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It was recently suggested that molecular junctions would be excellent elements for efficient and high-power thermoelectric energy conversion devices. However, experimental measurements of thermoelectric conversion in molecular junctions…

Mesoscale and Nanoscale Physics · Physics 2015-06-09 Elinor Zerah-Harush , Yonatan Dubi

We investigate the effect of vibrational degrees of freedom on the linear thermoelectric transport through a single-level quantum dot described by the spinless Anderson-Holstein impurity model. To study the effects of strong electron-phonon…

Strongly Correlated Electrons · Physics 2017-11-30 A. Khedri , V. Meden , T. A. Costi

We study electron transport in nanojunctions in which an electron on a quantum dot or a molecule is interacting with an N-state local impurity, a harmonic ("Holstein") mode, or a two-state system ("spin"). These two models, the…

Mesoscale and Nanoscale Physics · Physics 2014-07-23 Lena Simine , Dvira Segal

The search for the signature of non-thermal (so-called ``hot'') electrons in illuminated plasmonic nanostructures requires a detailed understanding of the non-equilibrium electron distribution under illumination, as well as a careful design…

Mesoscale and Nanoscale Physics · Physics 2023-03-31 Yonatan Dubi , Ieng-Wai Un , Yonatan Sivan

We study the model of a molecular switch comprised of a molecule with a soft vibrational degree of freedom coupled to metallic leads. In the presence of strong electron-ion interaction, different charge states of the molecule correspond to…

Mesoscale and Nanoscale Physics · Physics 2008-12-18 Fabio Pistolesi , Yaroslav M. Blanter , Ivar Martin

Understanding and controlling the flow of heat is a major challenge in nanoelectronics. When a junction is driven out of equilibrium by light or the flow of electric charge, the vibrational and electronic degrees of freedom are, in general,…

Mesoscale and Nanoscale Physics · Physics 2011-06-29 Daniel R. Ward , David A. Corley , James M. Tour , Douglas Natelson

Molecular adsorbates on metal surfaces exchange energy with substrate phonons and low-lying electron-hole pair excitations. In the limit of weak coupling, electron-hole pair excitations can be seen as exerting frictional forces on…

Materials Science · Physics 2016-09-28 Reinhard J. Maurer , Mikhail Askerka , Victor S. Batista , John C. Tully

The calculation of the nonlinear conductance of a single-molecule junction is revisited. The self energy on the junction resulting from the electron-phonon interaction has at low temperatures logarithmic singularities (in the real part) and…

Mesoscale and Nanoscale Physics · Physics 2015-05-14 O. Entin-Wohlman , Y. Imry , A. Aharony

The thermoelectric performance of a topological Josephson nonlocal heat engine is thoroughly investigated. The nonlocal response is obtained by using a normal metal probe coupled with only one of the proximized helical edges in the middle…

Mesoscale and Nanoscale Physics · Physics 2021-07-07 Gianmichele Blasi , Fabio Taddei , Liliana Arrachea , Matteo Carrega , Alessandro Braggio

We study full counting statistics for classical heat transport through anharmonic/nonlinear molecular junctions formed by interacting oscillators. Analytical result of the steady state heat flux for an overdamped anharmonic junction with…

Statistical Mechanics · Physics 2013-03-13 Sha Liu , Bjiay Kumar Agarwalla , Jian-Sheng Wang , Baowen Li

This work concerns the theoretical description of the quantum dynamics of molecular junctions with thermal fluctuations and probability losses To this end, we propose a theory for describing non-Hermitian quantum systems embedded in…

Quantum Physics · Physics 2021-02-24 Andrea Grimaldi , Alessandro Sergi , Antonino Messina

We investigate on the same footing the time-dependent electronic transport properties and vibrational dynamics of a molecular junction. We show that fluctuations of both the molecular vibron displacement and the electronic current across…

Mesoscale and Nanoscale Physics · Physics 2019-03-27 Rémi Avriller , R Souto , A. Martin-Rodero , A Yeyati

In condensed matter systems with the Coulomb interaction playing an important role one expects, besides the on-site (local) Hubbard-type interaction, that also other (non-local) terms depending on the site occupancy, known as correlated or…

Mesoscale and Nanoscale Physics · Physics 2024-12-30 Ulrich Eckern , Karol I. Wysokiński

The role of multimode vibrational dynamics in electron transport through single molecule junctions is investigated. The study is based on a generic model, which describes charge transport through a single molecule that is attached to metal…

Mesoscale and Nanoscale Physics · Physics 2010-10-26 R. Härtle , C. Benesch , M. Thoss

Thermal transmission in a molecular transistor with fully spin-polarized electrodes subjected to a temperature gradient is considered. The problem has been solved by using density matrix method in perturbation approach over small tunneling…

Mesoscale and Nanoscale Physics · Physics 2022-07-12 A. D. Shkop

The vibrational dynamics of adsorbate molecules in single-molecule junctions depend critically on the geometric structure and electronic interactions between molecule and substrate. Vibrations, excited mechanochemically or by external…

Mesoscale and Nanoscale Physics · Physics 2025-09-17 Lukas Hörmann , Reinhard J. Maurer

Advancing the debate on quantum effects in light-initiated reactions in biology requires clear identification of non-classical features that these processes can exhibit and utilise. Here we show that in prototype dimers present in a variety…

Quantum Physics · Physics 2014-01-10 Edward J. O'Reilly , Alexandra Olaya-Castro

We study the thermopower of a junction between a metal and a strongly correlated semiconductor. Both in the electronic ferroelectric regime and in the Kondo insulator regime the thermoelectric figures of merit, ZT, of these junctions are…

Strongly Correlated Electrons · Physics 2009-07-20 Massimo Rontani , L. J. Sham

We study the nonlinear thermoelectric cooling performance of a quantum spin Hall system. The setup consists of a nanomagnet contacting a Kramers' pair of helical edge states, resulting in a transmission probability with a rich structure…

Mesoscale and Nanoscale Physics · Physics 2020-11-04 Fatemeh Hajiloo , Pablo Terrén Alonso , Nastaran Dashti , Liliana Arrachea , Janine Splettstoesser

Charge and heat transport through a single molecule tunnel-coupled to external normal electrodes have been studied. The molecule with sufficiently strong interaction between lectrons and vibrational internal degrees of freedom can be…

Mesoscale and Nanoscale Physics · Physics 2012-04-16 Karol Izydor Wysokinski