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Tunneling ionization followed by strong-field excitation leads to important ultrafast phenomena such as charge migration and lasing. Recent theoretical developments suggest that the population of the ionic excited state can be greatly…

Quantum Physics · Physics 2026-01-29 Chi-Hong Yuen

Interfacial ultrafast electron migration processes are simulated in finite cluster models of dye-sensitized solar cells within a single active electron approach. Initially, three different donor-acceptor $\pi$-conjugated dyes supported on…

Chemical Physics · Physics 2017-07-06 Gunter Hermann , Felix Witte , Jean Christophe Tremblay

In crowded systems, particle currents can be mediated by propagating collective excitations which are generated as rare events, are localized and have a finite lifetime. The theoretical description of such excitations is hampered by the…

Statistical Mechanics · Physics 2022-11-16 Alexander P. Antonov , David Voráč , Artem Ryabov , Philipp Maass

An important physical process unique to neutral-ion systems is the charge-transfer (CT) reaction. Here, we present measurements of and models for CT processes between co-trapped ultracold Ca atoms and Yb ions under well-controlled…

Chemical Physics · Physics 2019-07-24 Ming Li , Michael Mills , Prateek Puri , Alexander Petrov , Eric R. Hudson , Svetlana Kotochigova

Phenomena involving electron transfer are ubiquitous in nature, photosynthesis and enzymes or protein activity being prominent examples. Their deep understanding thus represents a mandatory scientific goal. Moreover, controlling the…

Chemical Physics · Physics 2017-12-01 Carlo Andrea Rozzi , Filippo Troiani , Ivano Tavernelli

A detailed theoretical investigation of rare gas atom clusters under intense short laser pulses reveals that the mechanism of energy absorption is akin to {\it enhanced ionization} first discovered for diatomic molecules. The phenomenon is…

Atomic and Molecular Clusters · Physics 2009-11-07 Christian Siedschlag , Jan-Michael Rost

The ignition of two-quantum collective emission of inverted sub-ensemble of radiators due to mutual interaction of this sub-ensemble with other two dipole active atomic subsystems in process of two-photon exchanges between the atoms through…

Quantum Physics · Physics 2010-12-20 Nicolae A. Enaki

Massively parallel ionization of many atoms in a cluster or bio-molecule is identified as new phenomenon of light-matter interaction which becomes feasible through short and intense FEL pulses. Almost simultaneously emitted from the…

Atomic and Molecular Clusters · Physics 2012-04-25 Christian Gnodtke , Ulf Saalmann , Jan-Michael Rost

Ultracold collisions of the polyatomic species CaOH are considered, in internal states where the collisions should be dominated by long-range dipole-dipole interactions. The computed rate constants suggest that evaporative cooling can be…

Chemical Physics · Physics 2019-06-25 Lucie D. Augustovičová , John L. Bohn

We report the experimental observation of quantum interference in the nuclear wave-packet dynamics driving ultrafast excitation-energy transfer in argon dimers below the threshold of interatomic Coulombic decay (ICD). Using time-resolved…

Atomic and Molecular Clusters · Physics 2023-07-05 Meng Han , Jacqueline Fedyk , Jia-Bao Ji , Victor Despré , Alexander I. Kuleff , Hans Jakob Wörner

Electron capture by {\it isolated} atoms and ions proceeds by photorecombination. In this process a species captures a free electron by emitting a photon which carries away the excess energy. It is shown here that in the presence of an {\it…

Quantum Physics · Physics 2010-03-18 Kirill Gokhberg , Lorenz S. Cederbaum

Coherent nuclear excitation in strongly laser-driven muonic atoms is calculated. The nuclear transition is caused by the time-dependent Coulomb field of the oscillating charge density of the bound muon. A closed-form analytical expression…

Nuclear Theory · Physics 2014-11-18 A. Shahbaz , C. Müller , T. J. Buervenich , C. H. Keitel

The translational motion of molecular ions can be effectively cooled sympathetically to temperatures below 100 mK in ion traps through Coulomb interactions with laser-cooled atomic ions. The distribution of internal rovibrational states,…

Quantum Physics · Physics 2009-11-07 I. S. Vogelius , L. B. Madsen , M. Drewsen

Photoionization of an atom $A$, in the presence of a neighboring atom $B$, can proceed via resonant excitation of $B$ with subsequent energy transfer to $A$ through two-center electron-electron correlation. We demonstrate that this…

Atomic Physics · Physics 2015-05-19 B. Najjari , A. B. Voitkiv , C. Müller

Multifragmentation is the dominant decay mode of heavy nuclear systems with excitation energies near their binding energies and is characterized by a multiple production of nuclear fragments with intermediate mass. At relativistic…

Nuclear Experiment · Physics 2007-05-23 W. Trautmann

Iron-sulfur clusters conduct a wide variety of biochemical reactions that are conserved across all domains of life. The hyperfine structure of reactive ligands of these clusters can be studied experimentally and theoretically by means of…

Chemical Physics · Physics 2025-08-22 William C. Robinson , Victoria Pascutti , David A. Hall , Martín A. Mosquera

The ionization of atomic hydrogen in intense laser fields is studied theoretically. The calculations were performed applying both quantummechanical and classical approaches. Treating the problem quantummechanically, the time dependent…

Atomic Physics · Physics 2009-11-13 S. Borbély , K. Tőkési , L. Nagy

The swing-up of quantum emitter population (SUPER) scheme allows to populate the excited state of a quantum emitter with near-unity fidelity using two red-detuned laser pulses. Its off-resonant, yet fully coherent nature has attracted…

Quantum Physics · Physics 2024-09-19 Luca Vannucci , Niels Gregersen

The ion phase-space dynamics in the Coulomb explosion of very large ($\sim 10^6 - 10^7$ atoms) deuterium clusters can be tailored using two consecutive laser pulses with different intensities and an appropriate time delay. For suitable sets…

Plasma Physics · Physics 2007-05-23 F. Peano , R. A. Fonseca , J. L. Martins , L. O. Silva

A novel way to induce ultrafast currents in molecular wires using two incident laser frequencies, $\omega$ and $2\omega$, is demonstrated. The mechanism relies on Stark shifts, instead of photon absorption, to transfer population to the…

Quantum Physics · Physics 2009-11-13 Ignacio Franco , Moshe Shapiro , Paul Brumer