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We study the dynamics of a molecule's nuclear wave-function near an avoided crossing of two electronic energy levels, for one nuclear degree of freedom. We derive the general form of the Schroedinger equation in the n-th superadiabatic…

Mathematical Physics · Physics 2015-05-13 Volker Betz , Benjamin D. Goddard , Stefan Teufel

We explain the concept of superadiabatic approximations and show how in the context of the Born- Oppenheimer approximation they lead to an explicit formula that can be used to predict transitions at avoided crossings. Based on this formula,…

Chemical Physics · Physics 2016-06-29 Volker Betz , Benjamin D. Goddard , Uwe Manthe

We consider non-adiabatic transitions in multiple dimensions, which occur when the Born-Oppenheimer approximation breaks down. We present a general, multi-dimensional algorithm which can be used to accurately and efficiently compute the…

Chemical Physics · Physics 2018-04-16 V. Betz , B. D. Goddard , T. Hurst

Non-adiabatic quantum effects, often experimentally observed in semiconductors nano-devices such as single-electron pumps operating at high frequencies, can result in undesirable and uncontrollable behaviour. However, when combined with the…

Mesoscale and Nanoscale Physics · Physics 2022-02-16 Alan Gardin , Ross D. Monaghan , Tyler Whittaker , Rajib Rahman , Giuseppe C. Tettamanzi

We study non--adiabatic transitions in scattering theory for the time dependent molecular Schroedinger equation in the Born--Oppenheimer limit. We assume the electron Hamiltonian has finitely many levels and consider the propagation of…

Mathematical Physics · Physics 2009-11-10 G. A. Hagedorn , A. Joye

We consider nonadiabatic systems in which the classical Born-Oppenheimer approximation breaks down. We present a general theory that accurately captures the full transmitted wavepacket after multiple transitions through either a single or…

Chemical Physics · Physics 2018-04-16 Benjamin D. Goddard , Tim Hurst

The anomalous dynamical evolution and the crossing of nonadiabatic energy levels are investigated for exactly solvable time-dependent quantum systems through a reverse-engineering scheme. By exploiting a typical driven model, we elucidate…

Quantum Physics · Physics 2020-01-08 Hong Cao , Shao-Wu Yao , Li-Xiang Cen

A non-adiabatic nuclear wavepacket dynamics simulation of the H$_2$O$^+$ de-excitation process is performed based on electronic structure calculations using the variational quantum eigensolver. The adiabatic potential energy surfaces and…

Quantum Physics · Physics 2022-03-02 Hirotoshi Hirai , Sho Koh

Motivated by experiments with current biased superconducting atomic point contacts the general problem of nonadiabatic transitions between adiabatic surfaces in presence of strong dissipation is studied. For a single channel device the…

Mesoscale and Nanoscale Physics · Physics 2009-06-05 Hans Fritz , Joachim Ankerhold

A novel method of coherent manipulation of the electron tunneling in quantum-dots is proposed, which utilizes the quantum interference in nonadiabatic double-crossing of the discrete energy levels. In this method, we need only a smoothly…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 Keiji Saito , Yosuke Kayanuma

We present an approach for carrying out non-adiabatic molecular dynamics simulations of systems in which non-adiabatic transitions arise from the coupling between the classical atomic motions and a quasi-continuum of electronic quantum…

Computational Physics · Physics 2018-11-21 Jerome Daligault , Dmitry Mozyrsky

We examine structural and dynamical properties of quantum resonances associated with an avoided crossing and identify the parameter shifts where these properties attain maximal or extreme values, first at a general level, and then for a…

Quantum Physics · Physics 2015-05-13 I. Lizuain , E. Hernandez-Concepcion , J. G. Muga

Transitions in an artificial atom, driven non-adiabatically through an energy-level avoided crossing, can be controlled by carefully engineering the driving protocol. We have driven a superconducting persistent-current qubit with a…

We examine time-resolved X-ray diffraction from molecules in the gas phase which undergo nonadiabatic avoided-crossing dynamics involving strongly coupled electrons and nuclei. Several contributions to the signal are identified,…

Chemical Physics · Physics 2017-05-30 Markus Kowalewski , Kochise Bennett , Shaul Mukamel

We present a method to study rare nonadiabatic dynamics in open quantum systems using transition path sampling and quantum jump trajectories. As with applications of transition path sampling to classical dynamics, the method does not rely…

Statistical Mechanics · Physics 2021-12-08 Addison J. Schile , David T. Limmer

We exploit the concept of Landau-Zener transitions at avoided energy crossings as a quantum-control tool. In an avoided crossing the two quantum states interchange their characteristics as an external parameter is varied. Depending on the…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 D. A. Wisniacki , G. E. Murgida , P. I. Tamborenea

We analyze the propagation of coherent states through general systems of pseudodifferential form associated with Hamiltonian presenting codimension one eigen-value crossings. In particular, we calculate precisely the non adiabatic effects…

Analysis of PDEs · Mathematics 2021-07-21 Clotilde Fermanian-Kammerer , Caroline Lasser , Didier Robert

In this manuscript we report on adiabatic pumping in quasiperiodic stiffness modulated beams. We show that distinct topological states populating nontrivial gaps can nucleate avoided crossings characterized by edge-to-edge transitions. Such…

Applied Physics · Physics 2020-07-15 Emanuele Riva , Vito Casieri , Ferruccio Resta , Francesco Braghin

We discuss adiabatic quantum phenomena at a level crossing. Given a path in the parameter space which passes through a degeneracy point, we find a criterion which determines whether the adiabaticity condition can be satisfied. For paths…

Quantum Physics · Physics 2007-05-23 Mateusz Cholascinski

The approach by Ettore Majorana for non-adiabatic transitions between two quasi-crossing levels is revisited. We rederive the transition probability, known as the Landau-Zener-St\"{u}ckelberg-Majorana formula, and introduce Majorana's…

Quantum Physics · Physics 2024-08-20 Polina O. Kofman , Oleh V. Ivakhnenko , Sergey N. Shevchenko , Franco Nori
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