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Phase transformations can be difficult to characterize at the microscopic level due to the inability to directly observe individual atomic motions. Model colloidal systems, by contrast, permit the direct observation of individual particle…

Soft Condensed Matter · Physics 2015-04-21 Ye Yang , Lin Fu , Catherine Marcoux , Joshua E. S. Socolar , Patrick Charbonneau , Benjamin B. Yellen

It has been well established that particulate systems show the jamming transition and critical scaling behaviors associated with it. However, our knowledge is limited to (nearly) monodisperse systems. Recently, a binary mixture of jammed…

Soft Condensed Matter · Physics 2021-05-12 Yusuke Hara , Hideyuki Mizuno , Atsushi Ikeda

We report filling-fraction dependent dielectric spectroscopy measurements on the relaxation dynamics of the rod-like nematogen 7CB condensed in 13 nm silica nanochannels. In the film-condensed regime, a slow interface relaxation dominates…

Soft Condensed Matter · Physics 2015-04-21 Sylwia Calus , Andriy V. Kityk , Manfred Eich , Patrick Huber

Using Monte Carlo simulation, we analyse the behaviour of two-dimensional hard rods in four different types of geometric confinement: (i) a slit pore where the particles are confined between two parallel walls with homeotropic anchoring;…

Soft Condensed Matter · Physics 2018-11-13 Thomas Geigenfeind , Sebastian Rosenzweig , Matthias Schmidt , Daniel de las Heras

We consider a Lebwohl-Lasher model of chiral particles confined in a planar cell (slit pore) with different boundary conditions, and solve it using mean-field theory. The phase behaviour of the system with respect to temperature and pore…

Soft Condensed Matter · Physics 2015-09-18 Daniel de las Heras , Enrique Velasco , Yuri Martínez-Ratón

The influence of spatial confinement on the thermally excited stochastic cation dynamics of the room-temperature ionic liquid 1-N-butylpyridinium bis-((trifluoromethyl)sulfonyl)imide ([BuPy][Tf_2N]) inside porous carbide-derived carbons…

Chemical Physics · Physics 2020-06-02 Mark Busch , Tommy Hofmann , Bernhard Frick , Jan P. Embs , Boris Dyatkin , Patrick Huber

We use $^2$H NMR to study the rotational motion of supercooled water in silica pores of various diameters, specifically, in the MCM-41 materials C10, C12, and C14. Combination of spin-lattice relaxation, line-shape, and stimulated-echo…

Soft Condensed Matter · Physics 2015-06-22 Matthias Sattig , Stefan Reutter , Franz Fujara , Mayke Werner , Gerd Buntkowsky , Michael Vogel

In this paper we present a review on our recent experimental investigations into the phase behavior of the deeply cooled water confined in a nanoporous silica material, MCM-41, with elastic neutron scattering technique. Under such strong…

Soft Condensed Matter · Physics 2016-12-13 Zhe Wang , Kanae Ito , Sow-Hsin Chen

The behavior of a confined spherical symmetric anomalous fluid under high external pressure was studied with Molecular Dynamics simulations. The fluid is modeled by a ore-softened potential with two characteristic length scales, which in…

Soft Condensed Matter · Physics 2014-08-21 José Rafael Bordin , Leandro B. Krott , Marcia C. B. Barbosa

We study the structure and morphological changes of fluids that are in contact with solid composites formed by alternating and microscopically wide stripes of two different materials. One type of the stripes interacts with the fluid via…

Statistical Mechanics · Physics 2019-12-30 Martin Pospíšil , Martin Láska , Alexandr Malijevský

We show using computer simulations and mean field theory that a system of particles in two dimensions, when confined laterally by a pair of parallel hard walls within a quasi one dimensional channel, possesses several anomalous structural…

Soft Condensed Matter · Physics 2009-11-13 Debasish Chaudhuri , Surajit Sengupta

We investigate using molecular dynamics the effect of the structure of nanoconfinement for liquids with water-like anomalies and liquid-liquid phase transition (LLPT). We find that if the confinement is in an ordered matrix of nanoparticles…

Statistical Mechanics · Physics 2015-03-13 Elena G. Strekalova , Jiayuan Luo , H. Eugene Stanley , Giancarlo Franzese , Sergey V. Buldyrev

The impact of confinement on self-assembly of particles interacting with short-range attraction and long-range repulsion (SALR) potential is studied for thermodynamic states corresponding to local ordering of clusters or layers in the bulk.…

Soft Condensed Matter · Physics 2014-11-17 Jakub Pękalski , Alina Ciach , Noé G. Almarza

Close to a solid surface, the properties of a fluid deviate significantly from their bulk values. In this context, we study the surface adsorption profiles of a symmetric binary liquid confined to a slit pore by means of molecular dynamics…

Soft Condensed Matter · Physics 2025-01-15 Sutapa Roy , Felix Höfling

We present the first experimental measurements of the isotropic and nematic phases of mixtures of thin, charged semiflexible fd virus, and thick, fd-PEG created by covalently grafting poly-(ethylene glycol) to the the surface of fd, rods.…

Soft Condensed Matter · Physics 2009-11-10 Kirstin Purdy , Szabolcs Varga , Amparo Galindo , George Jackson , Seth Fraden

Despite their considerable practical and biological applications, the link between molecular properties, assembly conditions and self-organized structure in confined polymer solutions remains elusive. Here, we explore the lyotropic nematic…

Soft Condensed Matter · Physics 2023-03-21 Maxime M. C. Tortora , Daniel Jost

The effects of confinement on colloidal self-assembly in the case of fixed number of confined particles are studied in the one dimensional lattice model solved exactly in the Grand Canonical Ensemble (GCE) in [J. P\k{e}kalski et al. J.…

Soft Condensed Matter · Physics 2015-04-16 J. Pękalski , N. G. Almarza , A. Ciach

Computer simulations of (i) a [C12mim][Tf2N] film of nanometric thickness squeezed at kbar pressure by a piecewise parabolic confining potential reveal a mesoscopic in-plane density and composition modulation reminiscent of mesophases seen…

Materials Science · Physics 2009-11-19 N. Manini , M. Cesaratto , M. G. Del Popolo , P. Ballone

Fluid-induced alteration of rocks and mineral-based materials often starts at confined mineral interfaces where nm-thick water films can persist even at high overburden pressures and at low vapor pressures. These films enable transport of…

Materials Science · Physics 2019-07-04 Joanna Dziadkowiec , Bahareh Zareeipolgardani , Dag Kristian Dysthe , Anja Røyne

Using Brownian dynamics (BD) simulations and an analytical approach we investigate the shear-induced, nonequilibrium dynamics of dense colloidal suspensions confined to a narrow slit-pore. Focusing on situations where the colloids arrange…

Soft Condensed Matter · Physics 2017-01-04 Sascha Gerloff , Sabine H. L. Klapp
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