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Related papers: Alignment-Dependent Ionization of N$_2$, O$_2$, an…

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The alignment dependence of the ionization behavior of H$_2$ exposed to intense ultrashort laser pulses is investigated on the basis of solutions of the full time-dependent Schr\"odinger equation within the fixed-nuclei and dipole…

Quantum Physics · Physics 2013-05-29 Yulian V. Vanne , Alejandro Saenz

The alignment- and internuclear-distance dependent ionization of H$_2$ exposed to intense, ultrashort laser fields is studied by solving the time-dependent two-electron Schr\"odinger equation. In the regime of perturbative few-photon…

Atomic Physics · Physics 2015-06-23 Johann Förster , Yulian V. Vanne , Alejandro Saenz

We present three dimensional time-dependent calculations of ionization of arbitrarily spatially oriented H$_2^+$ by attosecond, intense, high-frequency laser fields. The ionization probability shows a strong dependence on both the…

Atomic Physics · Physics 2007-05-23 S. Selsto , M. Forre , J. P. Hansen , L. B. Madsen

The ionization of H2 in intense laser pulses is studied by numerical integration of the time-dependent Schr\"odinger equation for a single-active-electron model including the vibrational motion. The electron kinetic-energy spectra in…

Atomic Physics · Physics 2009-11-13 Stefan Pieper , Manfred Lein

We present a novel approach to calculating strong field ionization dynamics of multielectron molecular targets. Adopting a multielectron wavefunction ansatz based on field-free ab initio neutral and ionic multielectron states, a set of…

Atomic Physics · Physics 2015-05-14 Michael Spanner , Serguei Patchkovskii

Ionization and excitation of water molecules in intense laser pulses is studied theoretically by solving the three-dimensional time-dependent electronic Schr\"odinger equation within the single-active-electron approximation. The possibility…

Atomic Physics · Physics 2011-12-13 Simon Petretti , Alejandro Saenz , Alberto Castro , Piero Decleva

We develop a time-dependent theory to investigate electron dynamics and photoionization processes of diatomic molecules interacting with strong laser fields including electron-electron correlation effects. We combine the recently formulated…

Chemical Physics · Physics 2016-02-02 Henrik R. Larsson , Sebastian Bauch , Lasse Kragh Sørensen , Michael Bonitz

We study ionization dynamics of aligned diatomic molecules N$_2$ in strong elliptical laser fields experimentally and theoretically. The alignment dependence of photoelectron momentum distributions (PMDs) of N$_2$ measured in experiments is…

A theoretical framework for studying strong-field ionization of aligned molecules is presented, and alignment-dependent ionization yields are computed for CO2. Our calculations are in unprecedented agreement with recent experiments. We find…

Atomic Physics · Physics 2009-06-17 M. Abu-samha , L. B. Madsen

Ionization, excitation, and de-excitation to the ground state is studied theoretically for the first excited singlet state B $^1\Sigma_u^+$ of H$_2$ exposed to intense laser fields with photon energies in between about 3 eV and 13 eV. A…

Atomic Physics · Physics 2015-05-18 Manohar Awasthi , Alejandro Saenz

We present an exact single-electron picture that describes the correlated electron dynamics in strong laser fields. Our approach is based on the factorization of the electronic wavefunction as a product of a marginal and a conditional…

Chemical Physics · Physics 2017-04-26 Axel Schild , E. K. U. Gross

Modern laser systems are able to generate short and intense laser pulses ionizing matter in the poorly explored barrier-suppression regime. Field ionization in this regime is studied analytically and numerically. For analytical studies,…

Atomic Physics · Physics 2018-11-15 I. Yu. Kostyukov , A. A. Golovanov

A simple, analytical, nonrelativistic ionization rate formula for atoms and positive ions in intense ultraviolet and x-ray electromagnetic fields is derived. The rate is valid at arbitrary values of the Keldysh parameter and confirmed by…

Atomic Physics · Physics 2009-11-13 S. V. Popruzhenko , V. D. Mur , V. S. Popov , D. Bauer

The multiphoton ionization rate of molecules depends on the alignment of the molecular axis with respect to the ionizing laser polarization. By studying molecular frame photo-electron angular distributions from N$_2$, O$_2$ and benzene, we…

Chemical Physics · Physics 2015-06-15 C T L Smeenk , L Arissian , A V Sokolov , M Spanner , K F Lee , A Staudte , D M Villeneuve , P B Corkum

We investigate the photoelectron angular emission distributions obtained by strong field dissociative ionization of H$_2$ using cold target recoil ion momentum spectroscopy. In case of employing laser light with an ellipticity close to 0.9…

We study ab initio computations of the interaction of Lithium with a strong laser field. Numerical solutions of the time-dependent fully-correlated three-particle Schroedinger equation restricted to the one-dimensional soft-core…

Atomic Physics · Physics 2009-11-10 Camilo Ruiz , Luis Plaja , Luis Roso

In this paper we study the response in time of N$_2$, O$_2$ and F$_2$ to laser pulses having a wavelength of 390nm. We find single ionization suppression in O$_2$ and its absence in F$_2$, in accordance with experimental results at $\lambda…

Quantum Physics · Physics 2009-11-10 Daniel Dundas , Jan M. Rost

The fixed-nuclei full dimensional time-dependent Schr \"odinger equation is directly solved for H$_2^+$ in the linearly polarized laser field of $I \sim 1.0 \times 10^{14}$W cm$^{-2}$ and $\lambda \sim 1064 $nm Instantaneous ionization rate…

Atomic Physics · Physics 2007-05-23 Mohsen Vafaee , Hassan Sabzyan , Zahra Vafaee , Ali Katanforoush

We show that dynamic exchange is a dominant effect in strong field ionization of molecules. In $CO_2$ it fixes the peak ionization yield at the experimentally observed angle of $45^\circ$ between polarization direction and the molecular…

Atomic Physics · Physics 2015-09-09 Vinay Pramod Majety , Armin Scrinzi

Study on ionization process of molecules in an intense infrared laser field is of paramount interest in strong-field physics and constitutes the foundation of imaging of molecular valence orbitals and attosecond science. We show measurement…

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