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We present data on the magnetic and magneto-elastic coupling in the hexagonal multiferroic manganite LuMnO3 from inelastic neutron scattering, magnetization and thermal expansion measurements. We measured the magnon dispersion along the…

Strongly Correlated Electrons · Physics 2010-12-01 H. J. Lewtas , A. T. Boothroyd , M. Rotter , D. Prabhakaran , H. Mueller , M. D. Le , B. Roessli , J. Gavilano , P. Bourges

A phase transition is often accompanied by the appearance of an order parameter and symmetry breaking. Certain magnetic materials exhibit exotic hidden-order phases, in which the order parameters are not directly accessible to conventional…

Strongly Correlated Electrons · Physics 2019-10-10 Yao Shen , Changle Liu , Yayuan Qin , Shoudong Shen , Yao-Dong Li , Robert Bewley , Astrid Schneidewind , Gang Chen , Jun Zhao

With a combined ab initio density functional and model Hamiltonian approach we establish that in the recently discovered multiferroic phase of the manganite Sr$_{1/2}$Ba$_{1/2}$MnO$_{3}$ the polar distortion of Mn and O ions is stabilized…

Materials Science · Physics 2015-03-09 Gianluca Giovannetti , Sanjeev Kumar , Carmine Ortix , Massimo Capone , Jeroen van den Brink

Hexagonal HoMnO$_{3}$ is a frustrated antiferromagnet (T$_{N}$=72 K) ferroelectric (T$_{C}$=875 K) in which these two order parameters are coupled. Our neutron measurements of the spin wave dispersion for the S=2 Mn$^{3+}$ on the layered…

Strongly Correlated Electrons · Physics 2009-11-11 O. P. Vajk , M. Kenzelmann , J. W. Lynn , S. B. Kim , S. -W. Cheong

Two magnetic ordering transitions are found in InMnO3, the paramagnetic to antiferromagnetic transition near ~118 K and a lower possible spin rotation transition near ~42 K. Multiple length scale structural measurements reveal enhanced…

Materials Science · Physics 2015-06-22 T. Yu , T. A. Tyson , P. Gao , T. Wu , X. Hong , S. Ghose , Y. -S. Chen

The floating-zone method with different growth ambiances has been used to selectively obtain hexagonal or orthorhombic DyMnO$_{3}$ single crystals. The crystals were characterized by X-ray powder diffraction of ground specimen and a…

Strongly Correlated Electrons · Physics 2009-11-13 S Harikrishnan , S Roessler , C M Naveen Kumar , H L Bhat , U K Roessler , S Wirth , F Steglich , Suja Elizabeth

Magnetic structure evolution of multiferroic hexagonal $YMn_{1-x}Fe_{x}O_{3}$ (${x} = 0, 0.05,$ and $0.1$) has been studied by carrying out detailed temperature-dependent neutron diffraction at zero- and 5T-fields. Thermodynamic data…

Materials Science · Physics 2017-07-26 Sonu Namdeo , S. S. S. Rao , S. D. Kaushik , V. Siruguri , A. M. Awasthi

The magnetic phase diagrams of RMnO3 (R = Er, Yb, Tm, Ho) are investigated up to 14 Tesla via magnetic and dielectric measurements. The stability range of the AFM order below the Neel temperature of the studied RMnO3 extends to far higher…

Strongly Correlated Electrons · Physics 2016-06-29 F. Yen , C. dela Cruz , B. Lorenz , E. Galstyan , Y. Y. Sun , M. Gospodinov , C. W. Chu

We use a combination of symmetry analysis, phenomenological modelling and first-principles density functional theory to explore the interplay between the magnetic ground state and the detailed atomic structure in the hexagonal rare-earth…

Materials Science · Physics 2022-02-07 Tara N. Tošić , Quintin N. Meier , Nicola A. Spaldin

We used Raman and terahertz spectroscopies to investigate lattice and magnetic excitations and their cross-coupling in the hexagonal YMnO3 multiferroic. Two phonon modes are strongly affected by the magnetic order. Magnon excitations have…

Disorder in magnetic systems typically suppresses long-range order, promoting short-range states such as spin glasses and magnetic clusters. This is particularly prominent in high-entropy materials, characterized by the random distributions…

This work is devoted to the analysis of orbital patterns and related to them interatomic magnetic interactions in centrosymmetric monoclinic structures of BiMnO$_3$, which have been recently determined experimentally. First, we set up an…

Materials Science · Physics 2008-07-11 I. V. Solovyev , Z. V. Pchelkina

A series of manganites Tb1-xHoxMnO3 (0<=x<=0.6) with orthorhombic structure are synthesized and detailed investigations on their multiferroicity are performed. Successive magnetic transitions upon temperature variation are evidenced for all…

Strongly Correlated Electrons · Physics 2010-04-19 C. L. Lu , S. Dong , K. F. Wang , J. -M. Liu

Structural, magnetic and multiferroic properties of single crystals of Dy$_{1-x}$Ho$_x$MnO$_3$ ($x = 0, 0.2$) were investigated by the different methods of polarized and classical neutron diffraction and macroscopic methods in order to…

We have used in-field neutron and X-ray single crystal diffraction to measure the incommensurability &#948; of the crystal and magnetic structure of multiferroic TbMnO3 . We show that the flop in the electric polarization at the critical…

Strongly Correlated Electrons · Physics 2009-11-11 N. Aliouane , D. N. Argyriou , J. Strempfer , I. Zegkinoglou , S. Landsgesell , M. v. Zimmermann

Bi3Mn4O12(NO3), in which the Mn4+ ions carry S=3/2, is the first honeycomb lattice system that shows no long-range magnetic order. Using neutron scattering, we have determined that short-range antiferromagnetic correlations develop at low…

Strongly Correlated Electrons · Physics 2010-12-06 M. Matsuda , M. Azuma , M. Tokunaga , Y. Shimakawa , N. Kumada

We have studied the influence of antiferromagnetic ordering on the local dielectric moments of the MnO_5 and LuO_7 polyhedra by measuring neutron powder diffraction patterns of LuMnO_3 at temperatures near T_N. We show that the coupling is…

Strongly Correlated Electrons · Physics 2009-11-10 Bas B. Van Aken , Thomas T. M. Palstra

Translation domains differing in the phase but not in the orientation of the corresponding order parameter are resolved in two types of multiferroics. Hexagonal (h-) YMnO$_3$ is a split-order-parameter multiferroic in which commensurate…

Strongly Correlated Electrons · Physics 2010-08-20 D. Meier , N. Leo , T. Jungk , E. Soergel , P. Becker , L. Bohaty , M. Fiebig

We report single-crystal neutron diffraction study of the magnetic structure of the multiferroic compound YbMnO$_3$, a member of the hexagonal manganite family, in zero-field and under a magnetic field applied along the $c$-axis. We propose…

Strongly Correlated Electrons · Physics 2018-11-14 S. Chattopadhyay , V. Simonet , V. Skumryev , A. A. Mukhin , V. Yu. Ivanov , M. I. Aroyo , D. Z. Dimitrov , M. Gospodinov , E. Ressouche

The aim of this work is to unravel a basic microscopic picture behind complex magnetic properties of hexagonal manganites. For these purposes, we consider two characteristic compounds: YMnO3 and LuMnO3, which form different magnetic…

Materials Science · Physics 2012-08-10 I. V. Solovyev , M. V. Valentyuk , V. V. Mazurenko