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Ultrafast heating of FeRh by a femtosecond laser pulse launches a magneto-structural phase transition from an antiferromagnetic to a ferromagnetic state. Aiming to reveal the ultrafast kinetics of this transition, we studied magnetization…

Femtosecond laser light can transfer spin angular momentum between magnetic subspecies that exhibit hybridized valence bands within an alloy or compound, and represents the fastest route for manipulating the magnetization of a material. To…

Laser pulses are known to induce symmetric demagnetization: equal loss of magnetic moments in the identical sublattices of antiferromagnets and ferromagnets at ultrashort timescales. Using time-dependent density functional theory, we show…

Materials Science · Physics 2026-02-19 Zhaobo Zhou , Sangeeta Sharma , John Kay Dewhurst , Junjie He

Femtosecond laser pulses can be used to induce ultrafast changes of the magnetization in magnetic materials. Several microscopic mechanisms have been proposed to explain the observations, including the transport of ultrashort spin-polarized…

The discovery of femtosecond laser-induced ultrafast demagnetization in 1996 opened a new field, femtomagnetism, in which magnetic order can be quenched on timescales shorter than a picosecond. This seminal observation revealed that angular…

Materials Science · Physics 2026-04-29 Quentin Remy , Stéphane Mangin

Controlling ultrafast magnetization dynamics by a femtosecond laser is attracting interest both in fundamental science and industry because of the potential to achieve magnetic domain switching at ever advanced speed. Here we report…

Materials Science · Physics 2013-09-09 C. Ruchert , C. Vicario , F. Ardana-Lamas , P. M. Derlet , B. Tudu , J. Luning , C. P. Hauri

The idea to utilize not only the charge but also the spin of electrons in the operation of electronic devices has led to the development of spintronics, causing a revolution in how information is stored and processed. A novel advancement…

Mesoscale and Nanoscale Physics · Physics 2016-02-10 T. J. Huisman , R. V. Mikhaylovskiy , J. D. Costa , F. Freimuth , E. Paz , J. Ventura , P. P. Freitas , S. Blügel , Y. Mokrousov , Th. Rasing , A. V. Kimel

The ultrafast response to an optical pulse excitation of the spin-spin exchange interaction in transition metal anti-ferromagnets is studied within the framework of the time-dependent spin-density functional theory. We propose a formulation…

Mesoscale and Nanoscale Physics · Physics 2017-08-16 Jacopo Simoni , Maria Stamenova , Stefano Sanvito

The diverse nodal spin structures in d/g/i-wave altermagnets (AM) may cause distinct light-induced spin responses yet remain poorly understood. Using time-dependent density functional theory (TDDFT), we reveal that laser induced ultrafast…

Materials Science · Physics 2026-02-17 Zhaobo Zhou , Sangeeta Sharma , Junjie He

We analyze theoretically the novel pathway of ultrafast spin dynamics for ferromagnets with high enough single-ion anisotropy (non-Heisenberg ferromagnets). This longitudinal spin dynamics includes the coupled oscillations of the modulus of…

Strongly Correlated Electrons · Physics 2013-10-28 E. G. Galkina , V. I. Butrim , Yu. A. Fridman , B. A. Ivanov , F. Nori

Efficient and fast manipulation of antiferromagnets has to date remained a challenging task, hindering their application in spintronic devices. For ultrafast operation of such devices, it is highly desirable to be able to control the…

Materials Science · Physics 2023-05-31 Markus Weißenhofer , Francesco Foggetti , Ulrich Nowak , Peter M. Oppeneer

We demonstrate a novel method for the excitation of sizable magneto-optical effects in Au by means of the laser-induced injection of hot spin-polarized electrons in Au/Fe/MgO(001) heterostructures. It is based on the energy- and…

Mesoscale and Nanoscale Physics · Physics 2019-02-20 A. Alekhin , I. Razdolski , M. Berritta , D. Bürstel , V. Temnov , D. Diesing , U. Bovensiepen , G. Woltersdorf , P. M. Oppeneer , A. Melnikov

Ultrafast magnetization dynamics in metallic heterostructures consists of a combination of local demagnetization in the ferromagnetic constituent and spin-dependent transport contributions within and in between the constituents. Separation…

Ferrimagnets containing several partially compensated magnetic sublattices are considered the most promising materials for all-optical data storage and for ultrafast communications based on spin waves. There are two magnetic phases of the…

This paper presents a theoretical investigation of electron-magnon scattering processes in the ultrafast demagnetization in itinerant ferromagnets. In the framework of a ferromagnetic model system, we compute the spin-dependent dynamics of…

Materials Science · Physics 2026-03-10 Félix Dusabirane , Kai Leckron , Baerbel Rethfeld , Hans Christian Schneider

We present an extension to simple s-d models, aiming at simulating ultrafast magnetization dynamics and spin transport in metallic heterostructures. In particular, we consider an alternative spin dissipation channel due to a finite exchange…

Materials Science · Physics 2023-06-14 Quentin Remy

Since the beginning of femtomagnetism, it has been hotly debated how an ultrafast laser pulse can demagnetize a sample and switch its spins within a few hundred femtoseconds, but no consensus has been reached. In this paper, we propose that…

Materials Science · Physics 2015-06-22 G. P. Zhang , Mingqiang Gu , X. S. Wu

Ab initio and model calculations demonstrate that the spin motion of electrons transmitted through ferromagnetic films can be analyzed in detail by means of angle- and spin-resolved core-level photoelectron spectroscopy. The spin motion…

Condensed Matter · Physics 2013-05-29 J. Henk , P. Bose , Th. Michael , P. Bruno

This year the discovery of femtosecond demagnetization by laser pulses is 20 years old. For the first time this milestone work by Bigot and coworkers gave insight in a very direct way into the time scales of microscopic interactions that…

Mesoscale and Nanoscale Physics · Physics 2016-09-14 J. Walowski , M. Münzenberg

Laser-induced femtosecond magnetism or femtomagnetism simultaneously relies on two distinctive contributions: (a) the optical dipole interaction (ODI) between a laser field and a magnetic system and (b) the spin expectation value change…

Materials Science · Physics 2012-02-21 M. S. Si , G. P. Zhang