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We investigate the tagged-particle motion in a strongly interacting quasi-confined liquid using periodic boundary conditions along the confining direction. Within a mode-coupling theory of the glass transition (MCT) we calculate the…

Soft Condensed Matter · Physics 2021-09-14 Lukas Schrack , Charlotte F. Petersen , Michele Caraglio , Gerhard Jung , Thomas Franosch

Diffusive transport of particles or, more generally, small objects is a ubiquitous feature of physical and chemical reaction systems. In configurations containing confining walls or constrictions transport is controlled both by the…

Statistical Mechanics · Physics 2009-01-22 P. Sekhar Burada , Peter Hanggi , Fabio Marchesoni , Gerhard Schmid , Peter Talkner

Little is known about the coupling of rotation and translation in dense systems. Here, we report results of confocal fluorescence microscopy where simultaneous recording of translational and rotational particle trajectories from a…

Soft Condensed Matter · Physics 2024-11-08 John Geiger , Niklas Grimm , Matthis Fuchs , Andreas Zumbusch

When captured by a flat nematic-isotropic interface, colloidal particles can be dragged by it. As a result spatially periodic structures may appear, with the period depending on a particle mass, size, and interface…

Soft Condensed Matter · Physics 2009-11-11 J. L. West , K. Zhang , A. Glushchenko , D. Andrienko , M. Tasinkevych , Y. Reznikov

The behavior of particles driven through a narrow constriction is investigated in experiment and simulation. The system of particles adapts to the confining potentials and the interaction energies by a self-consistent arrangement of the…

Soft Condensed Matter · Physics 2008-10-15 P. Henseler , A. Erbe , M. Köppl , P. Leiderer , P. Nielaba

Single particle dynamics of water confined in a nanopore is studied through Computer Molecular Dynamics. The pore is modeled to represent the average properties of a pore of Vycor glass. Dynamics is analyzed at different hydration levels…

Statistical Mechanics · Physics 2009-10-31 P. Gallo , M. Rovere , E. Spohr

Thermally induced particle flow in a charged colloidal suspension is studied in a fluid-mechanical approach. The force density acting on the charged boundary layer is derived in detail. From Stokes' equation with no-slip boundary conditions…

Soft Condensed Matter · Physics 2014-01-31 S. Fayolle , T. Bickel , A. Würger

We use confocal microscopy to directly visualize the dynamics of aging colloidal glasses. We prepare a colloidal suspension at high density, a simple model system which shares many properties with other glasses, and initiate experiments by…

Disordered Systems and Neural Networks · Physics 2009-11-07 Rachel E. Courtland , Eric R. Weeks

Dynamical heterogeneities in a colloidal fluid close to gelation are studied by means of computer simulations. A clear distinction between some fast particles and the rest, slow ones, is observed, yielding a picture of the gel composed by…

Soft Condensed Matter · Physics 2009-11-10 Antonio M. Puertas , Matthias Fuchs , Michael E. Cates

The problem of measuring nontrivial static correlations in deeply supercooled liquids made recently some progress thanks to the introduction of amorphous boundary conditions, in which a set of free particles is subject to the effect of a…

Disordered Systems and Neural Networks · Physics 2015-06-11 G. Gradenigo , R. Trozzo , A. Cavagna , T. S. Grigera , P. Verrocchio

Understanding relaxation of supercooled fluids is a major challenge and confining such systems can lead to bewildering behaviour. Here we exploit an optically confined colloidal model system in which we use reduced pressure as a control…

Soft Condensed Matter · Physics 2020-11-10 Ian Williams , Erdal C. Oğuz , Paul Bartlettl , Hartmut Löwen , C. Patrick Royall

Gels in soft-matter systems are an important nonergodic state of matter. We study a colloid-polymer mixture which is quenched by increasing the polymer concentration, from a fluid to a gel. Using confocal microscopy, we study both the…

Soft Condensed Matter · Physics 2009-04-20 Takehiro Ohtsuka , C. Patrick Royall , Hajime Tanaka

We report an experimental investigation of the caging motion in a uniformly heated granular fluid, for a wide range of filling fractions, $\phi$. At low $\phi$ the classic diffusive behavior of a fluid is observed. However, as $\phi$ is…

Soft Condensed Matter · Physics 2009-11-11 Pedro M. Reis , Rohit A. Ingale , Mark D. Shattuck

We investigate how structural relaxation in mixtures with strong dynamical asymmetry is affected by the microscopic dynamics. Brownian and Newtonian dynamics simulations of dense mixtures of fast and slow hard spheres reveal a striking…

Soft Condensed Matter · Physics 2017-10-02 Suvendu Mandal , Thomas Franosch , Thomas Voigtmann

We examine the structural and dynamic properties of confined binary hard-sphere mixtures designed to mimic realizable colloidal thin films. Using computer simulations, governed by either Newtonian or overdamped Langevin dynamics, together…

Soft Condensed Matter · Physics 2015-05-01 Jonathan A. Bollinger , Avni Jain , James Carmer , Thomas M. Truskett

We calculate the configurational entropy of colloidal particles in a confined geometry interacting as hard disks using Monte Carlo integration method. In particular, we consider systems with three kinds of boundary conditions: hard,…

Soft Condensed Matter · Physics 2023-01-23 Duanduan Wan

The slow dynamics in a glassy hard-sphere system is dominated by cage breaking events, i.e., rearrangements where a particle escapes from the cage formed by its neighboring particles. We study such events for an overdamped colloidal system…

Soft Condensed Matter · Physics 2016-10-26 Matthias Kohl , Andreas Härtel , Michael Schmiedeberg

Understanding the out-of-equilibrium properties of noisy microscale systems and the extent to which they can be modulated externally, is a crucial scientific and technological challenge. It holds the promise to unlock disruptive new…

Soft Condensed Matter · Physics 2022-09-21 Stephen Williams , Raphaël Jeanneret , Idan Tuval , Marco Polin

We analyze a dilute suspension of active particles confined between walls and subjected to fields that can modulate particle speed as well as orientation. Generally, the particle distribution is different in the bulk compared to near the…

Soft Condensed Matter · Physics 2022-08-23 Vaseem A. Shaik , Zhiwei Peng , John F. Brady , Gwynn J. Elfring

The flow of a charged-stabilized suspension through a single constricted channel is studied experimentally by tracking the particles individually. Surprisingly, the behavior is found to be qualitatively similar to that of inertial dry…

Fluid Dynamics · Physics 2018-02-14 Alvaro Marin , Henri Lhuissier , Massimiliano Rossi , Christian J. Kaehler