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A Stark decelerator is an effective tool for controlling motional degrees of freedom of polar molecules. Due to technical limitations, many of the current Stark decelerators focus on molecules in low-field-seeking quantum states and are…

Atomic Physics · Physics 2017-05-25 Demitri Y. Balabanov , Liam M. Duffy

A microstructured array of 1254 electrodes on a substrate has been configured to generate an array of local minima of electric field strength with a periodicity of 120 $\mu$m about 25 $\mu$m above the substrate. By applying sinusoidally…

Atomic Physics · Physics 2009-05-20 Samuel A Meek , Horst Conrad , Gerard Meijer

With a Stark decelerator, beams of neutral polar molecules can be accelerated, guided at a constant velocity, or decelerated. The effectiveness of this process is determined by the 6D volume in phase space from which molecules are accepted…

Atomic and Molecular Clusters · Physics 2009-11-13 Ludwig Scharfenberg , Henrik Haak , Gerard Meijer , Sebastiaan Y. T. van de Meerakker

Stark deceleration has been utilized for slowing and trapping several species of neutral, ground-state polar molecules generated in a supersonic beam expansion. Due to the finite physical dimension of the electrode array and practical…

Atomic Physics · Physics 2009-11-10 Eric R. Hudson , J. R. Bochinski , H. J. Lewandowski , Brian C. Sawyer , Jun Ye

We demonstrate experimentally the guiding of cold and slow ND3 molecules along a thin charged wire over a distance of ~0.34 m through an entire molecular beam apparatus. Trajectory simulations confirm that both linear and quadratic…

Atomic and Molecular Clusters · Physics 2011-12-19 M. Strebel , S. Spieler , F. Stienkemeier , M. Mudrich

Stark deceleration is a technique that uses time-varying inhomogeneous electric fields to decelerate polar molecules for various molecular beam and trapping experiments. New ring-geometry Stark decelerators with continuously varying…

Chemical Physics · Physics 2017-12-20 Yomay Shyur , Jason A. Bossert , H. J. Lewandowski

We report on the deceleration of a beam of SrF molecules from 290 to 120~m/s. Following supersonic expansion, the molecules in the $X^2\Sigma$ ($v=0$, $N=1$) low-field seeking states are trapped by the moving potential wells of a…

Atomic Physics · Physics 2019-07-17 S. C. Mathavan , A. Zapara , Q. Esajas , S. Hoekstra

Stark deceleration enables the production of cold and dense molecular beams with applications in trapping, collisional studies, and precision measurement. Improving the efficiency of Stark deceleration, and hence the achievable molecular…

Chemical Physics · Physics 2020-07-22 David Reens , Hao Wu , Alexander Aeppli , Anna McAuliffe , Piotr Wcisło , Tim Langen , Jun Ye

We demonstrate feedback control optimization for the Stark deceleration and trapping of neutral polar molecules using evolutionary strategies. In a Stark-decelerator beamline pulsed electric fields are used to decelerate OH radicals and…

We produce SO_2 molecules with a centre of mass velocity near zero using a Stark decelerator. Since the initial kinetic energy of the supersonic SO_2 molecular beam is high, and the removed kinetic energy per stage is small, 326…

Atomic Physics · Physics 2009-11-13 O. Bucicov , M. Nowak , S. Jung , G. Meijer , E. Tiemann , Ch. Lisdat

We here report on the experimental realization of a microwave decelerator for neutral polar molecules, suitable for decelerating and focusing molecules in high-field-seeking states. The multi-stage decelerator consists of a cylindrical…

Chemical Physics · Physics 2015-06-04 Simon Merz , Nicolas Vanhaecke , Wolfgang Jäger , Melanie Schnell , Gerard Meijer

We present experiments on decelerating and trapping ammonia molecules using a combination of a Stark decelerator and a traveling wave decelerator. In the traveling wave decelerator a moving potential is created by a series of ring-shaped…

Stark deceleration allows for precise control over the velocity of a pulsed molecular beam and, by the nature of its limited phase-space acceptance, reduces the energy width of the decelerated packet. We describe an alternate method of…

Atomic Physics · Physics 2015-05-13 L. P. Parazzoli , N. Fitch , D. S. Lobser , H. J. Lewandowski

We demonstrate the deceleration of heavy polar molecules in low-field seeking states by combining a cryogenic source and a travelling-wave Stark decelerator. The cryogenic source provides a high intensity beam with low speed and…

We describe the production of cold, slow-moving LiH molecules. The molecules are produced in the ground state using laser ablation and supersonic expansion, and 68% of the population is transferred to the rotationally excited state using…

Atomic Physics · Physics 2015-05-13 S. K. Tokunaga , J. M. Dyne , E. A. Hinds , M. R. Tarbutt

We report on the Stark deceleration of a pulsed molecular beam of NO radicals. Stark deceleration of this chemically important species has long been considered unfeasible due to its small electric dipole moment of 0.16 D. We prepared the NO…

Chemical Physics · Physics 2013-01-11 Xingan Wang , Moritz Kirste , Gerard Meijer , Sebastiaan Y. T. van de Meerakker

A new type of decelerator is presented where polar neutral molecules are guided and decelerated using the principle of traveling electric potential wells, such that molecules are confined in stable three-dimensional traps throughout. This…

Atomic Physics · Physics 2010-05-24 Andreas Osterwalder , Samuel A. Meek , Georg Hammer , Henrik Haak , Gerard Meijer

Recently, a decelerator for neutral polar molecules has been presented that operates on the basis of macroscopic, three-dimensional, traveling electrostatic traps (Osterwalder et al., Phys. Rev. A 81, 051401 (2010)). In the present paper, a…

Producing large samples of slow molecules from thermal-velocity ensembles is a formidable challenge. Here we employ a centrifugal force to produce a continuous molecular beam with a high flux at near-zero velocities. We demonstrate…

Chemical Physics · Physics 2018-12-04 S. Chervenkov , X. Wu , J. Bayerl , A. Rohlfes , T. Gantner , M. Zeppenfeld , G. Rempe

We report the Stark deceleration of CaF molecules in the strong-field seeking ground state and in a weak-field seeking component of a rotationally-excited state. We use two types of decelerator, a conventional Stark decelerator for the…

Atomic Physics · Physics 2017-09-13 T. E. Wall , J. F. Kanem , J. M. Dyne , J. J. Hudson , B. E. Sauer , E. A. Hinds , M. R. Tarbutt
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