Related papers: Broadband Homonuclear Decoupling
We propose a scheme for sensing of an oscillating field in systems with large inhomogeneous broadening and driving field variation by applying sequences of phased, adiabatic, chirped pulses. The latter act as a double filter for dynamical…
Spins in semiconductor quantum dots constitute a promising platform for scalable quantum information processing. Coupling them strongly to the photonic modes of superconducting microwave resonators would enable fast non-demolition readout…
Nanoscale nuclear magnetic resonance (NMR) signals can be measured through hyperfine interaction to paramagnetic electron sensor spins. A heterodyne approach is widely used to overcome the electron spin lifetime limit in spectral…
Pulsed excitation of broad spectra requires very high field strengths if monochromatic pulses are used. If the corresponding high power is not available or not desirable, the pulses can be replaced by suitable low-power pulses that…
Scalar couplings between covalently bound nuclear spins are a ubiquitous feature in nuclear magnetic resonance (NMR) experiments, imparting valuable information to NMR spectra regarding molecular structure and conformation. Such couplings…
The use of spin echoes to refocus one spin interactions (chemical shifts) and two spin interactions (spin-spin couplings) plays a central role in both conventional NMR experiments and NMR quantum computation. Here we describe schemes for…
The NMR spectra of spin-1/2 pairs contains four peaks, with two inner peaks much stronger than the outer peaks in the near-equivalence regime. We have observed that the strong inner peaks have significantly different linewidths, when…
Nuclear magnetic resonance (NMR) is a powerful method for determining the structure of molecules and proteins. While conventional NMR requires averaging over large ensembles, recent progress with single-spin quantum sensors has created the…
We discuss two-photon correlations from the side peaks that are formed when a two-level system emitter is driven coherently, with a detuning between the driving source and the emitter (quasi-resonance fluorescence). We do so in the context…
We develop energy efficient, continuous microwave schemes to couple electron and nuclear spins, using phase or amplitude modulation to bridge their frequency difference. These controls have promising applications in biological systems,…
Nuclear magnetic resonance spectroscopy with solid-state spin sensors is a promising pathway for the detection of nuclear spins at the micro- and nanoscale. Although many nanoscale experiments rely on a single sensor spin for the detection…
Molecular spins offer promise in emerging quantum technologies such as quantum sensing and computing. At low temperatures, nuclear spin-spin interactions affect electron spin coherence lifetimes through pure dephasing. Nuclear-spin noise…
We analyze the suppression of decoherence by means of dynamical decoupling in the pure-dephasing spin-boson model for baths with power law spectra. The sequence of ideal $\pi$ pulses is optimized according to the power of the bath. We…
Using equivalencies between different models we reduce the model of two spin-1/2 Heisenberg chains crossed at one point to the model of free fermions. The spin-spin correlation function is calculated by summing the perturbation series in…
We use multi-pulse dynamical decoupling to increase the coherence lifetime (T2) of large numbers of nitrogen-vacancy (NV) electronic spins in room temperature diamond, thus enabling scalable applications of multi-spin quantum information…
We consider decoupling in the context of an effective quantum field theory of two scalar fields with well separated mass scales and a $Z_2\times Z_2$ symmetry. We first prove, using Wilson's exact renormalization group equation, that the…
Nuclear spins of noble gases can maintain coherence for hours at ambient conditions owing to their extraordinary isolation by the enclosing, complete electronic shells. This isolation, however, impedes the ability to manipulate and control…
We investigate full quantum mechanical evolution of two electrons nonlinearly coupled to quantum phonons and simulate the dynamical response of the system subject to a short spatially uniform optical pulse that couples to dipole-active…
We experimentally isolate, characterize and coherently control up to six individual nuclear spins that are weakly coupled to an electron spin in diamond. Our method employs multi-pulse sequences on the electron spin that resonantly amplify…
We demonstrate both theoretically and experimentally beam-dependent photonic spin-orbit coupling in a two-wave mixing process described by an equivalent of the Pauli equation in quantum mechanics. The considered structured light in the…