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We show that interference phenomena plays a big role for the electron yield in ionization of atoms by an ultra-short laser pulse. Our theoretical study of single ionization of atoms driven by few-cycles pulses extends the photoelectron…

Quantum Physics · Physics 2009-11-13 Diego Arbo , Emil Persson , Joachim Burgdoerfer

In conditions where the interaction betweeen an atom and a short high-frequency extreme ultraviolet laser pulse is a perturbation, we show that a simple theoretical approach, based on Coulomb-Volkov-type states, can make reliable…

Atomic Physics · Physics 2009-11-07 Guillaume Duchateau , Eric Cormier , Robert Gayet

We report a fully differential study of ionization of the Ne L-shell by Compton scattering of 20 keV photons. We find two physical mechanisms which modify the Compton-electron emission. Firstly, we observe scattering of the Compton…

Attosecond photoionisation time delays reveal information about the potential energy landscape an outgoing electron wavepacket probes upon ionisation. In this study we experimentally quantify, for the first time, the dependence of the time…

Experimental cross sections for m-fold photodetachment (m=2-5) of oxygen anions via K-shell excitation and ionization were measured in the photon-energy range of 525-1500 eV using the photon-ion merged-beams technique at a synchrotron light…

We propose a novel mechanism of electron localization and molecular symmetry breaking in dissociative photoionization of the H$_2$ molecule. The Coulomb field of the ejected electron can induce transition of the remaining H$_2^+$ ion from…

Atomic Physics · Physics 2014-03-12 Vladislav V. Serov , A. S. Kheifets

We report the cooling of an atomic ensemble with light, where each atom scatters only a single photon on average. This is a general method that does not require a cycling transition and can be applied to atoms or molecules which are…

It is known that homogeneous distribution of particles in Coulomb-like systems can be unstable, and spatially inhomogeneous structures can be formed. A simple method for describing such inhomogeneous systems and obtaining spacial…

Statistical Mechanics · Physics 2015-06-16 B. I. Lev , V. P. Ostroukh , V. B. Tymchyshyn , A. G. Zagorodny

Polyatomic molecules in strong laser fields can undergo substantial nuclear motion within tens of femtoseconds. Ion imaging methods based on dissociation or Coulomb explosion therefore have difficulty faithfully recording the geometry…

We report on kinematically complete measurements and ab initio non-perturbative calculations of double ionization of He and H2 by a single 800 eV circularly polarized photon. We confirm the quasifree mechanism of photoionization for H2 and…

Superradiance is a hallmark of cooperative quantum emission, where radiative decay is collectively enhanced by coherence among emitters. Here, extending superradiant effects to photon pair generation from multi-level atoms, two-photon…

Quantum Physics · Physics 2026-01-21 Heewoo Kim , Bojeong Seo , Han Seb Moon

L-shell ionisation and subsequent Coulomb explosion of fully deuterated methyl iodide, CD$_3$I, irradiated with hard x-rays has been examined by a time-of-flight multi-ion coincidence technique. The core vacancies relax efficiently by Auger…

Atmospheric pressure helium plasmas are investigated through molecular dynamics simulations at room temperature (300 K) for various ionization fractions ($\chi_i = 10^{-1} - 10^{-5}$) in the strongly coupled regime (ion coupling parameter,…

Plasma Physics · Physics 2024-10-24 Swati Swagatika Mishra , Pascal Brault , Sudeep Bhattacharjee

In anticipation of upcoming two-photon double ionization of atoms and particularly Helium, under strong short wavelength radiation sources (45 eV), we present quantitative signatures of direct two-photon double ejection, in the…

Atomic Physics · Physics 2009-11-11 P. Lambropoulos , L. A. A. Nikolopoulos , M. G. Makris

A scanning tunneling microscope (STM) can do more than atomic imaging and manipulation. Its tunneling current can also be used for the excitation of light, converting electron energy to photon energy. STM based single-molecule…

Optics · Physics 2019-01-01 Yao Zhang , Yang Zhang , Zhenchao Dong

We demonstrate a left-right asymmetry control of the photo\-electron angular distribution in multi\-photon ionization of Li atoms by a bichromatic laser field. By delaying the fundamental (780 nm) and its second harmonic relative to each…

Atomic Physics · Physics 2024-05-20 Silva Mezinska , Alexander Dorn , Thomas Pfeifer , Klaus Bartschat

We describe the results of experiments and simulations performed with the aim of extending photoelectron spectroscopy with intense laser pulses to the case of molecular compounds. Dimer frame photoelectron angular distributions generated by…

Diffraction of atoms from surfaces provides detailed insights into structures, interactions, and dynamical processes. However, currently the method is limited to measurements in reflection - diffraction through materials has only been…

We show that the correlation dynamics in coherently excited doubly excited resonances of helium can be followed in real time by two-photon interferometry. This approach promises to map the evolution of the two-electron wave packet onto…

Quantum Physics · Physics 2013-05-24 J. Feist , S. Nagele , C. Ticknor , B. I. Schneider , L. A. Collins , J. Burgdörfer

The time-dependent Schr\"{o}dinger equation for the hydrogen atom and its interaction with coherent intense high-frequency short laser pulses is solved numerically exactly by propagating the single-electron wave packets. Thereby, the…

Atomic Physics · Physics 2013-09-11 Philipp V. Demekhin , David Hochstuhl , Lorenz S. Cederbaum