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X-ray Photon Correlation Spectroscopy (XPCS) enables direct access to atomic-scale dynamics in disordered materials, revealing both spontaneous and X-ray-induced relaxation processes. Here, we study two compositionally similar alloy glasses…

Temperature dependence of relaxation dynamics of UX$_{3}$ (X = Al, Ga, Sn) compounds is studied using time resolved pump-probe technique in the reflectance geometry. UGa$_{3}$ is an itinerant antiferromagnet, while UAl$_{3}$ and USn$_{3}$…

Strongly Correlated Electrons · Physics 2015-06-05 Saritha K. Nair , J. -X. Zhu , J. L. Sarrao , A. J. Taylor , Elbert E. M. Chia

Modern detector technology and highly brilliant fourth-generation synchrotrons allow to improve the temporal resolution in time-resolved diffraction studies. Profiting from this, we applied temperature scanning X-ray photon correlation…

Orientational dynamics in a liquid crystalline system near the isotropic-nematic (I-N) phase transition is studied using Molecular Dynamics simulations of the well-known Lebwohl-Lasher (LL) model. As the I-N transition temperature is…

Soft Condensed Matter · Physics 2009-11-11 Suman Chakrabarty , Dwaipayan Chakrabarti , Biman Bagchi

Quantum fluctuations of the electromagnetic vacuum are responsible for physical effects such as the Casimir force and the radiative decay of atoms, and set fundamental limits on the sensitivity of measurements. Entanglement between photons…

Quantum Physics · Physics 2013-07-10 K. W. Murch , S. J. Weber , K. M. Beck , Eran Ginossar , I. Siddiqi

We use molecular dynamics computer simulations to study the relaxation dynamics of Na2O-2(SiO2) in its molten, highly viscous state. We find that at low temperatures the incoherent intermediate scattering function for Na relaxes about 100…

Statistical Mechanics · Physics 2009-11-07 Jurgen Horbach , Walter Kob

Using approximate partition functions and a master equation approach, we investigate the statistical relaxation toward equilibrium in selected CaAr$_n$ clusters. The Gaussian theory of absorption (previous article) is employed to calculate…

Chemical Physics · Physics 2009-11-07 F. Calvo , F. Spiegelman , D. J. Wales

We investigated temperature ($T$) dependent ultrafast near-infrared (NIR) transient reflectivity dynamics in coexisting superconducting (SC) and charge density wave (CDW) phases of two-dimensional 2H-NbSe$_{2}$ using NIR and visible…

A recently proposed expression to describe the temperature and volume dependences of the structural (or alpha) relaxation time is discussed. This equation satisfies the scaling law for the relaxation times, tau = f(TV^g), where T is…

Soft Condensed Matter · Physics 2009-11-13 R. Casalini , C. M. Roland

We theoretically study the propagation through a resonant absorbing medium of a time-dependent perturbation modulating the amplitude of a continuous wave (cw). Modeling the medium as a system of two-level atoms and linearizing the…

Optics · Physics 2010-09-13 Bruno Macke , Bernard Ségard

Complex systems, which consist of a large number of interacting constituents, often exhibit universal behavior near a phase transition. A slowdown of certain dynamical observables is one such recurring feature found in a vast array of…

Molecular dynamics simulations are used to investigate the connection between thermal history and physical aging in polymer glasses, in particular the effects of a temperature square step. Measurements of two-time correlation functions show…

Soft Condensed Matter · Physics 2009-11-13 Mya Warren , Joerg Rottler

The $\alpha$-process (segmental motion) of thin polystyrene films supported on glass substrate has been investigated in a wider frequency range from 10$^{-3}$ Hz to 10$^4$ Hz using dielectric relaxation spectroscopy and thermal expansion…

Soft Condensed Matter · Physics 2009-10-31 Koji Fukao , Yoshihisa Miyamoto

Applying coherent X-rays by the method of atomic-scale X-ray Photon Correlation Spectroscopy results in beam-induced dynamics in a number of oxide glasses. Here these studies are extended to rubidium and caesium borates with varying alkali…

Within the framework of V-T theory of monatomic liquid dynamics, an exact equation is derived for a general equilibrium time correlation function. The purely vibrational contribution to such a function expresses the system's motion in one…

Soft Condensed Matter · Physics 2007-05-23 Eric D. Chisolm , Giulia De Lorenzi-Venneri , Duane C. Wallace

We report X-ray Photon Correlation Spectroscopy (XPCS) results on a bidimensional (2D) gel formed by a Langmuir monolayer of gold nanoparticles. The system allows an experimental determination of the fourth order time correlation function…

Soft Condensed Matter · Physics 2012-03-29 D. Orsi , L. Cristofolini , G. Baldi , A. Madsen

We have experimentally studied the pump-probe Kerr rotation dynamics in WSe$_2$ monolayers. This yields a direct measurement of the exciton valley depolarization time $\tau_v$. At T=4K, we find $\tau_v\approx 6$ps, a fast relaxation time…

Mesoscale and Nanoscale Physics · Physics 2014-10-10 C. R. Zhu , K. Zhang , M. Glazov , B. Urbaszek , T. Amand , Z. W. Ji , B. L. Liu , X. Marie

We present Molecular Dynamics simulations of the thermal glass transition in a dense model polymer liquid. We performed a comparative study of both constant volume and constant pressure cooling of the polymer melt. Great emphasis was laid…

Statistical Mechanics · Physics 2009-10-30 C. Bennemann , W. Paul , K. Binder , B. Duenweg

We show that for any liquid or solid with strong correlation between its $NVT$ virial and potential-energy equilibrium fluctuations, the temperature is a product of a function of excess entropy per particle and a function of density,…

Soft Condensed Matter · Physics 2012-03-13 Trond S. Ingebrigtsen , Lasse Bøhling , Thomas B. Schrøder , Jeppe C. Dyre

We examine the interplay between electron correlations and phonons in an Anderson-Holstein impurity model with an Einstein phonon. When the phonons are slow compared to charge fluctuations (frequency $\omega_0 \ll U/2$, the onsite Coulomb…

Strongly Correlated Electrons · Physics 2025-07-08 Liam L. H. Lau , Andreas Gleis , Daniel Kaplan , Premala Chandra , Piers Coleman