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Spin-labeling of molecules with paramagnetic ions is an important approach for determining molecular structure, however current ensemble techniques lack the sensitivity to detect few isolated spins. In this Letter, we demonstrate…

Mesoscale and Nanoscale Physics · Physics 2014-12-03 Matthew Pelliccione , Bryan A. Myers , Laetitia Pascal , Ananda Das , Ania C. Bleszynski Jayich

Quantum sensors based on solid-state spins provide tremendous opportunities in a wide range of fields from basic physics and chemistry to biomedical imaging. However, integrating them into a scanning probe microscope to enable practical,…

Mesoscale and Nanoscale Physics · Physics 2016-01-19 Jean-Philippe Tetienne , Alain Lombard , David A. Simpson , Cameron Ritchie , Jianing Lu , Paul Mulvaney , Lloyd C. L. Hollenberg

Nuclear magnetic resonance (NMR) spectroscopy provides unparalleled access to molecular structure and dynamics but is traditionally limited by weak signal strength, requiring large sample volumes and high magnetic fields. Here, we…

Applied Physics · Physics 2026-04-29 Dileep Singh , Riley W. Hooper , Christoph Findler , Utsab Banerjee , Dominik B. Bucher

Nitrogen-vacancy (NV) centers in millimeter-scale diamond samples were produced by irradiation and subsequent annealing under varied conditions. The optical and spin relaxation properties of these samples were characterized using confocal…

Precision sensing and imaging of weak static magnetic fields are crucial for a variety of emerging nanoscale applications. While nitrogen-vacancy (NV) centers in diamond provide exceptional AC magnetic field sensitivity with nanoscale…

The last decade has seen an explosive growth in the use of color centers for metrology applications, the paradigm example arguably being the nitrogen-vacancy (NV) center in diamond. Here, we focus on the regime of cryogenic temperatures and…

Mesoscale and Nanoscale Physics · Physics 2023-12-06 Richard Monge , Tom Delord , Gergő Thiering , Ádám Gali , Carlos A. Meriles

The nitrogen vacancy (NV) center in diamond is a versatile color center used for magnetometry, quantum computing, and quantum communications. In this article, using a single laser beam as a pump and probe, we measure the spin states of the…

Applied Physics · Physics 2025-05-28 Reza Kashtiban , Gavin W. Morley , Mark E. Newton , A T M Anishur Rahman

When probing nuclear spins in materials on the nanometer scale, random fluctuations of the spin polarization will exceed the mean Boltzmann polarization for sample volumes below about (100nm)^3. In this work, we use magnetic resonance force…

Mesoscale and Nanoscale Physics · Physics 2008-01-14 C. L. Degen , M. Poggio , H. J. Mamin , D. Rugar

We employ the technique of optical detection of magnetic resonance to study dipolar interaction in diamond between nitrogen-vacancy color centers of different crystallographic orientations and substitutional nitrogen defects. We demonstrate…

Quantum Physics · Physics 2021-05-05 Sergei Masis , Sergey Hazanov , Nir Alfasi , Oleg Shtempluck , Eyal Buks

A single nitrogen-vacancy (NV) center in diamond is a prime candidate for a solid-state quantum magnetometer capable of detecting single nuclear spins with prospective application to nuclear magnetic resonance (NMR) at the nanoscale.…

Quantum Physics · Physics 2020-02-07 Daiki Misonou , Kento Sasaki , Shuntaro Ishizu , Yasuaki Monnai , Kohei M. Itoh , Eisuke Abe

Non-inductive magnetometers based on solid-state spins offer a promising solution for small-volume nuclear magnetic resonance (NMR) detection. A remaining challenge is to operate at a sufficiently high magnetic field to resolve chemical…

We present a highly sensitive miniaturized cavity-enhanced room-temperature magnetic-field sensor based on nitrogen-vacancy (NV) centers in diamond. The magnetic resonance signal is detected by probing absorption on the 1042\,nm…

While nitrogen-vacancy (NV-) centers have been extensively investigated in the context of spin-based quantum technologies, the spin-state readout is conventionally performed optically, which may limit miniaturization and scalability. Here,…

Nitrogen vacancy (NV) centers in diamond are widely deployed as local magnetic sensors, using coherent, single qubit control to measure both time-averaged fields and noise with nanoscale spatial resolution. Moving beyond single qubits to…

Quantum Physics · Physics 2025-04-18 Jared Rovny , Shimon Kolkowitz , Nathalie P. de Leon

Optically accessible spin-active nanomaterials are promising as quantum nanosensors for probing biological samples. However, achieving bioimaging-level brightness and high-quality spin properties for these materials is challenging and…

We propose an all-optical scheme to prolong the quantum coherence of a negatively charged nitrogen-vacancy (NV) center in diamond. Optical control of the NV spin suppresses energy fluctuations of the $^{3}\text{A}_{2}$ ground states and…

Quantum Physics · Physics 2014-08-18 Zhen-Yu Wang , Jian-Ming Cai , Alex Retzker , Martin B. Plenio

The nitrogen-vacancy (NV) center is a potential atomic-scale spin sensor for electric field sensing. However, its natural susceptibility to the magnetic field hinders effective detection of the electric field. Here we propose a robust…

Nuclear spin ensembles in diamond are promising candidates for quantum sensing applications, including rotation sensing. Here we perform a characterization of the optically detected nuclear-spin transitions associated with the 14N nuclear…

The excellent sensitivities of quantum sensors are a double-edged sword: minuscule quantities can be observed, but any undesired signal acts as noise. This is challenging when detecting quantities that are obscured by such noise. Decoupling…

We study the coupling of a single nitrogen-vacancy center in diamond to a nearby single nitrogen defect at room temperature. The magnetic dipolar coupling leads to a splitting in the electron spin resonance frequency of the nitrogen-vacancy…

Quantum Physics · Physics 2007-05-23 R. Hanson , F. M. Mendoza , R. J. Epstein , D. D. Awschalom