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We propose a new scenario to apply IR-pump-XUV-probe schemes to resolving strong field ionization induced and attosecond pulse driven electron-hole dynamics and coherence in real time. The coherent driving of both the infrared laser and the…

Atomic Physics · Physics 2016-02-26 Jing Zhao , Jianmin Yuan , Zengxiu Zhao

We consider the ionization of neon induced by a femtosecond laser pulse composed of overlapping, linearly polarized bichromatic extreme ultraviolet and infrared fields. In particular, we study the effects of the infrared light on a…

Atomic Physics · Physics 2017-01-25 Nicolas Douguet , Alexei N. Grum-Grzhimailo , Klaus Bartschat

Superfluid He nanodroplets resonantly excited by extreme ultraviolet (XUV) pulses exhibit complex relaxation dynamics, including the formation of metastable excited He$^*$ atoms trapped in bubbles, the desorption of excited atoms from the…

The evolution of electron wavepackets determines the course of many physical and chemical phenomena and attosecond spectroscopy aims to measure and control such dynamics in real-time. Here, we investigate radial electron wavepacket motion…

Atomic Physics · Physics 2015-09-04 Niranjan Shivaram , Xiao-Min Tong , Henry Timmers , Arvinder Sandhu

We propose an attosecond XUV-pump IR-probe photoionization protocol that employs pairs of counter-rotating consecutive harmonics and angularly resolved photoelectron detection, thereby providing direct measurement of ionization phases. The…

Atomic Physics · Physics 2019-10-02 Stefan Donsa , Nicolas Douguet , Joachim Burgdörfer , Iva Březinová , Luca Argenti

We study orientation and two-center interference effects in attosecond time-resolved photoionization of the H$_2$ molecule. Time resolution of XUV ionization of H$_2$ is gained through the phase retrieval capability of attosecond angular…

Atomic Physics · Physics 2026-03-03 Vladislav V. Serov , Anatoli S. Kheifets

We study the breakup of $\text{H}_2^+$ exposed to super-intense, femtosecond laser pulses with frequencies greater than that corresponding to the ionization potential. By solving the time-dependent Schr\"odinger equation in an extensive…

Atomic Physics · Physics 2016-04-12 Lun Yue , Lars Bojer Madsen

We present theoretical studies on real-time probing the electron density evolution of an atom in a strong infrared (IR) laser field with few-cycle near-infrared (NIR) and attosecond extreme-ultraviolet (XUV) pulses. Our results indicate…

Atomic Physics · Physics 2015-06-04 Yunpei Deng , Xinhua Xie

High intensity XUV radiation from a free-electron (FEL) was used to create a nanoplasma inside ammonia clusters with the intent of studying the resulting electron-ion interactions and their interplay with plasma evolution. In a plasma-like…

Photoelectron emission from excited states of laser-dressed atomic helium is analyzed with respect to laser intensity-dependent excitation energy shifts and angular distributions. In the two-color XUV (exteme ultra\-violet) -- IR (infrared)…

Coherent sources of attosecond extreme ultraviolet (XUV) radiation present many challenges if their full potential is to be realized. While many applications benefit from the broadband nature of these sources, it is also desirable to…

Coherence among rotational ion channels during photoionization is exploited to control the anisotropy of the resulting photoelectron angular distributions at specific photoelectron energies. The strategy refers to a robust and single…

Chemical Physics · Physics 2019-09-11 R. Chamakhi , M. Telmini , O. Atabek , E. Charron

Time delays of electrons emitted from an isotropic initial state and leaving behind an isotropic ion are assumed to be angle-independent. Using an interferometric method involving XUV attosecond pulse trains and an IR probe field in…

Attosecond pulses can be used to initiate and control electron dynamics on a sub-femtosecond time scale. The first step in this process occurs when an atom absorbs an ultraviolet photon leading to the formation of an attosecond electron…

Atomic Physics · Physics 2007-12-11 P. Johnsson , J. Mauritsson , T. Remetter , A. LHuillier , K. J. Schafer

Based on numerical solutions of the time-dependent Schr\"odinger equation for either one or two active electrons, we propose a method for observing instantaneous level shifts in an oscillating strong infrared (IR) field in time, using a…

Atomic Physics · Physics 2015-05-28 Feng He , Camilo Ruiz , Andreas Becker , Uwe Thumm

We investigate ionization of neon atoms by an isolated attosecond pump pulse in the presence of two coherent extreme ultraviolet or x-ray probe fields. The probe fields are tuned to a core-valence transition in the residual ion and induce…

Atomic Physics · Physics 2016-03-30 Jhih-An You , Nina Rohringer , Jan Marcus Dahlström

We present and discuss a new computationally inexpensive method to study, within the single active electron approximation, the interaction of a complex system with an intense ultrashort laser pulse. As a first application, we consider the…

Ionization of acetylene by linearly-polarized, vacuum ultraviolet (VUV) laser pulses is modelled using time-dependent density functional theory. Several laser wavelengths are considered including one that produces direct ionization to the…

Atomic Physics · Physics 2017-04-24 Daniel Dundas , Peter Mulholland , Abigail Wardlow , Alejandro de la Calle

We study the nonlinear and resonant process of two-photon ionization of atoms (He and H) in a pump-probe scheme. The pump pulse prepares the quantum system in a superposition of the ground state and an excited bound state. By varying the…

The development of attosecond technology has enabled the real-time observation of coherent electron motion in atoms, molecules and condensed phases. Experimentally, it is now possible to generate laser pulses of durations of only a few tens…

Chemical Physics · Physics 2017-05-18 David Ayuso