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Neutron scattering measurements on the pyrochlore magnet Ce$_2$Zr$_2$O$_7$ reveal an unusual crystal field splitting of its lowest $J$=5/2 multiplet, such that its ground state doublet is composed of m$_J$=$\pm$3/2, giving these doublets a…

In conventional quasi-one-dimensional antiferromagnets with quantum spins, magnetic excitations are carried by either magnons or spinons in different energy regimes: they do not coexist independently, nor could they interact with each…

Strongly Correlated Electrons · Physics 2020-07-30 H. Zhang , Z. Zhao , D. Gautreau , M. Raczkowski , A. Saha , V. O. Garlea , H. Cao , T. Hong , H. O. Jeschke , Subhendra D. Mahanti , T. Birol , F. F. Assaad , X. Ke

While the dominant magnetic interaction in La$_2$CuO$_4$ is superexchange between nearest-neighbor Cu moments, the pinning of the spin direction depends on weak anisotropic effects associated with spin-orbit coupling. The symmetry of the…

Strongly Correlated Electrons · Physics 2023-03-17 Xiao Hu , A. Sapkota , V. O. Galea , G. D. Gu , I. A. Zaliznyak , J. M. Tranquada

We performed susceptibility, magnetization, specific heat, and single crystal neutron diffraction measurements on single crystalline BaMn$_2$Si$_2$O$_7$. Based on the results, we revisited its spin structure with a more accurate solution…

Strongly Correlated Electrons · Physics 2019-07-31 G. H. Wang , C. Y. Xu , H. B. Cao , T. Hong , Q. Huang , Q. Y. Ren , J. Q. Xu , H. D. Zhou , W. D. Luo , D. Qian , J. Ma

The phenomenological theory of the flexomagnetoelectric coupling in crystals of the cubic, tetragonal and orthorhombic crystal systems has been suggested. Secondary role of the crystal structure chirality was shown. Oppositely, significant…

Materials Science · Physics 2015-05-30 B. M. Tanygin

The Ba3Cu3In4O12 stands for unique topology of the magnetic subsystem. It consists of rotated by 90\Box$^b$ relative to each other "paper-chain" columns made of vertex-sharing CuIO4 and CuIIO4 planar units. The overall pattern of the copper…

CuCrS2 is a triangular lattice Heisenberg antiferromagnet with a rhombohedral crystal structure. We report on neutron and synchrotron powder diffraction results which reveal a monoclinic lattice distortion at the magnetic transition and…

The mineral malachite, Cu2(OD)2CO3, has a quantum spin-liquid ground state and no long-range magnetic order down to at least T=0.4 K. Inelastic neutron scattering measurements show that the excitation spectrum consists of dispersive gapped…

Strongly Correlated Electrons · Physics 2015-03-05 E. Canevet , B. Fak , R. K. Kremer , J. H. Chun , M. Enderle , E. E. Gordon , J. L. Bettis , M. -H. Whangbo , J. W. Taylor , D. T. Adroja

Rare earth based cobalt-ruthenium double perovskites A$_2$CoRuO$_6$ (A = La, Pr, Nd and Sm) were synthesized and investigated for their structural and magnetic properties. All the compounds crystallize in the monoclinic $P2_1/n$ structure…

Materials Science · Physics 2019-07-24 Manjil Das , Prabir Dutta , Saurav Giri , Subham Majumdar

We report on the crystal structure of the quantum magnet (CuCl)LaNb2O7 that was controversially described with respect to its structural organization and magnetic behavior. Using high-resolution synchrotron powder x-ray diffraction,…

Materials Science · Physics 2015-03-17 Alexander A. Tsirlin , Artem M. Abakumov , Gustaaf Van Tendeloo , Helge Rosner

A three-dimensional system of interacting spins typically develops static long-range order when it is cooled. If the spins are quantum (S = 1/2), however, novel quantum paramagnetic states may appear. The most highly sought state among them…

Strongly Correlated Electrons · Physics 2015-05-13 S. -H. Lee , H. Kikuchi , Y. Qiu , B. Lake , Q. Huang , K. Habicht , K. Kiefer

We report the low temperature magnetic properties of Ce$_2$Sn$_2$O$_7$, a rare-earth pyrochlore. Our susceptibility and magnetization measurements show that due to the thermal isolation of a Kramers doublet ground state, Ce$_2$Sn$_2$O$_7$…

Strongly Correlated Electrons · Physics 2016-08-15 Romain Sibille , Elsa Lhotel , Vladimir Pomjakushin , Chris Baines , Tom Fennell , Michel Kenzelmann

The three-dimensional $S = {\frac{1}{2}}$ system Y$_{3}$Cu$_{2}$Sb$_{3}$O$_{14}$ consists of two inequivalent Cu$^{2+}$ sites, each forming an edge shared triangular lattice. Our magnetic susceptibility $\chi(T)$, specific heat $C_p(T)$,…

The unusual magnetic properties of a novel low-dimensional quantum ferrimagnet Cu$_2$Fe$_2$Ge$_4$O$_{13}$ are studied using bulk methods, neutron diffraction and inelastic neutron scattering. It is shown that this material can be described…

Strongly Correlated Electrons · Physics 2009-11-10 T. Masuda , A. Zheludev , B. Grenier , S. Imai , K. Uchinokura , E. Ressouche , S. Park

Spin liquids are highly correlated yet disordered states formed by the entanglement of magnetic dipoles$^1$. Theories typically define such states using gauge fields and deconfined quasiparticle excitations that emerge from a simple rule…

Low-dimensional quantum magnets are a versatile materials platform for studying the emergent many-body physics and collective excitations that can arise even in systems with only short-range interactions. Understanding their low-temperature…

The Stoner instability remains a cornerstone for understanding metallic ferromagnets. This instability captures the interplay of Coulomb repulsion, Pauli exclusion, and two-fold fermionic spin degeneracy. In materials with spin-orbit…

Strongly Correlated Electrons · Physics 2024-11-13 Yue Yu , Tatsuya Shishidou , Shuntaro Sumita , Michael Weinert , Daniel F. Agterberg

With octahedrally coordinated $t_{\rm 2g}$ orbitals which are active at filling $n=2$, the $\rm Sr_2CrO_4$ compound exhibits rich interplay of spin-orbital physics with tetragonal distortion induced crystal field tuning by external agent…

Strongly Correlated Electrons · Physics 2022-10-20 Shubhajyoti Mohapatra , Dheeraj Kumar Singh , Avinash Singh

Neutron scattering studies on powder and single crystals have provided new evidences for unconventional magnetism in Cu2Te2O5Cl2. The compound is built from tetrahedral clusters of S=1/2 Cu2+ spins located on a tetragonal lattice. Magnetic…

Strongly Correlated Electrons · Physics 2009-11-11 O. Zaharko , H. M. Ronnow , A. Daoud-Aladine , S. Streule , F. Juranyi , J. Mesot , H. Berger , P. J. Brown

Ba$_2$Cu$_3$O$_4$Cl$_2$ has two inter-penetrating square Cu sublattices, one with square root 2 times the in-plane spacing of the other. Isotropic magnetic interactions between the two sublattices are completely frustrated. Quantum…

Strongly Correlated Electrons · Physics 2009-11-11 M. K. Ramazanoglu , P. S. Clegg , S. Wakimoto , R. J. Birgeneau , S. Noro