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The rheology of coextruded layered films of polystyrene/poly(methyl methacrylate) (PS/PMMA) has been studied with small and large amplitude oscillations at a temperature above their glass transition. While the complex viscosity remains…

Soft Condensed Matter · Physics 2025-04-25 Anna Dmochowska , Jorge Peixinho , Cyrille Sollogoub , Guillaume Miquelard-Garnier

We investigate the effects of chain flexibility on the self-assembly behavior of symmetric diblock copolymers (BCPs) when they are confined as a thin film between two surfaces. Employing worm-like chain (WLC) self-consistent field theory,…

Soft Condensed Matter · Physics 2023-08-07 Mingyang Chen , Yuguo Chen , Yanyan Zhu , Ying Jiang , David Andelman , Xingkun Man

We demonstrate scaffolding of plasmonic nanoparticles by topological defects induced by colloidal microspheres to match their surface boundary conditions with a uniform far-field alignment in a liquid crystal host. Displacing energetically…

Block copolymers often create droplets when placed on a substrate. Such nanostructured droplets can be arranged into regular microstructured arrays, thereby forming hierarchically organized materials that can be used in microelectronics,…

Soft Condensed Matter · Physics 2026-05-04 Artem Petrov , Guillermo A. Hernández-Mendoza , Alfredo Alexander-Katz

The ordering of nanoparticles into predetermined configurations is of importance to the design of advanced technologies. In this work, we moderate the surface anchoring against the bulk elasticity of liquid crystals to dynamically shape…

Soft Condensed Matter · Physics 2023-12-01 Lisa Tran , Hye-Na Kim , Ningwei Li , Shu Yang , Kathleen J. Stebe , Randall D. Kamien , Martin F. Haase

The ability to assemble mesoscopic colloidal lattices above a surface is important for fundamental studies related with nucleation and crystallization, but also for a variety of technological applications in photonics and micro-engineering.…

Soft Condensed Matter · Physics 2019-08-27 Pietro Tierno

We explore the relative stability of three possible orientations of cylinder-forming di-block copolymer on a sinusoidally corrugated substrate. The cylinders can be aligned either parallel to the substrate, with their long axis being…

Soft Condensed Matter · Physics 2019-02-21 Yanyan Zhu , Karim Aissou , David Andelman , Xingkun Man

The surface properties of a substrate are among the most important parameters in the printing technology of functional materials, determining not only the printing resolution but also the stability of the printed features. This paper…

Applied Physics · Physics 2019-03-26 Aleksander Matavž , Vid Bobnar , Barbara Malič

Self-assembly of ordered nanometer-scale patterns is interesting in itself, but its practical value depends on the ability to predict and control pattern formation. In this paper we demonstrate theoretically and numerically that engineering…

Soft Condensed Matter · Physics 2020-06-30 Bjarke Frost Nielsen , Gaute Linga , Amalie Christensen , Joachim Mathiesen

The structure of lamellar phases of symmetric $AB$ diblock copolymers in a thin film is investigated. We quantitatively compare the composition profiles and profiles of individual segments in self-consistent field calculations with Monte…

Statistical Mechanics · Physics 2009-10-31 Thorsten Geisinger , Marcus Mueller , Kurt Binder

Nanocomposite materials made of block copolymer and nanoparticles display properties which can be different from the purely polymeric matrix. The resulting material is a crossover of the original properties of the block copolymer and the…

Soft Condensed Matter · Physics 2019-11-04 Javier Diaz , Marco Pinna , Andrei V. Zvelindovsky , Ignacio Pagonabarraga

The equilibrium properties of block copolymer micelles confined in polymer thin films are investigated using self-consistent field theory. The theory is based on a model system consisting of AB diblock copolymers and A homopolymers. Two…

Soft Condensed Matter · Physics 2014-01-16 Jiajia Zhou , An-Chang Shi

We study thin films of A/B diblock copolymer in a lamellar phase confined between two parallel plates (electrodes) that impose a constant voltage across the film. The weak-segregation limit is explored via a Ginzburg-Landau-like free-energy…

Soft Condensed Matter · Physics 2019-02-21 B. Zheng , X. -K. Man , Z. C. Ou-Yang , M. Schick , D. Andelman

Targeting specific technological applications requires the control of nanoparticle properties, especially the crystalline polymorph. Freezing a nanodroplet deposited on a solid substrate leads to the formation of crystalline structures. We…

Soft Condensed Matter · Physics 2018-03-02 Julien Lam , James F. Lutsko

Controlling the spatial distribution of liquid droplets on surfaces via surface energy patterning can be used to control material delivery to specified regions via selective liquid/solid wetting. While studies of the equilibrium shape of…

Soft Condensed Matter · Physics 2007-05-23 Gary S. Grest , David R. Heine , Edmund B. Webb

Two-dimensional lattices of chiral nanoholes in a plasmonic film with lattice constants being slightly larger than light wavelength are proposed for effective control of polarization and spatial properties of light beams. Effective…

Mesoscale and Nanoscale Physics · Physics 2016-03-15 V. V. Klimov , I. V. Zabkov , A. A. Pavlov , R. -C. Shiu , H. -C. Chan , G. Y. Guo

We consider the relative stability of parallel and perpendicular lamellar layers on corrugated surfaces. The model can be applied to smectic phases of liquid crystals, to lamellar phases of short-chain amphiphiles and to lamellar phases of…

Soft Condensed Matter · Physics 2009-11-10 Yoav Tsori , David Andelman

We investigated the formation of cocontinuous structures in polymer blends. These polymeric bijels (bicontinuous interfacially jammed emulsion gels) were composed of polystyrene oligomer, polybutene and fluorescent hydrophobic silica…

Soft Condensed Matter · Physics 2015-02-03 Lian Bai , John Fruehwirth , Xiang Cheng , Christopher W. Macosko

Effect of hydrophilicity of the confining walls on lamellar phases in oil-water-surfactant mixtures is studied in a slit geometry. In contrast to strongly hydrophilic or hydrophobic walls, which induce parallel orientation of lamellae, the…

Soft Condensed Matter · Physics 2007-05-23 A. Ciach , M. Tasinkevych

A mesoscopic model of a diblock copolymer is used to study the stability of a uniform lamellar phase under a reciprocating shear flow. Approximate viscosity contrast between the microphases is allowed through a linear dependence of the…

Soft Condensed Matter · Physics 2009-11-07 Peilong Chen , Jorge Vinals