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Neutron diffraction and bulk measurements are used to determine the nature of the low-temperature ordered state in LiCu$_2$O$_2$, a $S=1/2$ spin-chain compound with competing interactions. The magnetic structure is found to be helimagnetic,…

Strongly Correlated Electrons · Physics 2007-05-23 T. Masuda , A. Zheludev , A. Bush , M. Markina , A. Vasiliev

A ferroelectric transition occurring simultaneously with helical spin order has been found in both the polycrystalline and single crystal samples of LiCuVO4. The system has Cu2+ spins (s=1/2) of the CuO2 chains formed of edge-sharing CuO4…

Strongly Correlated Electrons · Physics 2015-06-25 Yutaka Naito , Kenji Sato , Yukio Yasui , Yusuke Kobayashi , Yoshiaki Kobayashi , Masatoshi Sato

We report susceptibility, specific heat, and neutron diffraction measurements on NaCu$_2$O$_2$, a spin-1/2 chain compound isostructural to LiCu$_2$O$_2$, which has been extensively investigated. Below 13 K, we find a long-range ordered,…

Strongly Correlated Electrons · Physics 2013-05-29 L. Capogna , M. Mayr , P. Horsch , M. Raichle , R. K. Kremer , M. Sofin , A. Maljuk , M. Jansen , B. Keimer

Neutron diffraction and 7Li-NMR have been applied to determine the multiferroic system LiCu2O2, which has four chains (ribbon chains) of edge-sharing CuO4 square planes in a unit cell. We have confirmed that there are successive magnetic…

Materials Science · Physics 2015-05-13 Yoshiaki Kobayashi , Kenji Sato , Yukio Yasui , Taketo Moyoshi , Masatoshi Sato , Kazuhisa Kakurai

Raman scattering studies of the frustrated spin chain system LiCu$_{2}$O$_{2}$ are reported. Two transitions into a magnetically ordered phase (taken place at temperatures $\sim$ 9 K and $\sim$ 24 K) have been confirmed from the analysis of…

Strongly Correlated Electrons · Physics 2009-11-10 K. -Y. Choi , S. A. Zvyagin , G. Cao , P. Lemmens

LiCu$_3$O$_3$ is a novel 2D S=1/2 antiferromagnet with randomly depleted square lattice. The crystal structure contains two types of square planes with different Cu$^{2+}\rightarrow$ Li$^{+}$ substitution rates (20% and 40%). $^7$Li NMR and…

Strongly Correlated Electrons · Physics 2024-09-09 A. A. Bush , S. K. Gotovko , V. Yu. Ivanov , V. I. Kozlov , E. G. Nikolaev , L. E. Svistov

A spin model of quasi-one dimensional LiCu$_{2}$O$_{2}$ compound with ground state of ellipsoidal helical structure in which the helical axis is along the diagonal of CuO$_{4}$ squares has been adopted. By taking into account the interchain…

Materials Science · Physics 2015-06-18 Yan Qi , An Du

From experimental and theoretical analyses of magnetic and specific-heat properties, we present the complete magnetic phase diagram of the quasi-one-dimensional antiferromagnet Cu(N$_2$H$_5$)$_2$(SO$_4$)$_2$. On cooling and at zero magnetic…

Strongly Correlated Electrons · Physics 2016-11-23 A. Paduan-Filho , A. P. Vieira , J. G. A. Ramon , R. S. Freitas

We investigate the spin $S=1/2$ Heisenberg model on the body centered cubic lattice in the presence of ferromagnetic and antiferromagnetic nearest-neighbor $J_{1}$, second-neighbor $J_{2}$, and third-neighbor $J_{3}$ exchange interactions.…

We report a long-wavelength helimagnetic superstructure in bulk samples of the ferrimagnetic insulator Cu2OSeO3. The magnetic phase diagram associated with the helimagnetic modulation inferred from small angle neutron scattering and…

Strongly Correlated Electrons · Physics 2012-06-13 T. Adams , A. Chacon , M. Wagner , A. Bauer , G. Brandl , B. Pedersen , H. Berger , P. Lemmens , C. Pfleiderer

Cu$_2$OSeO$_3$ is an insulating skyrmion-host material with a magnetoelectric coupling giving rise to an electric polarization with a characteristic dependence on the magnetic field $\vec H$. We report magnetic force microscopy imaging of…

Multiferroicity in LiCu2O2 single crystals is studied using resonant soft x-ray magnetic scattering, hard x-ray diffraction, heat capacity, magnetic susceptibility, and electrical polarization. Two magnetic transitions are found at 24.6 K…

We have performed muon spin rotation/relaxation (muSR) measurements on single crystals of the chiral helimagnet Cr1/3NbS2 at zero to low magnetic field. The transition from the paramagnetic to helical magnetically ordered phase at zero…

Materials Science · Physics 2015-06-23 D. Braam , C. Gomez , S. Tezok , E. V. L. de Mello , L. Li , D. Mandrus , Hae-Young Kee , J. E. Sonier

We report on a heat capacity study of high quality single crystal samples of \lcvo\ -- a frustrated spin $S=1/2$ chain system -- in magnetic field amounting to 3/4 of the saturation field. At low fields up to about 7~T, a linear temperature…

Strongly Correlated Electrons · Physics 2015-01-15 L. A. Prozorova , S. S. Sosin , L. E. Svistov , N. Buettgen , J. B. Kemper , A. P. Reyes , S. Riggs , O. A. Petrenko , A. Prokofiev

We apply a recent quasiparticle model for the electronic properties of metallic helimagnets to calculate the transport properties of three-dimensional systems in the helically ordered phase. We focus on the ballistic regime tau^2 T…

Strongly Correlated Electrons · Physics 2009-11-13 T. R. Kirkpatrick , D. Belitz , Ronojoy Saha

The microscopic origin of the recently observed helical structure in LiCu2O2 [1] is considered. It is shown that the frustrated antiferromagnetic double chain scenario adopted in Ref.1 is unrealistic. It should be replaced by a frustrated…

Strongly Correlated Electrons · Physics 2009-11-10 S. -L. Drechsler , J. Malek , J. Richter , A. S. Moskvin , A. A. Gippius , H. Rosner

We present an investigation of magnetic ordering in the two-dimensional S=1/2 quantum magnet Cu(Pz)_2(ClO_4)_2 using specific heat and zero field muon-spin relaxation (\mu^+SR). The magnetic contribution to the specific heat is consistent…

We present the general theory of clean, two-dimensional, quantum Heisenberg antiferromagnets which are close to the zero-temperature quantum transition between ground states with and without long-range N\'{e}el order. For N\'{e}el-ordered…

Condensed Matter · Physics 2009-10-22 Andrey V. Chubukov , Subir Sachdev , Jinwu Ye

Our experimental (neutron diffraction, M\"ossbauer spectroscopy, magnetic susceptibility, specific heat) and numerical studies on the evolution of short- and long-range magnetic order in $\gamma_{\rm II}$-Li\(_2\)FeSiO\(_4\) suggest a…

Strongly Correlated Electrons · Physics 2025-01-20 W. Hergett , N. Bouldi , M. Jonak , C. Neef , C. Ritter , M. Abdel-Hafiez , F. Seewald , H. -H. Klauss , M. W. -Haverkort , R. Klingeler

Magnetic skyrmions are nano-sized topological spin textures stabilized by a delicate balance of magnetic energy terms. The chemical substitution of the underlying crystal structure of skyrmion-hosting materials offers a route to manipulate…

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