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Metal organic magnets have enormous potential to host a variety of electronic and magnetic phases that originate from a strong interplay between the spin, orbital and lattice degrees of freedom. We control this interplay in the quantum…

Strongly Correlated Electrons · Physics 2017-08-14 M. Skoulatos , M. Månsson , C. Fiolka , K. W. Krämer , J. Schefer , J. S. White , Ch. Rüegg

1H nuclear magnetic resonance (NMR) measurements in [YPc2]0, an organic compound formed by radicals stacking along chains, are presented. The temperature dependence of the macroscopic susceptibility, of the NMR shift and of the spin-lattice…

Strongly Correlated Electrons · Physics 2015-05-20 F. Branzoli , P. Carretta , M. Filibian , S. Klyatskaya , M. Ruben

Compounds containing magnetic subsystems representing simple model spin systems with weak magnetic coupling constants are ideal candidates to test theoretical predictions for the generic behavior close to quantum phase transitions. We…

Strongly Correlated Electrons · Physics 2010-03-16 J. Rohrkamp , M. D. Phillips , M. M. Turnbull , T. Lorenz

By means of electron spin resonance investigations we revealed the crucial role of the interchain coupling in the spin dynamics of the spin-1/2 Heisenberg antiferromagnetic (AF) chain material copper-pyrazine-dinitrate,…

Strongly Correlated Electrons · Physics 2013-01-01 A. A. Validov , M. Ozerov , J. Wosnitza , S. A. Zvyagin , M. M. Turnbull , C. P. Landee , G. B. Teitel'baum

We present experiments on the thermal transport in the spin-1/2 chain compound copper pyrazine dinitrate Cu(C_4 H_4 N_2)(NO_3)_2. The heat conductivity shows a surprisingly strong dependence on the applied magnetic field B, characterized at…

Strongly Correlated Electrons · Physics 2007-05-23 A. V. Sologubenko , K. Berggold , T. Lorenz , A. Rosch , E. Shimshoni , M. D. Phillips , M. M. Turnbull

We consider the spin-1/2 antiferromagnetic Heisenberg model on the two-dimensional square-kagome lattice with almost dispersionless lowest magnon band. For a general exchange coupling geometry we elaborate low-energy effective Hamiltonians…

Strongly Correlated Electrons · Physics 2014-09-08 Oleg Derzhko , Johannes Richter , Olesia Krupnitska , Taras Krokhmalskii

We study the dynamic spin structure factor of the spin-$1/2$ square-lattice Heisenberg antiferromagnet and of the $J$-$Q$ model (with 4-spin interactions $Q$ and Heisenberg exchange $J$). Using an improved method for stochastic analytic…

Strongly Correlated Electrons · Physics 2018-01-03 Hui Shao , Yan Qi Qin , Sylvain Capponi , Stefano Chesi , Zi Yang Meng , Anders W. Sandvik

We use numerical techniques to study dynamical properties at finite temperature ($T$) of the Heisenberg spin chain with random exchange couplings, which realizes the random singlet (RS) fixed point in the low-energy limit. Specifically, we…

Strongly Correlated Electrons · Physics 2018-04-02 Yu-Rong Shu , Maxime Dupont , Dao-Xin Yao , Sylvain Capponi , Anders W. Sandvik

We study thermodynamic behaviors of the antiferromagnetic zigzag spin chain in magnetic fields, using the density-matrix renormalization group method for the quantum transfer matrix. We focus on the thermodynamics of the system near the…

Statistical Mechanics · Physics 2009-10-31 Nobuya Maeshima , Kouichi Okunishi

We consider the easy-plane anisotropic spin-1/2 Heisenberg chain in combined uniform longitudinal and transverse staggered magnetic fields. The low-energy limit of his model is described by the sine-Gordon quantum field theory. Using…

Strongly Correlated Electrons · Physics 2009-01-06 Igor Kuzmenko , Fabian H. L. Essler

Magnetic properties of the spin-3/2 Heisenberg system Cr2BP3O12 are investigated by magnetic susceptibility chi(T) measurements, electron spin resonance, neutron diffraction, and density functional theory (DFT) calculations, as well as…

Strongly Correlated Electrons · Physics 2013-02-25 O. Janson , S. Chen , A. A. Tsirlin , S. Hoffmann , J. Sichelschmidt , Q. Huang , Z. -J. Zhang , M. -B. Tang , J. -T. Zhao , R. Kniep , H. Rosner

We consider the isotropic $S=1$ Heisenberg chain with a finite Haldane gap $\Delta$ and use state-of-the-art numerical techniques to investigate its dynamical properties at finite temperature, focusing on the nuclear spin-lattice relaxation…

Strongly Correlated Electrons · Physics 2019-09-19 Sylvain Capponi , Maxime Dupont , Anders W. Sandvik , Pinaki Sengupta

We present an experimental study of the two-dimensional S=1/2 square-lattice antiferromagnet Cu(pz)$_2$(ClO$_4$)$_2$ (pz denotes pyrazine - $C_4H_4N_2$) using specific heat measurements, neutron diffraction and cold-neutron spectroscopy.…

Strongly Correlated Electrons · Physics 2010-07-15 N. Tsyrulin , F. Xiao , A. Schneidewind , P. Link , H. M. Rønnow , J. Gavilano , C. P. Landee , M. M. Turnbull , M. Kenzelmann

By means of nuclear spin-lattice relaxation rate 1/T1, we follow the spin dynamics as a function of the applied magnetic field in two gapped one-dimensional quantum antiferromagnets: the anisotropic spin-chain system NiCl2-4SC(NH2)2 and the…

Monte Carlo and spin dynamics simulations have been used to study the dynamic critical behavior of RbMnF$_3$, treated as a classical Heisenberg antiferromagnet on a simple cubic lattice. In an attempt to understand the difference in the…

Condensed Matter · Physics 2009-11-10 Shan-Ho Tsai , D. P. Landau

Spin-1/2 Heisenberg antiferromagnetic frustrated spin chain systems display exotic ground states with unconventional excitations and distinct quantum phase transitions as the ratio of next-nearest-neighbor to nearest-neighbor coupling is…

Low-dimensional quantum magnets, due to the existence of abundant exotic quantum phases therein and experimental feasibilities in laboratories, continues intriguing people in condensed matter physics. In this work, a comprehensive study of…

Strongly Correlated Electrons · Physics 2016-07-15 Junsen Xiang , Cong Chen , Wei Li , Xianlei Sheng , Na Su , Zhaohua Cheng , Qiang Chen , Ziyu Chen

We work out the magnetization and susceptibility of Heisenberg- and XXZ-model antiferromagnet spin-1/2 systems in $D$ dimensions under a rigorous constraint of single particle site occupancy. Quantum fluctuations are taken into account up…

Strongly Correlated Electrons · Physics 2016-08-31 Raoul Dillenschneider , Jean Richert

Low-dimensional copper oxide lattices naturally manifest electronic states with strong short range quantum entanglement, which are known to lead to remarkable emergent material properties. However the nanometer scale many-body wavefunction…

Carbon-based nanostructures possessing {\pi}-electron magnetism have attracted tremendous interest due to their great potential for nano spintronics. In particular, quantum chains with magnetic molecular units synthesized by on-surface…