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We predict large regions of the charge stability diagram using a multi-band and multi-electron configuration interaction model of a double quantum dot system. We account for many-body interactions within each quantum dot using full…

Mesoscale and Nanoscale Physics · Physics 2024-11-27 Nathan L. Foulk , Sankar Das Sarma

The Coulomb interactions between electrons play important roles in coupling multiple qubits in various quantum systems. Here we demonstrate controlled quantum operations of three electron charge qubits based on three capacitively coupled…

Mesoscale and Nanoscale Physics · Physics 2018-02-21 Hai-Ou Li , Gang Cao , Guo-Dong Yu , Ming Xiao , Guang-Can Guo , Hong-Wen Jiang , Guo-Ping Guo

We investigate configuration-interaction (CI) calculations on a basis of molecular orbitals generated by preliminary density-functional theory (DFT) calculations. We use this CI/DFT framework to improve the modeling of core-excited states…

Chemical Physics · Physics 2025-09-11 Giorgio Visentin , Francois Mauger

We present the concept, derivation, and implementation of dynamical configuration interaction, a quantum embedding theory that combines Green's function methodology with the many-body wave function. In a strongly-correlated active space, we…

Chemical Physics · Physics 2019-04-03 Marc Dvorak , Patrick Rinke

Exchange-coupled singlet-triplet spin qubits in two gate-defined double quantum dots are considered theoretically. Using charge density operators to describe the double-dot orbital states, we calculate the Coulomb couplings between the…

Mesoscale and Nanoscale Physics · Physics 2015-05-28 Guy Ramon

We consider the nonstationary circuit QED architecture in which a single-mode cavity interacts with N>1 identical qubits, and some system parameters undergo a weak external perturbation. It is shown that in the dispersive regime one can…

Quantum Physics · Physics 2018-02-16 A. V. Dodonov

Two-electron states bound to donors in silicon are important for both two qubit gates and spin readout. We present a full configuration interaction technique in the atomistic tight-binding basis to capture multi-electron exchange and…

Recent experiments on semiconductor quantum dots have demonstrated the ability to utilize a large quantum dot to mediate superexchange interactions and generate entanglement between distant spins. This opens up a possible mechanism for…

Mesoscale and Nanoscale Physics · Physics 2020-07-29 Kuangyin Deng , Edwin Barnes

Accurate atomic structure calculations of complicated atoms with 4 or more valence electrons begin to push the memory and time limits of supercomputers. This paper presents a robust method of decreasing the size of \textit{ab initio}…

Atomic Physics · Physics 2018-10-24 A. J. Geddes , D. A. Czapski , E. V. Kahl , J. C. Berengut

We studied the dynamics of a pair of single-electron double quantum dots (DQD) under longitudinal and transverse static magnetic fields and time-dependent harmonic modulation of their interaction couplings. We propose to modulate the tunnel…

Mesoscale and Nanoscale Physics · Physics 2026-02-12 Alejandro D. Bendersky , Sergio S. Gomez , Rodolfo H. Romero

Numerous numerical studies have shown that geminal-based methods are a promising direction to model strongly correlated systems with low computational costs. Several strategies have been introduced to capture the missing dynamical…

Chemical Physics · Physics 2023-03-22 Artur Nowak , Katharina Boguslawski

We present a variational method to calculate the exchange interactions among donor clusters in a semiconductor. Such clusters are candidates for a so-called control-qubit architecture for quantum information, where the effective exchange…

Materials Science · Physics 2007-11-02 W. Wu , P. T. Greenland , A. J. Fisher

We study controllable exchange coupling between two singlet-triplet qubits. We start from the original second quantized Hamiltonian of a quadruple quantum dot system and obtain the effective spin-spin interaction between the two qubits…

Mesoscale and Nanoscale Physics · Physics 2013-05-13 Rui Li , Xuedong Hu , J. Q. You

Orbital modeling of two electron spins confined in a double quantum dot is revisited. We develop an extended Hund Mulliken approach that includes excited orbitals, allowing for a triplet configuration with both electrons residing in a…

Mesoscale and Nanoscale Physics · Physics 2018-01-31 Zack White , Guy Ramon

We present a new quantum embedding theory called dynamical configuration interaction (DCI) that combines wave function and Green's function theories. DCI captures static correlation in a correlated subspace with configuration interaction…

Chemical Physics · Physics 2019-11-21 Marc Dvorak , Dorothea Golze , Patrick Rinke

Doubly occupied configuration interaction (DOCI) with optimized orbitals often accurately describes strong correlations while working in a Hilbert space much smaller than that needed for full configuration interaction. However, the scaling…

Chemical Physics · Physics 2016-02-25 Thomas M. Henderson , Ireneusz W. Bulik , Tamar Stein , Gustavo E. Scuseria

Exchange interaction has been studied for electrons in coupled quantum dots (QD's) by a configuration interaction method using confinement potentials with different profiles. The confinement potential has been parametrized by a two-centre…

Mesoscale and Nanoscale Physics · Physics 2015-05-13 A. Kwasniowski , J. Adamowski

In double quantum dot singlet-triplet qubits, the exchange interaction is used in both quantum gate operation and the measurement of the state of the qubit. The exchange can be controlled electronically by applying gate voltage pulses. We…

Mesoscale and Nanoscale Physics · Physics 2013-10-21 Tuukka Hiltunen , Juha Ritala , Topi Siro , Ari harju

This paper presents a conceptual design for quantum heat machines using a pair of coupled double quantum dots (DQDs), each DQD with an excess electron to interact, as an working substance. We define a compression ratio as the ratio between…

Quantum Physics · Physics 2021-08-04 Jefferson Luan D. de Oliveira , Moises Rojas , Cleverson Filgueiras

Quantum dots (QDs) are semiconductor nanostructures in which a three dimensional potential trap produces an electronic quantum confinement, thus mimicking the behaviour of single atomic dipole-like transitions. However unlike atoms, QDs can…