English
Related papers

Related papers: Non-mean-field theory of anomalously large double-…

200 papers

A nonlinear phase-field model is developed to simulate corrosion damage. The motion of the electrode$-$ electrolyte interface follows the usual kinetic rate theory for chemical reactions based on the Butler-Volmer equation. The model links…

Chemical Physics · Physics 2024-08-28 M. Makuch , S. Kovacevic , M. R. Wenman , E. Martínez-Pañeda

Electrochemical devices often consist of multicomponent electrolyte solutions. Two processes influence the overall dynamics of these devices: the formation of electrical double layers and chemical conversion due to redox reactions. However,…

Chemical Physics · Physics 2022-06-20 Nathan Jarvey , Filipe Henrique , Ankur Gupta

The nonlinear capacitors are important devices in modern technologies and applied physics. The aim of this paper is to calculate exactly the capacitance and the electrostatic potential energy of a nonlinear parallel-plate capacitor by using…

Classical Physics · Physics 2017-04-12 Seyed Kamran Moayedi , Farkhondeh Fathi

The primitive model of ionic systems is investigated within a field-theoretic description for the whole range of size-, \lambda, and charge, Z, ratios of the two ionic species. Two order parameters (OP) are identified, and their relations…

Statistical Mechanics · Physics 2009-11-11 A. Ciach , W. T. Gozdz , G. Stell

We investigate generalized potentials for a mean-field density functional theory of a three-phase contact line. Compared to the symmetrical potential introduced in our previous article [1], the three minima of these potentials form a small…

Statistical Mechanics · Physics 2013-02-12 Chang-You Lin , Michael Widom , Robert F. Sekerka

Colossal Ion Conductivity (CIC) is the phenomenon in which large changes in oxygen conductivity are observed when a solid state oxygen electrolyte is placed in a heterolayer super lattice. Several hypotheses have been posed concerning both…

Materials Science · Physics 2019-01-04 M. F. Francis

We theoretically studied electric double layer by using the mean-field approach including the non-uniform size effect and the orientational ordering of water dipoles in electrolyte solution. Performing the minimization of the free energy,…

Soft Condensed Matter · Physics 2022-02-15 Jun-Sik Sin , Kwang-Il Kim , Chung-Sik Sin

In this work, we analyze the creation of the discharge asymmetry and the concomitant formation of the DC self-bias voltage in capacitively coupled radio frequency plasmas driven by multi-frequency waveforms, as a function of the electrode…

Plasma Physics · Physics 2024-06-19 R. U. Masheyeva , K. N. Dzhumagulova , M. Myrzaly , J. Schulze , Z. Donko

The electric double layer (EDL) governs electrocatalysis, energy conversion, and storage, yet its atomic structure, capacitance, and reactivity remain elusive. Here we introduce a machine learning interatomic potential framework that…

Chemical Physics · Physics 2025-09-18 Xiaoyu Wang , Junmin Chen , Zezhu Zeng , Frederick Stein , Junho Lim , Bingqing Cheng

Numerous measurements of the dielectric constant $\epsilon$ of the recently discovered ferroelectric nematic ($N_F$) liquid crystal (LC) phase report extraordinarily large values of $\epsilon^\prime$ (up to ~30,000). We show that what is in…

Soft Condensed Matter · Physics 2024-02-26 Noel A. Clark , Xi Chen , Joseph E. Maclennan , Matthew A. Glaser

We have realized a hybrid solid-state quantum device in which a single-electron semiconductor double quantum dot is dipole coupled to a superconducting microwave frequency transmission line resonator. The dipolar interaction between the two…

The recently developed modified Donnan (mD) model provides a simple and useful description of the electrical double layer in microporous carbon electrodes, suitable for incorporation in porous electrode theory. By postulating an attractive…

Chemical Physics · Physics 2014-01-22 P. M. Biesheuvel , S. Porada , M. Levi , M. Z. Bazant

Supercapacitors store energy via the formation of an electric double layer, which generates a strong electric field at the electrode-electrolyte interface. Unlike conventional metallic electrodes, graphene-derived materials suffer from a…

Materials Science · Physics 2015-03-12 Maxwell D. Radin , Tadashi Ogitsu , Minoru Otani , Juergen Biener , Brandon C. Wood

We develop an inhomogeneous mean-field theory for the extended Bose-Hubbard model with a quadratic, confining potential. In the absence of this potential, our mean-field theory yields the phase diagram of the homogeneous extended…

Quantum Gases · Physics 2012-02-01 Jamshid Moradi Kurdestany , Ramesh V. Pai , Rahul Pandit

We model cyclic voltammetry experiments on supported lipid films where a non-trivial dependence of the capacitance on the applied voltage is observed. Previously, based on a mean-field treatment of the Flory-Huggins type, under the…

Soft Condensed Matter · Physics 2010-07-28 Andrey V. Brukhno , Anna Akinshina , Zachary Coldrick , Andrew Nelson , Stefan Auer

With an implicit Particle-in-cell/Monte Carlo model, capacitively coupled plasmas are studied in two-dimensional and axisymmetric geometry. Self-bias dc voltage effects are self-consistently considered. Due to finite length effects, the…

Plasma Physics · Physics 2011-04-22 Wei Jiang , Hong-yu Wang , Zhen-hua Bi , You-nian Wang

A mean-field theory based on Gibbs-Bogoliubov inequality is constructed to study the interactions between two like-charged polyions. It is shown that contrary to the previously established paradigm, a properly constructed mean-field theory…

Soft Condensed Matter · Physics 2009-10-31 Jeferson J. Arenzon , Yan Levin , Juergen F. Stilck

Recent experimental and theoretical (both improved semiclassical and fully quantum-mechanical) results for B III and Ne VII delta n = 0 transitions with n = 2 or 3, respectively, are discussed. The probable reasons for disagreements by…

Atomic Physics · Physics 2009-10-31 Hans R. Griem , Yuri V. Ralchenko

Two-dimensional mixtures of dipolar colloidal particles with different dipole moments exhibit extremely rich self-assembly behaviour and are relevant to a wide range of experimental systems, including charged and super-paramagnetic colloids…

Soft Condensed Matter · Physics 2019-04-16 W. R. C. Somerville , J. L. Stokes , A. M. Adawi , T. S. Horozov , A. J. Archer , D. M. A. Buzza

We consider the effect of mobile ions on the applied potential needed to reorient a lamellar system of two different materials placed between two planar electrodes. The reorientation occurs from a configuration parallel to the electrodes…

Soft Condensed Matter · Physics 2012-07-19 Gregory Garbès Putzel , David Andelman , Yoav Tsori , Michael Schick