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X-ray as well as electron diffraction are powerful tools for structure determination of molecules. Studies on randomly oriented molecules in the gas-phase address cases in which molecular crystals cannot be generated or the interaction-free…

Modifications of photoionization arising from resonant electron-electron correlations between neighbouring atoms in an atomic sample are studied. The sample contains atomic species A and B, with the ionization potential of A being smaller…

Atomic Physics · Physics 2015-06-04 B. Najjari , C. Müller , A. B. Voitkiv

The results are presented of a detailed combined experimental and theoretical investigation of the influence of coadsorbed electron-donating alkali atoms and the prototypical electron acceptor molecule TCNQ…

Ab initio electronic structure methods give accurate results for small systems, but do not scale well to large systems. Chemical insight tells us that molecular functional groups will behave approximately the same way in all molecules,…

Chemical Physics · Physics 2007-05-23 Benjamin G. Janesko , David Yaron

An adhesive unilateral contact between visco-elastic bodies at small strains and in a Kelvin-Voigt rheology is scrutinized, neglecting inertia. The flow-rule for debonding the adhesive is considered rate independent, unidirectional, and…

Analysis of PDEs · Mathematics 2013-09-30 Martin Kruzik , Christos G. Panagiotopoulos , Tomas Roubicek

We describe a QCD based model which incorporates the main properties of the inclusive particle distributions expected for diffractive processes, including the diffractive dissociation at high energies. We study, in turn, the total cross…

High Energy Physics - Phenomenology · Physics 2021-03-17 V. A. Khoze , A. D. Martin , M. G. Ryskin

We investigated the dissociation of dications and trications of three polycyclic aromatic hydrocarbons (PAHs), fluorene, phenanthrene, and pyrene. PAHs are a family of molecules ubiquitous in space and involved in much of the chemistry of…

We analyze the electric dipole moments (PDMs) and static electric dipole polarizabilities of the alkali--alkaline-earth (Alk-AlkE) dimers by employing finite-field coupled-cluster methods, both in the frameworks of non-relativistic and…

Atomic Physics · Physics 2022-06-29 R. Mitra , V. S. Prasannaa , B. K. Sahoo

It is shown that the dipole moment of polar (water, methanol, formamide, acetone and acetonitrile) molecules in the neighborhood of a cation is increased primarily by polarization from the bare electrostatic charge of the cation, although…

Chemical Physics · Physics 2021-03-31 Imre Bakó , Dániel Csókás , István Mayer , Szilvia Pothoczki , László Pusztai

We study the core hole-electron correlation in coherently coupled molecules by energy dispersive near edge X-ray absorption fine-structure spectroscopy. In a transient phase, which exists during the transition between two bulk arrangements,…

Materials Science · Physics 2013-12-03 M. Scholz , F. Holch , C. Sauer , M. Wiessner , A. Schöll , F. Reinert

Electron-electron correlation forms the basis of difficulties encountered in many-body physics. Accurate treatment of the correlation problem is likely to unravel some nice physical properties of matter embedded in the correlation. In an…

Atomic Physics · Physics 2021-03-17 E. Jobunga

In the context of describing electrons in solids as a fluid in the hydrodynamic regime, we consider a flow of electrons in a channel of finite width, i.e.~a Poiseuille flow. The electrons are accelerated by a constant electric field. We…

Mesoscale and Nanoscale Physics · Physics 2018-12-05 Johanna Erdmenger , Ioannis Matthaiakakis , Rene Meyer , David Rodríguez Fernández

Fusion of lipid bilayers in membranes is important in processes from vesicle-cell interactions (as in drug delivery) to exosome-cell signaling, while transient transmembrane electric fields are known to occur spontaneously. Two contacting…

Soft Condensed Matter · Physics 2024-04-09 Yu Zhang , Di Jin , Jacob Klein

We investigate the molecular acceptors 3,4,9,10-perylene-tetracarboxylic acid dianhydride (PTCDA), 2,3,5,6-tetra uoro-7,7,8,8-tetracyanoquinodimethane (F4TCNQ), and 4,5,9,10-pyrenetetraone (PYTON) on Ag(111) using densityfunctional theory.…

Materials Science · Physics 2015-06-17 Oliver T. Hofmann , Viktor Atalla , Nikolaj Moll , Patrick Rinke , Matthias Scheffler

First-principles calculations are performed to investigate the interaction of physisorbed small molecules, including CO, H2, H2O, NH3, NO, NO2, and O2, with phosphorene, and their energetics, charge transfer, and magnetic moment are…

Materials Science · Physics 2015-02-17 Yongqing Cai , Qingqing Ke , Gang Zhang , Yong-Wei Zhang

Interactions between silica surfaces across isopropanol solutions are measured with colloidal probe technique based on atomic force microscope. In particular, the influence of 1:1 electrolytes on the interactions between silica particles is…

Soft Condensed Matter · Physics 2020-07-01 Biljana Stojimirovic , Marco Galli , Gregor Trefalt

Amino acids are essential to all life. However, our understanding of some aspects of their intrinsic structure, molecular chemistry, and electronic structure is still limited. In particular the nature of amino acids in their crystalline…

Materials Science · Physics 2020-11-02 Anna Regoutz , Marta S. Wolinska , Nathalie K. Fernando , Laura E. Ratcliff

Electrostatics plays a key role in biomolecular assembly. Oppositely charged biomolecules, for instance, can co-assembled into functional units, such as DNA and histone proteins into nucleosomes and actin-binding protein complexes into…

Materials Science · Physics 2009-11-11 Y. S. Velichko , M. Olvera de la Cruz

Quantum interference between multiple pathways in molecular photodissociation often results in angular momentum polarization of atomic products and this can give deep insight into fundamental physical processes. For dissociation of diatomic…

Chemical Physics · Physics 2022-04-26 Chaya Weeraratna , Arthur G. Suits , Oleg S. Vasyutinskii

The theoretical description and the properties of Frenkel excitons in non-covalently bonded molecular aggregates are reviewed from a multi-exciton perspective of dissipative quantum dynamics. First, the photophysical and quantum chemical…

Chemical Physics · Physics 2012-04-23 Oliver Kühn , Stefan Lochbrunner