaussian basis functions is used. The…

High Energy Physics - Phenomenology · Physics 2026-03-09 A. V. Eskin , A. P. Martynenko , F. A. Martynenko , D. K. Pometko

Results of accurate computations of bound states in three- and four-electron atomic systems are discussed. Bound state properties of the four-electron lithium ion Li$^{-}$ in its ground $2^{2}S-$state are determined from the results of…

Atomic and Molecular Clusters · Physics 2016-07-08 Alexei M. Frolov , David M. Wardlaw

By the use of the variational method with exponential trial functions the upper and lower bounds of energy are calculated for a number of non-relativistic three-body Coulomb and nuclear systems. The formulas for calculation of upper and…

Atomic Physics · Physics 2007-05-23 A. G. Donchev , N. N. Kolesnikov , V. I. Tarasov

A rigorous characterization of the information content of any highest-spin three-fermion wave function is presented. It is based upon a formal decomposition of the wave function into a finite set of fixed invariants, called shapes, whose…

Quantum Physics · Physics 2026-05-28 Jerzy Cioslowski , Krzysztof Strasburger , Denis K. Sunko

A one-electron Schroedinger equation based on special one-electron potentials for atoms is shown to exist that produces orbitals for an arbitrary molecule that are sufficiently accurate to be used without modification to construct single-…

Chemical Physics · Physics 2022-05-16 Jerry L. Whitten

The nodal structure of bound-state wave functions for one-dimensional quantum systems with quartic energy-momentum dispersion and polynomial potentials is analysed by using the semiclassical approximation and variational approach. For…

Strongly Correlated Electrons · Physics 2026-03-06 E. V. Gorbar , B. E. Grinyuk , V. P. Gusynin

In the framework of the study of helium-like atomic systems possessing the collinear configuration, we propose a simple method for computing compact but very accurate wave functions describing the relevant $S$ state. It is worth noting that…

Atomic Physics · Physics 2021-05-13 Evgeny Z. Liverts , Nir Barnea

A simple, seven-parameter trial function is proposed for a description of the ground state of the Lithium atom. It includes both spin functions. Inter-electronic distances appear in exponential form as well as in a pre-exponential factor,…

Atomic Physics · Physics 2015-05-13 Nicolais L. Guevara , Frank E Harris , Alexander V Turbiner

The resonance states of one- and two-particle Hamiltonians are studied using variational expansions with real basis-set functions. The resonance energies, $E_r$, and widths, $\Gamma$, are calculated using the density of states and an…

Atomic Physics · Physics 2013-06-19 Federico M. Pont , Pablo Serra , Omar Osenda

We propose an efficient basis expansion for electron orbitals to describe real-time electron dynamics in crystalline solids. Although a conventional grid representation in the three-dimensional Cartesian coordinates works robustly, it…

Materials Science · Physics 2014-07-02 Shunsuke A. Sato , Kazuhiro Yabana

The method of McCurdy, Baertschy, and Rescigno, J. Phys. B, 37, R137 (2004) is generalized to obtain a straightforward, surprisingly accurate, and scalable numerical representation for calculating the electronic wave functions of molecules.…

For a given many-electron molecule, it is possible to define a corresponding one-electron Schr\"odinger equation, using potentials derived from simple atomic densities, whose solution predicts fairly accurate molecular orbitals for single-…

Chemical Physics · Physics 2022-05-16 Jerry L. Whitten

The variational method, within the Hamiltonian formalism of reformulated QED is used to determine relativistic wave equations for a system of three fermions of arbitrary mass interacting electromagnetically. The interaction kernels of the…

Atomic Physics · Physics 2007-06-21 Mark Barham , Jurij W. Darewych

The Configuration Interaction (CI) method using a large Laguerre basis restricted to l = 0 orbitals is applied to the calculation of the He ground state. The maximum number of orbitals included was 60. The numerical evidence suggests that…

Atomic Physics · Physics 2007-05-23 J. Mitroy , M. W. J. Bromley , K. Ratnavelu

We present here a new approach to determine an accurate variational wavefunction for general quantum antiferromagnets, completely defined by the requirement to reproduce the simple and well known spin-wave expansion. By this wavefunction,…

Condensed Matter · Physics 2007-05-23 Franjo Franjic , Sandro Sorella

We present a variational wavefunction which explains the behaviour of the supersolid state formed by hard-core bosons on the triangular lattice. The wavefunction is a linear superposition of {\em only and all} configurations minimising the…

Statistical Mechanics · Physics 2009-11-13 Arnab Sen , Prasenjit Dutt , Kedar Damle , R. Moessner

Complete orthonormal sets of exponential-type orbitals with non-integer principal quantum numbers are discussed as basis functions in non-relativistic Hartree-Fock-Roothaan electronic structure calculations of atoms. A method is proposed to…

Quantum Physics · Physics 2025-07-08 Ali Bagci , Philip E. Hoggan

We describe bound states, resonances and elastic scattering of light ions using a $\delta$-shell potential. Focusing on low-energy data such as energies of bound states and resonances, charge radii, asymptotic normalization coefficients,…

Nuclear Theory · Physics 2019-11-11 Benjamin K. Luna , T. Papenbrock
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