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We identify carrier scattering at densities below which it has previously been observed in semiconductor quantum wells. These effects are evident in the peakshapes of 2D double-quantum spectra, which change as a function of excitation…

Optics · Physics 2016-05-25 Jonathan O. Tollerud , Jeffrey A. Davis

Studying the excited states of doublets is challenging for their typically multiconfigurational character. We employ light-scanning-tunneling microscopy (light-STM) to investigate photon-induced currents on a single open-shell PTCDA anion…

Atomic and Molecular Clusters · Physics 2025-02-14 Rodrigo Cezar de Campos Ferreira , Amandeep Sagwal , Jiří Doležal , Tomáš Neuman , Martin Švec

It is controversial what is the true role of entanglement in two-photon virtual-state spectroscopy [Saleh et al, Phys. Rev. Lett. 80, 3483, 1998], a two-photon absorption spectroscopic technique that can retrieve information about the…

Quantum Physics · Physics 2015-06-11 R. de J. León-Montiel , J. Svozilík , L. J. Salazar-Serrano , J. P. Torres

We introduce the particle-hole map (PHM), a visualization tool to analyze electronic excitations in molecules in the time or frequency domain, to be used in conjunction with time-dependent density-functional theory (TDDFT) or other ab…

Chemical Physics · Physics 2015-10-15 Yonghui Li , Carsten A. Ullrich

Resonant two-photon ionization in a system consisting of two spatially well-separated atoms is studied. Due to two-center electron-electron correlations, the ionization may also proceed through photo-excitation of both atoms with subsequent…

Atomic Physics · Physics 2015-05-27 C. Müller , A. B. Voitkiv

Double deeply virtual Compton scattering (DDVCS) is the process where an electron scatters off a nucleon and produces a lepton pair. The main advantage of this process in contrast with deeply virtual and timelike Compton scatterings (DVCS…

High Energy Physics - Phenomenology · Physics 2023-04-11 K. Deja , V. Martinez-Fernandez , B. Pire , P. Sznajder , J. Wagner

Relativistic Hartree-Fock and random phase approximation methods for open shells are used to calculate ionization potentials and static scalar polarizabilities of eight superheavy elements with open $6d$-shell, which include Db, Sg, Bh, Hs,…

Atomic Physics · Physics 2016-04-06 V. A. Dzuba

Two-photon excitation spectroscopy is a nonlinear technique that has gained rapidly in interest and significance for studying the complex energy-level structure and transition probabilities of materials. While the conventional spectroscopy…

Quantum Physics · Physics 2022-11-23 Yuanyuan Chen , Roberto de J. León-Montiel , Lixiang Chen

Propylene oxide, a favorite target of experimental and theoretical studies of circular dichroism, was recently discovered in interstellar space, further amplifying the attention to its role in the current debate on protobiological…

We demonstrate an efficient method to engineer the quantum confinement in a system of two quantum dots grown in a vertical stack. We achieve this by using materials with a different lattice constant for the growth of the outer and inner…

Mesoscale and Nanoscale Physics · Physics 2015-02-13 Ł. Kłopotowski , P. Wojnar , S. Kret , M. Parlińska-Wojtan , K. Fronc , G. Karczewski , T. Wojtowicz

An accessible tabletop source for the production of entangled x rays is crucial for the field of high-energy quantum optics. Here, we present a detailed analysis of the entanglement and polarization of the two photons emitted by an electron…

Quantum Physics · Physics 2024-11-01 T. D. C. de Vos , J. J. Postema , B. H. Schaap , A. Di Piazza , O. J. Luiten

Split-pulse x-ray photon correlation spectroscopy has been proposed as one of the unique capabilities made possible with the x-ray free electron lasers. It enables characterization of atomic scale structural dynamics that dictates the…

Instrumentation and Detectors · Physics 2020-05-06 Yanwen Sun , Mike Dunne , Paul Fuoss , Taito Osaka , Aymeric Robert , Mark Sutton , Makina Yabashi , Diling Zhu

The internal structure of doped holes in the Mott insulator may provide important insight into the physics of doped cuprates. Its observability via a single-particle probe by scanning tunneling spectroscopy (STS) and angle-resolved…

Strongly Correlated Electrons · Physics 2024-08-27 Jing-Yu Zhao , Zheng-Yu Weng

A model of the non-concentric spherical core-shell quantum dot under the influence of an externally applied electric field was proposed. It was established that the energy spectrum of both the electron and the hole depends on the intensity…

Mesoscale and Nanoscale Physics · Physics 2024-12-31 R. Ya. Leshko , I. V. Bilynskyi , O. V. Leshko , M. Yu. Popov , A. O. Ocheretyanyi

We studied a vertical ``quantum dot molecule'', where one of the dots is occupied with electrons and the other with holes. We find that different phases occur in the ground state, depending on the carrier density and the interdot distance.…

Mesoscale and Nanoscale Physics · Physics 2009-11-10 K. Karkkainen , M. Koskinen , M. Manninen , S. M. Reimann

Two-dimensional electronic spectroscopy (2DES) can be implemented with different geometries, e.g., BOXCARS, collinear and pump-probe geometries. The pump-probe geometry has its advantage of overlapping only two beams and reducing phase…

Quantum Physics · Physics 2024-03-04 Mao-Rui Cai , Xue Zhang , Zi-Qian Cheng , Teng-Fei Yan , Hui Dong

The analytical structure and absolute values of the generalized cross-section of the two-photon resonance single ionization of the K-shell of a heavy neon-like ion of an iron atom (Fe$^{16+}$) were theoretically predicted. A pronounced…

Excited states in single quantum dots (QDs) have been shown to be useful for spin state initialization and manipulation. For scalable quantum information processing it is necessary to have multiple spins interacting. Therefore, we present…

Excitons -- two-particle correlated electron-hole pairs -- are the dominant low-energy optical excitation in the broad class of semiconductor materials, which range from classical silicon to perovskites, and from two-dimensional to organic…

Materials Science · Physics 2025-11-25 Marcel Reutzel , G. S. Matthijs Jansen , Stefan Mathias

Molecules show a much increased multiple ionization rate in a strong laser field as compared to atoms of similar ionization energy. A widely accepted model attributes this to the action of the joint fields of the adjacent ionic core and the…

Atomic Physics · Physics 2013-05-16 J. Wu , M. Meckel , L. Ph. H. Schmidt , M. Kunitski , S. Voss , H. Sann , H. Kim , T. Jahnke , A. Czasch , R. Dörner