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We present a detailed analysis of the fluctuation dissipation theorem (FDT) close to the glass transition in colloidal suspensions under steady shear using mode coupling approximations. Starting point is the many-particle Smoluchowski…

Soft Condensed Matter · Physics 2010-01-27 Matthias Krüger , Matthias Fuchs

A microscopic approach is presented for calculating general properties of interacting Brownian particles under steady shearing. We start from exact expressions for shear-dependent steady-state averages, such as correlation and structure…

Soft Condensed Matter · Physics 2009-07-02 Matthias Fuchs , Michael E. Cates

By means of molecular dynamics computer simulations we investigate the out of equilibrium relaxation dynamics of a simple glass former, a binary Lennard-Jones system, after a quench to low temperatures. We study both one time quantities and…

Disordered Systems and Neural Networks · Physics 2009-10-31 Walter Kob , Jean-Louis Barrat

We numerically study dynamics and correlation length scales of a colloidal liquid in both quiescent and sheared conditions to further understand the origin of slow dynamics and dynamic heterogeneity in glass-forming systems. The simulation…

Soft Condensed Matter · Physics 2015-06-05 Wen-Sheng Xu , Zhao-Yan Sun , Li-Jia An

The transient behaviour of highly concentrated colloidal liquids and dynamically arrested states (glasses) under time-dependent shear is reviewed. This includes both theoretical and experimental studies and comprises the macroscopic…

Soft Condensed Matter · Physics 2013-09-03 K J Mutch , M Laurati , C P Amann , M Fuchs , S U Egelhaaf

We analyze the behavior of supercooled fluids under shear both theoretically and numerically. Theoretically, we generalize the mode-coupling theory of supercooled fluids to systems under stationary shear flow. Our starting point is the set…

Soft Condensed Matter · Physics 2009-11-10 Kunimasa Miyazaki , David R. Reichman , Ryoichi Yamamoto

We compute the rheological properties of inelastic hard spheres in steady shear flow for general shear rates and densities. Starting from the microscopic dynamics we generalise the Integration Through Transients (\textsc{itt}) formalism to…

Soft Condensed Matter · Physics 2020-03-03 W. Till Kranz , Fabian Frahsa , Annette Zippelius , Matthias Fuchs , Matthias Sperl

We investigate stresses and particle motion during the start up of flow in a colloidal dispersion close to arrest into a glassy state. A combination of molecular dynamics simulation, mode coupling theory and confocal microscopy experiment…

Soft Condensed Matter · Physics 2009-11-13 J. Zausch , J. Horbach , M Laurati , S. U. Egelhaaf , J. M. Brader , Th. Voigtmann , M. Fuchs

We investigate a general scenario for ``glassy'' or ``jammed'' systems driven by an external, non-conservative force, analogous to a shear force in a fluid. In this scenario, the drive results in the suppression of the usual aging process,…

Soft Condensed Matter · Physics 2009-10-31 Ludovic Berthier , Jean-Louis Barrat , Jorge Kurchan

We investigate by means of molecular dynamics simulation a coarse-grained polymer glass model focusing on (quasi-static and dynamical) shear-stress fluctuations as a function of temperature T and sampling time $\Delta t$. The linear…

Soft Condensed Matter · Physics 2018-01-17 I. Kriuchevskyi , J. P. Wittmer , H. Meyer , O. Benzerara , J. Baschnagel

We consider a model dense colloidal dispersion at the glass transition, and investigate the connection between equilibrium stress fluctuations, seen in linear shear moduli, and the shear stresses under strong flow conditions far from…

Soft Condensed Matter · Physics 2009-11-13 J. J. Crassous , M. Siebenbürger , M. Ballauff , M. Drechsler , D. Hajnal , O. Henrich , M. Fuchs

We study the dynamics of a tagged particle in a glassy system under shear. The recently developed integration through transients approach based on mode coupling theory, is continued to arrive at the equations for the tagged particle…

Soft Condensed Matter · Physics 2011-07-07 Matthias Krüger , Fabian Weysser , Matthias Fuchs

The fluctuation dissipation theorem (FDT) is studied close to the glass transition in colloidal suspensions under steady shear. Shear breaks detailed balance in the many-particle Smoluchowski equation, and gives response functions in the…

Soft Condensed Matter · Physics 2009-11-13 Matthias Krüger , Matthias Fuchs

The nonlinear rheological properties of dense colloidal suspensions under steady shear are discussed within a first principles approach. It starts from the Smoluchowski equation of interacting Brownian particles in a given shear flow,…

Soft Condensed Matter · Physics 2008-10-15 Matthias Fuchs

Hydrodynamic fluctuations in simple fluids under shear flow are demonstrated to be spatially correlated, in contrast to the fluctuations at equilibrium, using mesoscopic hydrodynamic simulations. The simulation results for the equal-time…

Soft Condensed Matter · Physics 2024-06-03 Anoop Varghese , Gerhard Gompper , Roland G. Winkler

While deeply supercooled liquids exhibit divergent viscosity and increasingly heterogeneous dynamics as the temperature drops, their structure shows only seemingly marginal changes. Understanding the nature of relaxation processes in this…

Materials Science · Physics 2022-11-03 Matthias Lerbinger , Armand Barbot , Damien Vandembroucq , Sylvain Patinet

The interrelation of dynamic processes active on separated time-scales in glasses and viscous liquids is investigated using a model displaying two time-scale bifurcations both between fast and secondary relaxation and between secondary and…

Disordered Systems and Neural Networks · Physics 2015-03-19 Andrea Crisanti , Luca Leuzzi , Matteo Paoluzzi

The dynamical glass transition is typically taken to be the temperature at which a glassy liquid is no longer able to equilibrate on experimental timescales. Consequently, the physical properties of these systems just above or below the…

Soft Condensed Matter · Physics 2017-03-08 Samuel S. Schoenholz , Ekin D. Cubuk , Efthimios Kaxiras , Andrea J. Liu

We develop a nonequilibrium mode-coupling theory for uniformly sheared systems starting from microscopic, thermostatted SLLOD equations of motion. Our theory aims at describing stationary-state properties including rheological ones of…

Soft Condensed Matter · Physics 2009-11-13 Song-Ho Chong , Bongsoo Kim

We study the responses of fluid-immersed soft hydrogel spheres that are sheared under controlled volume fractions. Slippery, deformable particles along with the density-matched interstitial fluid are sandwiched between two opposing rough…

Soft Condensed Matter · Physics 2020-07-22 J. -C. Tsai , M. -R. Chou , P. -C. Huang , H. -T. Fei
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