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Multi-band Gutzwiller-correlated wave functions reconcile the contrasting concepts of itinerant band electrons versus electrons localized in partially filled atomic shells. The exact evaluation of these variational ground states in the…

Strongly Correlated Electrons · Physics 2007-05-23 W. Weber , J. Buenemann , F. Gebhard

Upon reduction of the film thickness we observe a metal-insulator transition in epitaxially stabilized, spin-orbit coupled SrIrO$_3$ ultrathin films. By comparison of the experimental electronic dispersions with density functional theory at…

Strongly Correlated Electrons · Physics 2017-12-27 P. Schütz , D. Di Sante , L. Dudy , J. Gabel , M. Stübinger , M. Kamp , Y. Huang , M. Capone , M. -A. Husanu , V. Strocov , G. Sangiovanni , M. Sing , R. Claessen

We investigate the effect of pressure on the electronic and magnetic states of CdV$_2$O$_4$ by using ab initio electronic structure calculations. The Coulomb correlation and spin-orbit coupling play important role in deciding the…

Strongly Correlated Electrons · Physics 2012-08-06 Sudhir K. Pandey

Studies of different experimental groups that explore the properties of a two-dimensional electron gas in silicon semiconductor systems ((100) Si metal-oxide-semiconductor field-effect transistors (MOSFETs) and (100) SiGe/Si/SiGe quantum…

Strongly Correlated Electrons · Physics 2019-10-15 V. T. Dolgopolov

Skutterudites are promising materials for thermoelectric and spintronics applications. Here we explore spin fluctuations in the FeSb$_{3}$ skutterudite and their effect on its electronic structure using Hubbard-corrected density-functional…

Materials Science · Physics 2026-01-29 Enrico Di Lucente , Flaviano José dos Santos , Nicola Marzari

LiV$_2$O$_4$ is a member of the so-called $3d$ heavy fermion compounds, with effective electron mass exceeding 60 times the free electron mass, comparable to $4f$ heavy fermion compounds. The origin of the strong electron correlation in…

Strongly Correlated Electrons · Physics 2025-01-07 Steffen Backes , Yusuke Nomura , Ryotaro Arita , Hiroshi Shinaoka

Dynamical properties of the lattice structure was studied by optical spectroscopy in ACr2O4 chromium spinel oxide magnetic semiconductors over a broad temperature region of T=10-335K. The systematic change of the A-site ions (A=Mn, Fe, Co,…

Strongly Correlated Electrons · Physics 2013-07-24 V. Kocsis , S. Bordács , D. Varjas , K. Penc , A. Abouelsayed , C. A. Kuntscher , K. Ohgushi , Y. Tokura , I. Kézsmárki

Electronic structure calculations obtained with an approach with density functional theory with an enhanced local Coulomb interaction, DFT+$U$, are presented for the relativistic magnetic insulator Sr$_{2}$IrO$_{4}$. The results are in…

Strongly Correlated Electrons · Physics 2013-12-20 Shreemoyee Ganguly , Oscar Granas , Lars Nordstrom

We investigate the violation of the first Hund's rule in 4$d$ and 5$d$ transition metal oxides that form solids of dimers. Bonding states within these dimers reduce the magnetization of such materials. We parametrize the dimer formation…

Strongly Correlated Electrons · Physics 2019-01-16 Malte Harland , Alexander I. Poteryaev , Sergey V. Streltsov , Alexander I. Lichtenstein

The Hohenberg-Kohn theorem of density functional theory (DFT) for the case of electrons interacting with an external magnetic field (that couples to spin only) is examined in more detail than previously. A unexpected generalization is…

Strongly Correlated Electrons · Physics 2009-10-31 H. Eschrig , W. E. Pickett

We have investigated the electronic structure of fluorite Cu$_{2}$Se using density functional theory calculations within the LDA, PBE and AM05 approximations as well as with the non-local hybrid PBE0 and HSE approximations. Our results show…

Materials Science · Physics 2013-03-04 Mikael Råsander , Lars Bergqvist , Anna Delin

The semiconductor Sr2FeOsO6, depending on temperature, adopts two types of spin structures that differ in the spin sequence of ferrimagnetic iron - osmium layers along the tetragonal c-axis. Neutron powder diffraction experiments, 57Fe…

Alloying effects by T=Mn,Co,Ni-substitution on FeS$_2$ have been investigated using density-functional calculations. The ferromagnetic alloys Fe$_{1-x}$T$_x$S$_2$ have been investigated for concentrations…

Materials Science · Physics 2015-12-16 Abdesalem Houari , Peter E. Blöchl

We investigate the thickness-dependent electronic structure of ultrathin SrIrO$_3$ and discover a transition from a semimetallic to a correlated insulating state below 4 unit cells. Low-temperature magnetoconductance measurements show that…

The chromium spinels MgCr2O4 and ZnCr2O4 are prime examples of the highly frustrated pyrochlore lattice antiferromagnet. Experiment has carefully established that both materials, upon cooling, distort to lower symmetry and order…

Strongly Correlated Electrons · Physics 2025-02-28 Ludovic D. C. Jaubert , Yasir Iqbal , Harald O. Jeschke

In contrast to the previous reports that the divalent perovskite SrCrO$_3$ was believed to be cubic structure and nonmagnetic metal, recent measurements suggest coexistence of majority tetragonally distorted weak antiferromagnetic phase and…

Strongly Correlated Electrons · Physics 2009-10-01 K. -W. Lee , W. E. Pickett

We investigate magnetic properties of the $s$ = 1/2 compound K$_{2}$Cu$_{3}$(MoO$_{4}$)$_{4}$ by combining magnetic susceptibility, magnetization, specific heat, and electron spin resonance (ESR) with density functional calculations. Its…

Density functional calculations are used to investigate the doping dependence of the electronic structure and magnetic properties in hexagonal Na$_x$CoO$_2$. The electronic structure is found to be highly two dimensional, even without…

Superconductivity · Physics 2009-11-10 D. J. Singh

Using the first-principles density functional approach, we investigate Ca$_2$FeOsO$_6$, a material of double perovskite structure synthesized recently. According to the calculations, Ca$_2$FeOsO$_6$ is a ferrimagnetic Mott-insulator…

Mesoscale and Nanoscale Physics · Physics 2017-01-04 Madhav P. Ghimire , Xiao Hu

We present the self-interaction corrected local spin density (SIC-LSD) electronic structure and total energy calculations, leading also to valencies of the ground state configurations, for the half-metallic double perovskites such as…

Strongly Correlated Electrons · Physics 2009-11-10 Z. Szotek , W. M. Temmerman , A. Svane , L. Petit , H. Winter