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Recent work showed that the exact exchange-correlation potential of time-dependent density functional theory generically displays dynamical step structures. These have a spatially non-local and time-non-local dependence on the density in…

Chemical Physics · Physics 2013-12-09 K. Luo , P. Elliott , N. T. Maitra

We consider nonequilibrium transport in a simple chain of identical mechanical cells in which particles move around. In each cell, there is a rotating disc, with which these particles interact, and this is the only interaction in the model.…

Statistical Mechanics · Physics 2008-07-15 Jean-Pierre Eckmann , Carlos Mejia-Monasterio , Emmanuel Zabey

As a new approach to efficiently describe correlation effects in the relativistic quantum world we propose to consider reduced density matrix functional theory, where the key quantity is the first-order reduced density matrix (1-RDM). In…

Chemical Physics · Physics 2022-05-05 M. Rodríguez-Mayorga , K. J. H. Giesbertz , L. Visscher

We consider the energy averaged two-point correlator of spectral determinants and calculate contributions beyond the diagonal approximation using semiclassical methods. Evaluating the contributions originating from pseudo-orbit correlations…

Chaotic Dynamics · Physics 2015-05-13 Daniel Waltner , Stefan Heusler , Juan Diego Urbina , Klaus Richter

The correlation part of the pair density is separated into two components, one of them being predominant at short electronic ranges and the other at long ranges. The analysis of the intracular part of these components permits to classify…

Chemical Physics · Physics 2019-07-10 Mireia Via-Nadal , Mauricio Rodríguez-Mayorga , Eloy Ramos-Cordoba , Eduard Matito

We extend a previous analysis of spatial correlation functions for classical electromagnetic vector fields near a perfectly conducting boundary [PRE, vol. 73, 036604 (2006)] to the case of an isotropic semi-infinite medium with planar…

Optics · Physics 2009-11-13 Luk R. Arnaut

We present an in-depth study of the universal correlations of scattering-matrix entries required in the framework of non-stationary many-body scattering where the incoming states are localized wavepackets. Contrary to the stationary case…

Statistical Mechanics · Physics 2021-05-19 Andreas Bereczuk , Barbara Dietz , Jiongning Che , Jack Kuipers , Juan-Diego Urbina , Klaus Richter

The density-density correlations of the non-interacting finite temperature electron gas are discussed in detail. Starting from the ideal linear density response function and utilizing general relations from linear response theory, known and…

Plasma Physics · Physics 2025-09-24 Panagiotis Tolias , Tobias Dornheim , Jan Vorberger

The design of better exchange-correlation functionals for Density Functional Theory (DFT) is a central challenge of modern electronic structure theory. However, current developments are limited by the mathematical form of the functional,…

Chemical Physics · Physics 2024-08-19 Kyle Bystrom , Boris Kozinsky

We introduce a new functional for simulating ground-state and time-dependent electronic systems within density-functional theory. The functional combines an expression for the exact Kohn-Sham (KS) potential in the limit of complete electron…

Mesoscale and Nanoscale Physics · Physics 2021-01-15 M. J. P. Hodgson , J. D. Ramsden , T. R. Durrant , R. W. Godby

Density Functional Theory has long struggled to obtain the exact exchange-correlational (XC) functional. Numerous approximations have been designed with the hope of achieving chemical accuracy. However, designing a functional involves…

Chemical Physics · Physics 2025-03-10 Aditi Singh , Eduardo Fabiano , Szymon Śmiga

In the human brain, internal states are often correlated over time (due to local recurrence and other intrinsic circuit properties), punctuated by abrupt transitions. At first glance, temporal smoothness of internal states presents a…

Machine Learning · Computer Science 2023-05-24 Shima Rahimi Moghaddam , Fanjun Bu , Christopher J. Honey

In principle, machine learning (ML) can be used to obtain any electronic property of a many-body system from its electron density within density functional theory. However, some physical quantities are highly sensitive to small variations…

Materials Science · Physics 2026-02-19 L. Arnstein , J. Wetherell , R. Lawrence , P. J. Hasnip , M. J. P. Hodgson

The force-balance equation of time-dependent density-functional theory presents a promising route towards obtaining approximate functionals, however, so far, no practical correlation functionals have been derived this way. In this work,…

Chemical Physics · Physics 2025-04-08 Nicolas Tancogne-Dejean , Markus Penz , Michael Ruggenthaler , Angel Rubio

Causal decomposition depicts a cause-effect relationship that is not based on the concept of prediction, but based on the phase dependence of time series. It has been validated in both stochastic and deterministic systems and is now…

Signal Processing · Electrical Eng. & Systems 2020-08-18 Yi Zhang , Qin Yang , Lifu Zhang , Branko Celler , Steven Su , Peng Xu , Dezhong Yao

The primitive model describes ions by point charges with an additional hard-core interaction. In classical density-functional theory the mean-field electrostatic contribution can be obtained from the first order of a functional perturbation…

Soft Condensed Matter · Physics 2022-04-06 Moritz Bültmann , Andreas Härtel

Parametric correlations are studied in several classes of covariant density functional theories (CDFTs) using a statistical analysis in a large parameter hyperspace. In the present manuscript, we investigate such correlations for two…

Nuclear Theory · Physics 2020-03-17 A. Taninah , S. E. Agbemava , A. V. Afanasjev , P. Ring

We propose a method that incorporates explicit derivative discontinuity of the total energy with respect to the number of electrons and treats both delocalization and static correlation effects in density functional calculations. Our…

Strongly Correlated Electrons · Physics 2018-03-08 Fei Zhou , Vidvuds Ozolins

The exact universal functional of integer charge leads to an extension to fractional charge asymptotically when it is applied to a system made of asymptotically separated densities. The extended functional is asymptotically local and is…

Chemical Physics · Physics 2024-12-17 Jing Kong

The standard semiclassical calculation of transmission correlation functions for chaotic systems is severely influenced by unitarity problems. We show that unitarity alone imposes a set of relationships between cross sections correlation…

Chaotic Dynamics · Physics 2009-11-07 Raul O. Vallejos , Caio H. Lewenkopf