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We report observation of two-photon emission from coherently excited vibrational state of solid parahydrogen, known as one of quantum solids. The coherent state between the ground and the excited states is prepared by stimulated Raman…

The reconstruction of attosecond beating by interference of two-photon transitions (RABBIT) is one of the most widely used techniques for obtaining both the relative phases of harmonics forming an attosecond pulse train and the phase of…

Optics · Physics 2023-09-13 R. E. F. Silva , Á. Jiménez-Galán

The coupling between single-photon emitters and phonons opens many possibilities to store and transmit quantum properties. In this paper we apply the independent boson model to describe the coupling between an optically driven two-level…

Mesoscale and Nanoscale Physics · Physics 2019-07-18 Thilo Hahn , Daniel Groll , Tilmann Kuhn , Daniel Wigger

A broadband squeezed vacuum photon field is characterized by a complex squeezing function. We show that by controlling the wavelength dependence of its phase it is possible to change the dynamics of the atomic polarization interacting with…

Quantum Physics · Physics 2008-03-11 Itay Rabinak , Eran Ginossar , Shimon Levit

The inclusion of atomic inversion in Raman scattering can significantly alter field dynamics in plasmonic settings. Our calculations show that large local fields and femtosecond pulses combine to yield: (i) population inversion within hot…

Optics · Physics 2015-06-15 M. Scalora , M. A. Vincenti , D. de Ceglia , M. Grande , J. W. Haus

An entangled photon experiment has been performed with a large variation of the temperature of the non-linear crystal generating the entangled pair by spontaneous downconversion. The photon pairs are separated by a nonpolarizing…

Quantum Physics · Physics 2019-09-04 Joakim Bergli , Guillaume Adenier , Andreas P. Thörn , Arnt Inge Vistnes

We consider the Raman process developing in a disordered medium of alkali-metal atoms when the scattered modes are trapped on a closed transition. Our theoretical analysis, based on numerical simulations of the Bethe-Salpeter equation for…

Atomic Physics · Physics 2014-07-22 L. V. Gerasimov , V. M. Ezhova , D. V. Kupriyanov , Q. Baudouin , W. Guerin , R. Kaiser

Vibrational motions in electronically excited states can be observed by either time and frequency resolved infrared absorption or by off resonant stimulated Raman techniques. Multipoint correlation function expressions are derived for both…

Quantum Physics · Physics 2017-09-13 Konstantin E. Dorfman , Benjamin P. Fingerhut , Shaul Mukamel

Within the framework of quantization of the macroscopic electromagnetic field, equations of motion and an effective Hamiltonian for treating both the resonant dipole-dipole interaction between two-level atoms and the resonant atom-field…

Quantum Physics · Physics 2016-08-16 Ho Trung Dung , Ludwig Knöll , Dirk-Gunnar Welsch

Stimulated Raman interaction of a classically pumped single three-level $\Lambda$-type atom in a resonator cavity featuring both radiative and unwanted losses is studied. It is shown that in the regime of stimulated adiabatic Raman passage…

Quantum Physics · Physics 2016-09-08 Mikayel Khanbekyan , Dirk-Gunnar Welsch

The electronic states at the direct band gap of monolayer WSe2 at the $K^+$ and $K^-$ valleys are related by time reversal and may be viewed as pseudo-spins. The corresponding optical interband transitions are governed by robust excitons.…

Materials Science · Physics 2015-09-16 G. Wang , M. M. Glazov , C. Robert , T. Amand , X. Marie , B. Urbaszek

It has been observed experimentally [H.R. Xia, C.Y. Ye, and S.Y. Zhu, Phys. Rev. Lett. {\bf 77}, 1032 (1996)] that quantum interference between two molecular transitions can lead to a suppression or enhancement of spontaneous emission. This…

Quantum Physics · Physics 2009-10-31 Jin Wang , H. M. Wiseman , Z. Ficek

Superradiance in an ensemble of atoms leads to the collective enhancement of radiation in a particular mode shared by the atoms in their spontaneous decay from an excited state. The quantum aspects of this phenomenon are highlighted when…

Giant atoms are known for the frequency-dependent spontaneous emission and associated interference effects. In this paper, we study the spontaneous emission dynamics of a two-level giant atom with dynamically modulated transition frequency.…

Quantum Physics · Physics 2022-11-28 Lei Du , Yan Zhang , Yong Li

In contrary to the widely reported single and symmetric peak feature of G' (or 2D) band in Raman spectrum of graphene, we herein report the observation of splitting in G' band in free standing graphene. Our experimental findings provide a…

Materials Science · Physics 2015-06-04 Zhiqiang Luo , Chunxiao Cong , Jun Zhang , Qihua Xiong , Ting Yu

The atom-photon entanglement of dressed atom and its spontaneous emission in a Double-Lambda closed-loop atomic system is studied in multi-photon resonance condition. It is shown that, even in the absence of quantum interference due to the…

Atomic and Molecular Clusters · Physics 2015-02-03 Zeinab Kordi , Saeed Ghanbari , Mohammad Mahmoudi

We study the second-order Raman process of mono- and few-layer MoTe$_2$, by combining {\em ab initio} density functional perturbation calculations with experimental Raman spectroscopy using 532, 633 and 785 nm excitation lasers. The…

The visibility of two-photon interference is limited by the indistinguishability of the photons. In the cascaded emission of a three-level system, such as a single quantum dot, the indistinguishability of each photon in the pair is…

We provide a theoretical framework to study the effect of dephasing on the quantum indistinguishability of single photons emitted from a coherently driven cavity QED $\Lambda$-system. We show that with a large excited-state detuning, the…

Quantum Physics · Physics 2015-05-13 Charles Santori , David Fattal , Kai-Mei C. Fu , Paul E. Barclay , Raymond G. Beausoleil

We study phonon-induced relaxation of quantum states of a particle (e.g., electron or proton) in a rigid double-well potential in a solid. Relaxation rate due to Raman two-phonon processes have been computed. We show that in a two-state…

Statistical Mechanics · Physics 2008-05-05 Jaroslav Albert , E. M. Chudnovsky , D. A. Garanin