English
Related papers

Related papers: Block Copolymer at Nano-Patterned Surfaces

200 papers

Motivated by the idea that intrinsically disordered proteins (IDPs) condense into liquid-like droplets within cells, we carry out Monte Carlo simulations of a polymer lattice model to study the relationship between charge patterning and…

Soft Condensed Matter · Physics 2019-12-11 Nicholas A. S. Robichaud , Ivan Saika-Voivod , Stefan Wallin

The phase behavior of asymmetrically interacting ABC star triblock copolymer melts is investigated by the self-consistent field theory (SCFT). Motivated by the experimental systems, in this study, we focus on the systems in which the…

Soft Condensed Matter · Physics 2015-08-25 Kai Jiang , Juan Zhang , Qin Liang

We present a self-consistent field theory (SCFT) study of spherical micelle formation in a blend of poly(styrene-butadiene) diblocks and homopolystyrene. The micelle core radii, corona thicknesses and critical micelle concentrations are…

Soft Condensed Matter · Physics 2011-06-28 M. J. Greenall , D. M. A. Buzza , T. C. B. McLeish

We numerically investigate local defectiveness control of self-assembled diblock copolymer patterns through appropriate substrate design. We use a nonlocal Cahn-Hilliard (CH) equation for the phase separation dynamics of diblock copolymers.…

Soft Condensed Matter · Physics 2017-02-13 D. Jeong , Y. Choi , J. Kim

The polymer systems are discussed in the framework of the Landau-Ginzburg model. The model is derived from the mesoscopic Edwards hamiltonian via the conditional partition function. We discuss flexible, semiflexible and rigid polymers. The…

Condensed Matter · Physics 2007-05-23 Robert Holyst , T. A. Vilgis

We examine the symmetry-breaking effect of fixed constellations of particles on the surface-directed spinodal decomposition of binary blends in the presence of particles whose surfaces have a preferential affinity for one of the components.…

Chemical Physics · Physics 2020-06-16 Supriyo Ghosh , Arnab Mukherjee , Raymundo Arroyave , Jack F. Douglas

We study stress relaxation in a strongly segregated lamellar mesophase of diblock copolymers. We consider the extreme limit in which chains are highly stretched and with their junction points confined to narrow interfaces. A lamella can be…

Soft Condensed Matter · Physics 2009-09-25 Adolfo M. Nemirovsky , Thomas A. Witten

Cell dynamics simulation is used to investigate the phase behavior of block copolymer/homopolymer mixture subjected to a steady shear flow. Phase transitions occur from transverse to parallel and then to perpendicular lamellar structure…

Soft Condensed Matter · Physics 2015-06-29 Y. Guo , J. Zhang , B. Wang , H. Wu , M. Sun , J. Pan

A laser focussed onto a semiconductor film can create a disordered lamellae pattern of coexisting molten-solid regions. We present a continuum model based on the higher reflectivity of the molten regions. For large latent heat, this model…

Condensed Matter · Physics 2009-10-22 Chuck Yeung , Rashmi Desai

In this paper we review some recent results, obtained jointly with Stu Whittington, for a mathematical model describing a copolymer in an emulsion. The copolymer consists of hydrophobic and hydrophilic monomers, concatenated randomly with…

Probability · Mathematics 2007-06-14 F. den Hollander , N. Petrelis

The present paper is a continuation of \cite{dHP07b}. The object of interest is a two-dimensional model of a directed copolymer, consisting of a random concatenation of hydrophobic and hydrophilic monomers, immersed in an emulsion,…

Probability · Mathematics 2009-11-13 Frank den Hollander , Nicolas Petrelis

We use a semi-supervised, neural-network based machine learning technique, the confusion method, to investigate structural transitions in magnetic polymers, which we model as chains of magnetic colloidal nanoparticles characterized by…

Soft Condensed Matter · Physics 2025-06-27 Dilina Perera , Samuel McAllister , Joan Josep Cerdà , Thomas Vogel

We apply self consistent field theory to twist grain boundaries of block copolymer melts. The distribution of monomers throughout the grain boundary is obtained as well as the grain boundary free energy per unit area as a function of twist…

Soft Condensed Matter · Physics 2009-10-31 Daniel Duque , Michael Schick

Functional nanoparticles (NPs) have gained significant attention as a promising application in various fields, including sensor, smart coating, drug delivery, and more. Here, we propose a novel mechanism assisted by machine-learning…

Soft Condensed Matter · Physics 2024-08-06 Changhuang Huang , Kechun Bai , Yanyan Zhu , David Andelman , Xingkun Man

We model a melt of monodisperse side-chain liquid crystalline polymers as a melt of comb copolymers in which the side groups are rod-coil diblock copolymers. We consider both excluded volume and Maier-Saupe interactions. The first acts…

Soft Condensed Matter · Physics 2007-05-23 Marcela Hernandez , Harry Westfahl Junior

The phase behavior of a melt of monodisperse rod-coil diblocks is studied. We derive a Landau free energy functional for both a compositional and a nematic order parameter. The excluded volume interaction between the rod blocks is modeled…

Soft Condensed Matter · Physics 2009-11-07 Manuel Reenders , Gerrit ten Brinke

Introducing nanorods into a polymeric matrix can enhance the physical and mechanical properties of the resulting material. In this paper, we focus on understanding the dispersion and orientation patterns of nanorods in an unentangled…

Soft Condensed Matter · Physics 2023-04-05 Navid Afrasiabian , Venkat Balasubramanian , Colin Denniston

Solutions of semiflexible polymers confined by repulsive planar walls are studied by density functional theory and Molecular Dynamics simulations, to clarify the competition between the chain alignment favored by the wall and the depletion…

Soft Condensed Matter · Physics 2016-05-25 Sergei A. Egorov , Andrey Milchev , Peter Virnau , Kurt Binder

The self-assembly behaviour of a diblock copolymer-diblock copolymer mixture under an oscillating shear field is investigated via cell dynamics simulation. The results indicate that the macrophase separation of the composite system is…

Soft Condensed Matter · Physics 2024-07-02 Y. Guo , H. He , X. Fu

We study AB$_n$ miktoarm star block copolymers in the strong segregation limit, focussing on the role that the AB interface plays in determining the phase behavior. We develop an extension of the kinked-path approach which allows us to…

Soft Condensed Matter · Physics 2007-05-23 Gregory M. Grason , Randall D. Kamien