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In addition to the well-known Landauer-Buttiker scattering theory and the nonequilibrium Green's function technique for mesoscopic transports, an alternative (and very useful) scheme is quantum master equation approach. In this article, we…

Quantum Physics · Physics 2016-07-04 Xin-Qi Li

Coupling the vibrations of an oscillator to electronic transport is a key building block for nanoelectromechanical systems. They describe many nanoscale electrical components such as molecular junctions. Inspired by recent experimental…

Quantum Physics · Physics 2025-06-26 Sofia Sevitz , Federico Cerisola , Janet Anders

We recall theoretical studies on transient transport through interacting mesoscopic systems. It is shown that a generalized master equation (GME) written and solved in terms of many-body states provides the suitable formal framework to…

Mesoscale and Nanoscale Physics · Physics 2019-08-02 Valeriu Moldoveanu , Andrei Manolescu , Vidar Gudmundsson

We consider a molecular aggregate consisting of $N$ identical monomers. Each monomer comprises two electronic levels and a single harmonic mode. The monomers interact with each other via dipole-dipole forces. The monomer vibrational modes…

Statistical Mechanics · Physics 2012-04-12 Maxim F. Gelin , Dassia Egorova , Wolfgang Domcke

A generalized master equation (GME) governing quantum evolution of modular exciton density (MED) is derived for large scale light harvesting systems composed of weakly interacting modules of multiple chromophores. The GME-MED offers a…

Quantum Physics · Physics 2013-11-12 Seogjoo Jang , Stephan Hoyer , Graham Fleming , K. Birgitta Whaley

Modern 4-wave mixing spectroscopies are expensive to obtain experimentally and computationally. In certain cases, the unfavorable scaling of quantum dynamics problems can be improved using a generalized quantum master equation (GQME)…

Chemical Physics · Physics 2024-05-16 Thomas Sayer , Andrés Montoya-Castillo

We put forth a new class of quantum master equations that correctly reproduce the asymptotic state of an open quantum system beyond the infinitesimally weak system-bath coupling limit. Our method is based on incorporating the knowledge of…

Quantum Physics · Physics 2022-11-10 Tobias Becker , Alexander Schnell , Juzar Thingna

A quantum master equation is obtained for identical fermions by including a relaxation term in addition to the mean-field Hamiltonian. [Huang C F and Huang K N 2004 Chinese J. Phys. ${\bf 42}$ 221; Gebauer R and Car R 2004 Phys. Rev. B…

Quantum Physics · Physics 2007-06-30 C. F. Huang , K. -N. Huang

Time-dependent currents in molecular junctions can be caused by structural fluctuations or interaction with external fields. In this publication, we demonstrate how the hierarchical quantum master equation approach can be used to study…

Mesoscale and Nanoscale Physics · Physics 2019-03-27 Andre Erpenbeck , Lukas Götzendörfer , Christian Schinabeck , Michael Thoss

Methods derived from the generalized quantum master equation (GQME) framework have provided the basis for elucidating energy and charge transfer in systems ranging from molecular solids to photosynthetic complexes. Recently, the…

Chemical Physics · Physics 2019-07-24 William C. Pfalzgraff , Andrés Montoya Castillo , Aaron Kelly , Thomas E. Markland

The population transfer dynamics of model donor-bridge-acceptor systems is studied by comparing a recently developed polaron-transformed quantum master equation (PQME) with the well-known Redfield and Forster theories of quantum transport.…

Mesoscale and Nanoscale Physics · Physics 2015-08-12 Seogjoo Jang , Timothy C. Berkelbach , David R. Reichman

We discuss recent findings about properties of quantum nonequilibrium steady states. In particular we focus on transport properties. It is shown that the time dependent density matrix renormalization method can be used successfully to find…

Quantum Physics · Physics 2011-11-15 Marko Znidaric

We present an efficient theoretical method for calculating the time evolution of the density matrix of a multilevel quantum system weakly interacting with incoherent light. The method combines the Bloch-Redfield theory with a partial…

Chemical Physics · Physics 2015-06-23 Timur V. Tscherbul , Paul Brumer

A perturbative quantum master equation is derived for a system interacting with its environment, which is more general than the ones derived before. Our master equation takes into account the effect of the energy exchanges between the…

Statistical Mechanics · Physics 2009-11-10 M. Esposito , P. Gaspard

Generalized quantum master equations (GQMEs) are an important tool in modeling chemical and physical processes. For a large number of problems it has been shown that exact and approximate quantum dynamics methods can be made dramatically…

Chemical Physics · Physics 2016-05-25 Aaron Kelly , Andrés Montoya-Castillo , Lu Wang , Thomas E. Markland

Understanding nonsecular dynamics in open quantum systems is addressed here, with emphasis on systems with large numbers of Bohr frequencies, zero temperature, and fast driving. We employ the master equation, which replaces arithmetic…

Quantum Physics · Physics 2022-11-15 Dragomir Davidovic

The propagation of a fast particle in a low-density gas at thermal equilibrium is studied in the context of quantum mechanics. A quantum master equation in the Redfield form governing the reduced density matrix of the particle is derived…

Quantum Physics · Physics 2022-12-20 David Gaspard

Master equations are a vital tool to model heat flow through nanoscale thermodynamic systems. Most practical devices are made up of interacting sub-system, and are often modelled using either local master equations (LMEs) or global master…

Quantum Physics · Physics 2021-05-05 Stefano Scali , Janet Anders , Luis A. Correa

In this article we show how Ehrenfest mean field theory can be made both a more accurate and efficient method to treat nonadiabatic quantum dynamics by combining it with the generalized quantum master equation framework. The resulting mean…

Chemical Physics · Physics 2015-06-23 Aaron Kelly , Nora Brackbill , Thomas E. Markland

We discuss methods for numerically solving the generalized Master equation GME which governs the time-evolution of the reduced density matrix of a mechanically movable mesoscopic device in a dissipative environment. As a specific example,…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Antti-Pekka Jauho , Tomas Novotny , Andrea Donarini , Christian Flindt