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We present a quantum mechanical theory of optically induced dynamic nuclear polarization applicable to quantum dots and other interacting spin systems. The exact steady state of the optically driven coupled electron-nuclear system is…

Mesoscale and Nanoscale Physics · Physics 2019-02-04 Thomas Nutz , Edwin Barnes , Sophia E. Economou

We investigate in micro-photoluminescence experiments the dynamical nuclear polarization in individual InGaAs quantum dots. Experiments carried out in an applied magnetic field of 2T show that the nuclear polarization achieved through the…

Other Condensed Matter · Physics 2009-11-13 B. Urbaszek , P. -F. Braun , X. Marie , O. Krebs , A. Lemaitre , P. Voisin , T. Amand

We report on the influence of hyperfine interaction on the optical orientation of singly charged excitons X+ and X- in self-assembled InAs/GaAs quantum dots. All measurements were carried out on individual quantum dots studied by…

Materials Science · Physics 2009-04-10 O. Krebs , B. Eble , A. Lemaître , P. Voisin , B. Urbaszek , X. Marie , T. Amand

Sharp threshold-like transitions between two stable nuclear spin polarizations are observed in optically pumped individual InGaAs self-assembled quantum dots embedded in a Schottky diode when the bias applied to the diode is tuned. The…

Current-induced electron spin polarization is shown to produce nuclear hyperpolarization through dynamic nuclear polarization. Saturated fields of several millitesla are generated upon the application of electric field over a timescale of a…

Mesoscale and Nanoscale Physics · Physics 2014-10-31 C. J. Trowbridge , B. M. Norman , Y. K. Kato , D. D. Awschalom , V. Sih

We demonstrate dynamical nuclear spin polarization in the absence of an external magnetic field, by resonant circularly polarized optical excitation of a single electron or hole charged quantum dot. Optical pumping of the electron spin…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 C. W. Lai , P. Maletinsky , A. Badolato , A. Imamoglu

We demonstrate that efficient optical pumping of nuclear spins in semiconductor quantum dots (QDs) can be achieved by resonant pumping of optically "forbidden" transitions. This process corresponds to one-to-one conversion of a photon…

Mesoscale and Nanoscale Physics · Physics 2015-05-13 E. A. Chekhovich , M. N. Makhonin , K. V. Kavokin , A. B. Krysa , M. S. Skolnick , A. I. Tartakovskii

We propose a new method for dynamic nuclear polarisation in a quasi one-dimensional quantum wire utilising the spin-orbit interaction, the hyperfine interaction, and a finite source-drain potential difference. In contrast with current…

Mesoscale and Nanoscale Physics · Physics 2008-03-05 V. Tripathi , A. C. H. Cheung , N. R. Cooper

We investigate how the strain-induced nuclear quadrupole interaction influences the degree of nuclear spin polarization in self-assembled quantum dots. Our calculation shows that the achievable nuclear spin polarization in In_{x}Ga_{1-x}As…

Mesoscale and Nanoscale Physics · Physics 2013-05-29 Chia-Wei Huang , Xuedong Hu

Optical and electrical control of the nuclear spin system allows enhancing the sensitivity of NMR applications and spin-based information storage and processing. Dynamic nuclear polarization in semiconductors is commonly achieved in the…

Mesoscale and Nanoscale Physics · Physics 2014-09-09 G. Sallen , S. Kunz , T. Amand , L. Bouet , T. Kuroda , T. Mano , D. Paget , O. Krebs , X. Marie , K. Sakoda , B. Urbaszek

We investigated optical spin orientation and dynamic nuclear polarization (DNP) in individual self-assembled InGaAs/GaAs quantum dots (QDs) doped by a single Mn atom, a magnetic impurity providing a neutral acceptor A$^0$ with an effective…

Mesoscale and Nanoscale Physics · Physics 2016-11-15 O. Krebs , E. Baudin , A. Lemaître

Exciton spin and related optical polarization in self-assembled InAs/In$_{0.53}$Ga$_{0.23}$Al$_{0.24}$As/InP(001) quantum dashes emitting at 1.55 {\mu}m are investigated by means of polarization- and time-resolved photoluminescence, as well…

Mesoscale and Nanoscale Physics · Physics 2018-07-25 M. Syperek , Ł. Dusanowski , M. Gawełczyk , G. Sęk , A. Somers , J. P. Reithmaier , S. Höfling , J. Misiewicz

We investigate the dynamic nuclear polarization from the hyperfine interaction between nonequilibrium electronic spins and nuclear spins coupled to them in semiconductor nanostructures. We derive the time and position dependence of the…

Materials Science · Physics 2007-05-23 Ionel Tifrea , Michael E. Flatte

Using the emission of the positively charged exciton as a probe, we analyze the dynamics of the optical pumping and the dynamics of the relaxation of a Mn spin exchange-coupled with a confined hole spin in a II-VI semiconductor quantum dot.…

Mesoscale and Nanoscale Physics · Physics 2015-06-22 B. Varghese , H. Boukari , L. Besombes

We investigate the dynamic nuclear polarization process by frequently injecting polarized electron spins into a quantum dot. Due to the suppression of the direct dipolar and indirect electron-mediated nuclear spin interactions, by the…

Mesoscale and Nanoscale Physics · Physics 2016-07-26 Na Wu , Wenkui Ding , Anqi Shi , Wenxian Zhang

We investigate site-controlled In$_{0.25}$Ga$_{0.75}$As quantum dots in (111)B GaAs pyramidal recesses as spin qubits. Combining scanning confocal cryomicroscopy, magneto-photoluminescence studies and resonant excitation, we identify and…

Mesoscale and Nanoscale Physics · Physics 2025-09-09 R. A. Barcan , I. Samaras , K. Barr , G. Juska , E. Pelucchi , K. G. Lagoudakis

The ability to discriminate between simultaneously occurring noise sources in the local environment of semiconductor InGaAs quantum dots, such as electric and magnetic field fluctuations, is key to understanding their respective dynamics…

Mesoscale and Nanoscale Physics · Physics 2014-11-18 Megan J. Stanley , Clemens Matthiesen , Jack Hansom , Claire Le Gall , Carsten H. H. Schulte , Edmund Clarke , Mete Atatüre

We studied the zero-field dynamic nuclear spin polarization in a single In$_{0.75}$Al$_{0.25}$As/Al$_{0.3}$Ga$_{0.7}$As quantum dot. Even without any external magnetic field, the positive trion excited by the circularly-polarized light…

Mesoscale and Nanoscale Physics · Physics 2017-03-20 Ryosuke Matsusaki , Reina Kaji , Sohta Yamamoto , Hirotaka Sasakura , Satoru Adachi

By using highly time-resolved spectroscopy with an alternative {\sigma}+/{\sigma} - laser pulse modulation technique, we are able to measure the fast buildup and decay times of the dynamical nuclear spin polarization (DNSP) at 5 K for a…

Mesoscale and Nanoscale Physics · Physics 2015-06-03 X. M. Dou , B. Q. Sun , D. S. Jiang , H. Q. Ni , Z. C. Niu

The interplay of optical driving and hyperfine interaction between an electron confined in a quantum dot and its surrounding nuclear spin environment produces a range of interesting physics such as mode-locking. In this work, we go beyond…

Mesoscale and Nanoscale Physics · Physics 2024-03-12 Arian Vezvaee , Gargee Sharma , Sophia E. Economou , Edwin Barnes