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Long-range ion induced water-water correlations were recently observed in femtosecond elastic second harmonic scattering experiments of electrolyte solutions. To further the qualitative understanding of these correlations, we derive an…

Statistical Mechanics · Physics 2017-09-06 David M. Wilkins , David E. Manolopoulos , Sylvie Roke , Michele Ceriotti

The dielectric constant of ionic solutions is known to reduce with increasing ionic concentrations. However, the origin of this effect has not been thoroughly explored. In this paper we study two such possible sources: long-range Coulombic…

Statistical Mechanics · Physics 2022-08-04 Ram M. Adar , Tomer Markovich , Amir Levy , Henri Orland , David Andelman

A Bose-Einstein condensate is the ground state of a dilute gas of bosons, such as atoms cooled to temperatures close to absolute zero. With much smaller mass, excitons (bound electron-hole pairs) are expected to condense at significantly…

Mesoscale and Nanoscale Physics · Physics 2021-03-31 Zefang Wang , Daniel A. Rhodes , Kenji Watanabe , Takashi Taniguchi , James C. Hone , Jie Shan , Kin Fai Mak

The conductance of a weakly interacting electron gas in the presense of a single scatterer is found at arbitrary strength of the scattering potential. At weak interaction, a simple renormalization group approach can be used instead of the…

Condensed Matter · Physics 2009-10-22 K. A. Matveev , Dongxiao Yue , L. I. Glazman

The osmotic coefficient of solutions of rod-like polyelectrolytes is considered by comparing current theoretical treatments and simulations to recent experimental data. The discussion is restricted to the case of monovalent counterions and…

Soft Condensed Matter · Physics 2009-11-07 M. Deserno , C. Holm , J. Blaul , M. Ballauff , M. Rehahn

We calculate ion distributions near a planar oil-water interface within non-linear Poisson-Boltzmann theory, taking into account the Born self-energy of the ions in the two media. For unequal self-energies of cations and anions, a…

Soft Condensed Matter · Physics 2013-06-06 Jos Zwanikken , Joost de Graaf , Markus Bier , René van Roij

The structure of cylindrical double layers is studied using a modified Poisson Boltzmann theory and the density functional approach. In the model double layer, the electrode is a cylindrical polyion that is infinitely long, impenetrable,…

Soft Condensed Matter · Physics 2013-12-18 V. Dorvilien , C. N. Patra , L. B. Bhuiyan , C. W. Outhwaite

Poisson-Boltzmann theory is the cornerstone for soft matter electrostatics. We provide novel exact analytical solutions to this non-linear mean-field approach, for the diffuse layer of ions in the vicinity of a planar or a cylindrical…

Soft Condensed Matter · Physics 2020-01-29 L. Samaj , E. Trizac

Inhomogeneity of ion correlation widely exists in many physicochemical, soft matter, and biological systems. Here, we apply the modified Gaussian renormalized fluctuation theory to study the classic example of the vapor-liquid interface of…

Soft Condensed Matter · Physics 2022-11-22 Nikhil R. Agrawal , Rui Wang

Why kinetically stable oil droplets in water spontaneously acquire a negative charge remains one of the most vigorously debated questions in interfacial science. Here, we combine neural-network based deep potential molecular dynamics with a…

We study theoretically a gas consisting of charged bosons (ions) over the flat dielectric surface at low temperatures and its tendency to form a state with a Bose-Einstein condensate. For the stability of a system, an additional external…

Quantum Gases · Physics 2021-09-22 I. V. Lukin , A. G. Sotnikov , Yu. V. Slyusarenko

Three analytic results are proposed for a linear form of the modified Poisson-Boltzmann equation in the theory of bulk electrolytes. Comparison is also made with the mean spherical approximation results. The linear theories predict a…

Statistical Mechanics · Physics 2019-06-28 C. W. Outhwaite , L. B. Bhuiyan

In this thesis, the electrostatic interaction between two chemically identical colloids, both carrying constant surface potential is studied in the limit of short inter-particle separation at the interface of two immiscible fluids. Using an…

Soft Condensed Matter · Physics 2020-01-01 Rick Bebon

Light scattering and viscometric measurements on weak polyelectrolytes show two important aspects of counterion condensation, namely, non-monotonic variation in the polyelectrolyte size with the increase in the electrostatic strength, and,…

Statistical Mechanics · Physics 2014-08-12 Prasanta Kundu , Arti Dua

The effective electrostatic interaction between a pair of colloids, both of them located close to each other at an electrolyte interface, is studied by employing the full, nonlinear Poisson-Boltzmann (PB) theory within classical density…

Soft Condensed Matter · Physics 2016-08-17 Arghya Majee , Markus Bier , S. Dietrich

We study a classical system of identically charged counter-ions near a planar wall carrying a uniform surface charge density. The equilibrium statistical mechanics of the system depends on a single dimensionless coupling parameter. A new…

Soft Condensed Matter · Physics 2019-01-21 I. Palaia , M. Trulsson , L. Samaj , E. Trizac

Attraction between two indentical objects uniformly charged in solution seems intuitively surprising on the one hand because we know that such objects do repel in vacuum and on another hand because this simple mental picture is still…

Soft Condensed Matter · Physics 2013-12-02 Fabien Paillusson

Within a dipolar Poisson-Boltzmann theory including electrostatic correlations, we consider the effect of explicit solvent structure on solvent and ion partition confined to charged nanopores. We develop a relaxation scheme for the solution…

Soft Condensed Matter · Physics 2015-10-28 Sahin Buyukdagli

We discuss Bose-Einstein condensation in a trapped gas of bosonic particles interacting dominantly via dipole-dipole forces. We find that in this case the mean-field interparticle interaction and, hence, the stability diagram are governed…

Condensed Matter · Physics 2009-10-31 L. Santos , G. V. Shlyapnikov , P. Zoller , M. Lewenstein

A modified Poisson-Nernst-Planck system in a bounded domain with mixed Dirichlet-Neumann boundary conditions is analyzed. It describes the concentrations of ions immersed in a polar solvent and the correlated electric potential due to the…

Analysis of PDEs · Mathematics 2023-05-25 Ansgar Jüngel , Annamaria Massimini