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High-harmonic generation (HHG) in condensed-matter systems is both a source of fundamental insight into quantum electron motion and a promising candidate to realize compact ultraviolet and ultrafast light sources. Here we argue that the…

Mesoscale and Nanoscale Physics · Physics 2017-03-08 Joel D. Cox , Andrea Marini , F. Javier García de Abajo

We theoretically investigate high-order harmonic generation (HHG) in Rydberg atoms driven by spatially inhomogeneous laser fields, induced, for instance, by plasmonic enhancement. It is well known that the laser intensity should to exceed…

Atomic Physics · Physics 2016-07-08 Y. Tikman , I. Yavuz , M. F. Ciappina , A. Chacon , Z. Altun , M. Lewenstein

Employing non-Hermitian Floquet theory, the strong-field process of high harmonic (HH) generation by a classical continuous-wave field irradiating ground-state atom is discovered to be controllable by placing the irradiated atom inside a…

Quantum Physics · Physics 2025-09-05 Zohar Amitay , Nimrod Moiseyev

We demonstrate that high-harmonic generation (HHG) in solids dominantly originates from strongly localized surface states through non-perturbative processes. Measurements reveal that HHG from bulk states is suppressed by at least 1-2 orders…

Optics · Physics 2018-05-02 J. Seres , E. Seres , C. Serrat , T. Schumm

The generation of harmonics by atoms interacting with two circularly polarized and frequency related laser fields is addressed through ab initio numerical simulations. A detailed charaterization of a few specific harmonics is given. In…

Atomic Physics · Physics 2009-11-10 F. Ceccherini , N. Davini , D. Bauer , F. Cornolti

We present theoretical predictions of high-order harmonic generation (HHG) resulting from the interaction of short femtosecond laser pulses with metal nanotips. It has been demonstrated that high energy electrons can be generated using…

Anomalous high-harmonic generation (HHG) arises in certain solids when irradiated by an intense laser field, as the result of a nonlinear perpendicular current akin to a Hall current. Here, we theoretically characterize the anomalous HHG…

Optics · Physics 2023-05-03 Lun Yue , Mette B. Gaarde

High harmonic generation (HHG) is a powerful probe of electron dynamics on attosecond to femtosecond timescales and has been successfully used to detect electronic and structural changes in solid-state quantum materials, including…

Materials Science · Physics 2026-01-21 Daniel A. Rehn , Towfiq Ahmed , Jinkyoung Yoo , Rohit Prasankumar , Jian-Xin Zhu

High-order harmonic generation (HHG) from molecular ion HeH$^{2+}$ in two initial states of $1s\sigma$ (ground state) and $2p\sigma$ (first excited state) is investigated theoretically, in homogeneous and plasmonic-enhanced laser fields.…

Atomic Physics · Physics 2018-07-04 Nehzat Safaei

Applying time-dependent local density approximation (TDLDA), we study the high-order harmonic generation (HHG) of ethylene subjected to the one-color ($\omega=2.72$ eV) and the two-color ($\omega_1=2.72$ eV and $\omega_2=5.44$ eV)…

Atomic and Molecular Clusters · Physics 2009-03-31 Z. P. Wang , P. M. Dinh , P. -G. Reinhard , E. Suraud , F. S. Zhang

We perform a detailed analysis of high-order harmonic generation in diatomic molecules within the strong-field approximation, with emphasis on quantum-interference effects. Specifically, we investigate how the different types of electron…

Atomic Physics · Physics 2011-11-10 C. Figueira de Morisson Faria

The polarization state of light plays a central role in strong-field light--matter interactions and is widely used to probe electronic structure in solids via high-order harmonic generation (HHG). In particular, helicity-resolved HHG has…

We theoretically study multielectron effects in high-harmonic generation (HHG), using all-electron first-principles simulations for a one-dimensional (1D) model atom. In addition to usual plateau and cutoff (from a cation in the present…

Atomic Physics · Physics 2017-05-24 Iliya Tikhomirov , Takeshi Sato , Kenichi L. Ishikawa

High-harmonic generation (HHG), a typical nonlinear optical effect, has been actively studied in electron systems such as semiconductors and superconductors. As a natural extension, we theoretically study HHG from electric polarization,…

Strongly Correlated Electrons · Physics 2020-03-10 Tatsuhiko N. Ikeda , Masahiro Sato

In quantum sideband high harmonic generation (QSHHG), high harmonic generation is perturbed by a bright quantum field resulting in harmonic sidebands, with the intent to transfer non-classical properties from the quantum perturbation to the…

Quantum Physics · Physics 2025-05-29 Neda Boroumand , Adam Thorpe , Graeme Bart , Lu Wang , David N. Purschke , Giulio Vampa , Thomas Brabec

We perform a detailed analysis of high-order harmonic generation (HHG) in atoms within the strong field approximation (SFA) by considering spatially inhomogeneous monochromatic laser fields. We investigate how the individual pairs of…

Atomic Physics · Physics 2015-06-05 T. Shaaran , M. F. Ciappina , M. Lewenstein

We present ab initio calculations using the $R$-matrix with time dependence (RMT) method for high-order harmonic generation (HHG) in argon in a short, intense pulse regime. The calculations employ a $6$-cycle $\sin^2$ pulse at $850$ nm with…

Atomic Physics · Physics 2026-04-23 Aaron T. Bondy , Klaus Bartschat

High-harmonic generation is typically thought of as a sub-laser-cycle process, with the electron's excursion in the continuum lasting a fraction of the optical cycle. However, it was recently suggested that long-lived Rydberg states can…

We observe a new regime of coherent XUV radiation generation in noble gases induced by femtosecond pulses at very high intensities. This XUV emission has both a reduced divergence and spectral width as compared to high-order harmonic…

We analytically describe the strong-field light-electron interaction using a quantized coherent laser state with arbitrary photon number. We obtain a light-electron wave function which is a closed-form solution of the time-dependent…

Atomic Physics · Physics 2017-03-20 I. A. Gonoskov , N. Tsatrafyllis , I. K. Kominis , P. Tzallas
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